1,805 research outputs found

    Nanosized Sodium-Doped Lanthanum Manganites: Role of the Synthetic Route on their Physical Properties

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    In this paper we present the results of the synthesis and characterisation of nanocrystalline La1-xNaxMnO3+delta samples. Two synthetic routes were employed: polyacrylamide-based sol-gel and propellant synthesis. Pure, single phase materials were obtained with grain size around 35 nm for the sol-gel samples and around 55 nm for the propellant ones, which moreover present a more broaden grain size distribution. For both series a superparamagnetic behaviour was evidenced by means of magnetisation and EPR measurements with peculiar features ascribable to the different grain sizes and morphology. Preliminary magnetoresistivity measurements show enhanced low-field (< 1 T) magnetoresistance values which suggest an interesting applicative use of these manganites.Comment: 31 Pages 10 Figures to appear in Chem. Mate

    ĐŸĐŸŃ‚Ń€Ń–ĐčĐœĐ° ŃĐžŃŃ‚Đ”ĐŒĐ° Er-Cr-Ge

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    The isothermal section of the phase diagram of the Er–Cr–Ge ternary system was constructed at 1070 K over the whole concentration range using X-ray diffractometry, metallography and electron microprobe (EPM) analysis. The interaction between the elements in the Er−Cr−Ge system results in the formation of two ternary compounds: ErCr6Ge6 (MgFe6Ge6-type, space group P6/mmm, Pearson symbol hP13; a = 5.15149(3), c = 8.26250(7) Çș; RBragg = 0.0493, RF = 0.0574) and ErCr1-хGe2 (CeNiSi2-type, space group Cmcm, Pearson symbol oS16, a = 4.10271(5), b = 15.66525(17), c = 3.99017(4) Çș; RBragg = 0.0473, RF = 0.0433) at investigated temperature. For the ErCr1-xGe2 compound, the homogeneity region was determined (ErCr0.28-0.38Ge2; a = 4.10271(5)-4.1418(9), b = 15.6652(1)-15.7581(4), c = 3.99017(4)-3.9291(1) Çș).Đ†Đ·ĐŸŃ‚Đ”Ń€ĐŒŃ–Ń‡ĐœĐžĐč пДрДріз ĐŽŃ–Đ°ĐłŃ€Đ°ĐŒĐž ŃŃ‚Đ°ĐœŃƒ ĐżĐŸŃ‚Ń€Ń–ĐčĐœĐŸŃ— ŃĐžŃŃ‚Đ”ĐŒĐž Er–Cr–Ge ĐżĐŸĐ±ŃƒĐŽĐŸĐČĐ°ĐœĐžĐč Đ·Đ° Ń‚Đ”ĐŒĐżĐ”Ń€Đ°Ń‚ŃƒŃ€Đž 1070&nbsp;K ĐČ ĐżĐŸĐČĐœĐŸĐŒŃƒ ĐșĐŸĐœŃ†Đ”ĐœŃ‚Ń€Đ°Ń†Ń–ĐčĐœĐŸĐŒŃƒ Ń–ĐœŃ‚Đ”Ń€ĐČалі ĐŒĐ”Ń‚ĐŸĐŽĐ°ĐŒĐž Ń€Đ”ĐœŃ‚ĐłĐ”ĐœĐŸŃ„Đ°Đ·ĐŸĐČĐŸĐłĐŸ, Ń€Đ”ĐœŃ‚ĐłĐ”ĐœĐŸŃŃ‚Ń€ŃƒĐșŃ‚ŃƒŃ€ĐœĐŸĐłĐŸ і ĐŒŃ–ĐșŃ€ĐŸŃŃ‚Ń€ŃƒĐșŃ‚ŃƒŃ€ĐœĐŸĐłĐŸ Đ°ĐœĐ°Đ»Ń–Đ·Ń–ĐČ. Đ’Đ·Đ°Ń”ĐŒĐŸĐŽŃ–Ń ĐșĐŸĐŒĐżĐŸĐœĐ”ĐœŃ‚Ń–ĐČ Ńƒ ŃĐžŃŃ‚Đ”ĐŒŃ– Er–Cr–Ge Đ·Đ° Ń‚Đ”ĐŒĐżĐ”Ń€Đ°Ń‚ŃƒŃ€Đž ĐŽĐŸŃĐ»Ń–ĐŽĐ¶Đ”ĐœĐœŃ хараĐșŃ‚Đ”Ń€ĐžĐ·ŃƒŃ”Ń‚ŃŒŃŃ утĐČĐŸŃ€Đ”ĐœĐœŃĐŒ ĐŽĐČĐŸŃ… Ń‚Đ”Ń€ĐœĐ°Ń€ĐœĐžŃ… ŃĐżĐŸĐ»ŃƒĐș ErCr6Ge6 (струĐșŃ‚ŃƒŃ€ĐœĐžĐč топ MgFe6Ge6, ĐżŃ€ĐŸŃŃ‚ĐŸŃ€ĐŸĐČĐ° група P6/mmm, ŃĐžĐŒĐČĐŸĐ» ĐŸŃ–Ń€ŃĐŸĐœĐ° hP13; a = 5,15149(3), c = 8,26250(7) Çș; RBragg = 0,0493, RF = 0,0574) іErCr1-хGe2 (струĐșŃ‚ŃƒŃ€ĐœĐžĐč топ CeNiSi2, ĐżŃ€ĐŸŃŃ‚ĐŸŃ€ĐŸĐČĐ° група Cmcm, ŃĐžĐŒĐČĐŸĐ» ĐŸŃ–Ń€ŃĐŸĐœĐ° oS16, a = 4,10271(5), b = 15,6652(1), c = 3,99017(4) Çș; RBragg = 0,0473, RF = 0,0433). Đ”Đ»Ń ŃĐżĐŸĐ»ŃƒĐșĐž ErCr1-хGe2 ĐČĐžĐ·ĐœĐ°Ń‡Đ”ĐœĐ° ĐŸĐ±Đ»Đ°ŃŃ‚ŃŒ ĐłĐŸĐŒĐŸĐłĐ”ĐœĐœĐŸŃŃ‚Ń– (ErĐĄr0,28-0,38Ge2; a&nbsp;=&nbsp;4,10271(5)-4,1418(9), b&nbsp;=&nbsp;15,6652(1)-15,7581(4), c&nbsp;=&nbsp;3,99017(4)-3,9291(1)&nbsp;Çș)

