347 research outputs found
Picosecond X-ray Absorption Spectroscopy of Photochemical Transient Species in Solution
A photoinduced Fe(II) spin crossover reaction in solution is studied with ultrafast x-ray absorption spectroscopy. The iron-nitrogen bond lengthens by 0.21+-0.03 Angstrom in the high-spin transient excited state relative to the ground state
Does femtosecond time-resolved second-harmonic generation probe electron temperatures at surfaces?
Femtosecond pump-probe second-harmonic generation (SHG) and transient linear
reflectivity measurements were carried out on polycrystalline Cu, Ag and Au in
air to analyze whether the electron temperature affects Fresnel factors or
nonlinear susceptibilities, or both. Sensitivity to electron temperatures was
attained by using photon energies near the interband transition threshold. We
find that the nonlinear susceptibility carries the electron temperature
dependence in case of Ag and Au, while for Cu the dependence is in the Fresnel
factors. This contrasting behavior emphasizes that SHG is not a priori
sensitive to electron dynamics at surfaces or interfaces, notwithstanding its
cause.Comment: 11 pages, 4 figure
Probing impulsive strain propagation with x-ray pulses
Pump-probe time-resolved x-ray diffraction of allowed and nearly forbidden
reflections in InSb is used to follow the propagation of a coherent acoustic
pulse generated by ultrafast laser-excitation. The surface and bulk components
of the strain could be simultaneously measured due to the large x-ray
penetration depth. Comparison of the experimental data with dynamical
diffraction simulations suggests that the conventional model for impulsively
generated strain underestimates the partitioning of energy into coherent modes.Comment: 4 pages, 2 figures, LaTeX, eps. Accepted for publication in Phys.
Rev. Lett. http://prl.aps.or
Disruption of Immune Homeostasis in Human Dendritic Cells via Regulation of Autophagy and Apoptosis by
As fundamental processes of immune homeostasis, autophagy, and apoptosis must be maintained to mitigate risk of chronic inflammation and autoimmune diseases. Periodontitis is a chronic inflammatory disease characterized by oral microbial dysbiosis, and dysregulation of dendritic cell (DC) and T cell responses. The aim of this study was to elucidate the underlying mechanisms by which the oral microb
Self-energy of image states on copper surfaces
We report extensive calculations of the imaginary part of the electron
self-energy in the vicinity of the (100) and (111) surfaces of Cu. The
quasiparticle self-energy is computed by going beyond a free-electron
description of the metal surface, either within the GW approximation of
many-body theory or with inclusion, within the GW approximation, of
short-range exchange-correlation effects. Calculations of the decay rate of the
first three image states on Cu(100) and the first image state on Cu(111) are
also reported, and the impact of both band structure and many-body effects on
the electron relaxation process is discussed.Comment: 8 pages, 5 figures, to appear in Phys. Rev.
Response theory for time-resolved second-harmonic generation and two-photon photoemission
A unified response theory for the time-resolved nonlinear light generation
and two-photon photoemission (2PPE) from metal surfaces is presented. The
theory allows to describe the dependence of the nonlinear optical response and
the photoelectron yield, respectively, on the time dependence of the exciting
light field. Quantum-mechanical interference effects affect the results
significantly. Contributions to 2PPE due to the optical nonlinearity of the
surface region are derived and shown to be relevant close to a plasmon
resonance. The interplay between pulse shape, relaxation times of excited
electrons, and band structure is analyzed directly in the time domain. While
our theory works for arbitrary pulse shapes, we mainly focus on the case of two
pulses of the same mean frequency. Difficulties in extracting relaxation rates
from pump-probe experiments are discussed, for example due to the effect of
detuning of intermediate states on the interference. The theory also allows to
determine the range of validity of the optical Bloch equations and of
semiclassical rate equations, respectively. Finally, we discuss how collective
plasma excitations affect the nonlinear optical response and 2PPE.Comment: 27 pages, including 11 figures, version as publishe
Scientific Opportunities with an X-ray Free-Electron Laser Oscillator
An X-ray free-electron laser oscillator (XFELO) is a new type of hard X-ray
source that would produce fully coherent pulses with meV bandwidth and stable
intensity. The XFELO complements existing sources based on self-amplified
spontaneous emission (SASE) from high-gain X-ray free-electron lasers (XFEL)
that produce ultra-short pulses with broad-band chaotic spectra. This report is
based on discussions of scientific opportunities enabled by an XFELO during a
workshop held at SLAC on June 29 - July 1, 2016Comment: 21 pages, 12 figure
Measurement of the Bottom-Strange Meson Mixing Phase in the Full CDF Data Set
We report a measurement of the bottom-strange meson mixing phase \beta_s
using the time evolution of B0_s -> J/\psi (->\mu+\mu-) \phi (-> K+ K-) decays
in which the quark-flavor content of the bottom-strange meson is identified at
production. This measurement uses the full data set of proton-antiproton
collisions at sqrt(s)= 1.96 TeV collected by the Collider Detector experiment
at the Fermilab Tevatron, corresponding to 9.6 fb-1 of integrated luminosity.
We report confidence regions in the two-dimensional space of \beta_s and the
B0_s decay-width difference \Delta\Gamma_s, and measure \beta_s in [-\pi/2,
-1.51] U [-0.06, 0.30] U [1.26, \pi/2] at the 68% confidence level, in
agreement with the standard model expectation. Assuming the standard model
value of \beta_s, we also determine \Delta\Gamma_s = 0.068 +- 0.026 (stat) +-
0.009 (syst) ps-1 and the mean B0_s lifetime, \tau_s = 1.528 +- 0.019 (stat) +-
0.009 (syst) ps, which are consistent and competitive with determinations by
other experiments.Comment: 8 pages, 2 figures, Phys. Rev. Lett 109, 171802 (2012
- …