    Đ†Đ·ĐŸŃ‚Đ”Ń€ĐŒŃ–Ń‡ĐœĐžĐč пДрДріз ĐżĐŸŃ‚Ń€Ń–ĐčĐœĐŸŃ— ŃĐžŃŃ‚Đ”ĐŒĐž Ho–Cu–Sn про 670 K

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    The interaction of the components in the Ho-Cu-Sn ternary system was investigated at 670 K over the whole concentration range using X-ray diffraction and EPM analyses. Four ternary compounds were formed in the Ho–Cu–Sn system at 670 K: HoCuSn (LiGaGe type, space group P63mc), Ho3Cu4Sn4 (Gd3Cu4Ge4-type, space group Immm), HoCu5Sn (CeCu5Au-type, space group Pnma), and Ho1.9Cu9.2Sn2.8 (Dy1.9Cu9.2Sn2.8-type, space group P63/mmc). The formation of the interstitial solid solution based on HoSn2 (ZrSi2-type) binary compound up to 5 at. % Cu was found.Đ’Đ·Đ°Ń”ĐŒĐŸĐŽŃ–Ń ĐșĐŸĐŒĐżĐŸĐœĐ”ĐœŃ‚Ń–ĐČ Ńƒ ĐżĐŸŃ‚Ń€Ń–ĐčĐœŃ–Đč ŃĐžŃŃ‚Đ”ĐŒŃ– Ho-Cu-Sn ĐŽĐŸŃĐ»Ń–ĐŽĐ¶Đ”ĐœĐ° Đ·Đ° Ń‚Đ”ĐŒĐżĐ”Ń€Đ°Ń‚ŃƒŃ€Đž 670 K ĐČ ĐżĐŸĐČĐœĐŸĐŒŃƒĐșĐŸĐœŃ†Đ”ĐœŃ‚Ń€Đ°Ń†Ń–ĐčĐœĐŸĐŒŃƒ Ń–ĐœŃ‚Đ”Ń€ĐČалі ĐŒĐ”Ń‚ĐŸĐŽĐ°ĐŒĐž Ń€Đ”ĐœŃ‚ĐłĐ”ĐœŃ–ĐČсьĐșĐŸŃ— ЮофраĐșції і Ń€Đ”ĐœŃ‚ĐłĐ”ĐœĐŸŃĐżĐ”ĐșŃ‚Ń€Đ°Đ»ŃŒĐœĐŸĐłĐŸ Đ°ĐœĐ°Đ»Ń–Đ·Ńƒ. Про 670K ĐČ ŃĐžŃŃ‚Đ”ĐŒŃ– утĐČĐŸŃ€ŃŽŃŽŃ‚ŃŒŃŃ Ń‡ĐŸŃ‚ĐžŃ€Đž Ń‚Đ”Ń€ĐœĐ°Ń€ĐœŃ– ŃĐżĐŸĐ»ŃƒĐșĐž: HoCuSn (струĐșŃ‚ŃƒŃ€ĐœĐžĐč топ LiGaGe, ĐżŃ€ĐŸŃŃ‚ĐŸŃ€ĐŸĐČĐ° групаP63mc), Ho3Cu4Sn4 (струĐșŃ‚ŃƒŃ€ĐœĐžĐč топ Gd3Cu4Ge4, ĐżŃ€ĐŸŃŃ‚ĐŸŃ€ĐŸĐČĐ° група Immm), HoCu5Sn (струĐșŃ‚ŃƒŃ€ĐœĐžĐč топCeCu5Au, ĐżŃ€ĐŸŃŃ‚ĐŸŃ€ĐŸĐČĐ° група Pnma) і Ho1.9Cu9.2Sn2.8 (струĐșŃ‚ŃƒŃ€ĐœĐžĐč топ Dy1.9Cu9.2Sn2.8, ĐżŃ€ĐŸŃŃ‚ĐŸŃ€ĐŸĐČĐ° групаP63/mmc). Đ’ŃŃ‚Đ°ĐœĐŸĐČĐ»Đ”ĐœĐŸ утĐČĐŸŃ€Đ”ĐœĐœŃ тĐČĐ”Ń€ĐŽĐŸĐłĐŸ Ń€ĐŸĐ·Ń‡ĐžĐœŃƒ ĐČĐșĐ»ŃŽŃ‡Đ”ĐœĐœŃ ĐœĐ° ĐŸŃĐœĐŸĐČі Đ±Ń–ĐœĐ°Ń€ĐœĐŸŃ— ŃĐżĐŸĐ»ŃƒĐșĐž HoSn2(струĐșŃ‚ŃƒŃ€ĐœĐžĐč топ ZrSi2) ĐŽĐŸ ĐČĐŒŃ–ŃŃ‚Ńƒ 5 aт. % Cu

    Đ”ĐŸŃĐ»Ń–ĐŽĐ¶Đ”ĐœĐœŃ струĐșŃ‚ŃƒŃ€ĐœĐžŃ…, ĐșŃ–ĐœĐ”Ń‚ĐžŃ‡ĐœĐžŃ… та Đ”ĐœĐ”Ń€ĐłĐ”Ń‚ĐžŃ‡ĐœĐžŃ… ĐČластОĐČĐŸŃŃ‚Đ”Đč ĐœĐ°ĐżŃ–ĐČĐżŃ€ĐŸĐČŃ–ĐŽĐœĐžĐșĐŸĐČĐŸĐłĐŸ тĐČĐ”Ń€ĐŽĐŸĐłĐŸ Ń€ĐŸĐ·Ń‡ĐžĐœŃƒ Zr1-xVxNiSn

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    Structural, electrokinetic and energy state characteristics of the Zr1-xVxNiSn semiconductive solid solution (х=0–0.10) were investigated in the temperature interval 80–400 К. It was shown that doping of the ZrNiSn compound by V atoms (rV=0.134 nm) due to substitution of Zr (rZr=0.160 nm) results in increase of lattice parameter&nbsp;Đ°(х) of Zr1-xVxNiSn indicating unforecast structural change. Based on analysis of the motion rate of the Fermi level ΔΔF/Δх&nbsp;for Zr1-xVxNiSn in direction of the conduction band it was concluded about simultaneous generation of the structural defects of the donor and acceptor nature (donor-acceptor pairs) by unknown mechanism and creation of the corresponding energy levels in the band gap of the semiconductor.Đ”ĐŸŃĐ»Ń–ĐŽĐ¶Đ”ĐœĐŸ ĐŸŃĐŸĐ±Đ»ĐžĐČĐŸŃŃ‚Ń– струĐșŃ‚ŃƒŃ€ĐœĐžŃ…, ĐșŃ–ĐœĐ”Ń‚ĐžŃ‡ĐœĐžŃ… та Đ”ĐœĐ”Ń€ĐłĐ”Ń‚ĐžŃ‡ĐœĐžŃ… хараĐșтДрОстОĐș ĐœĐ°ĐżŃ–ĐČĐżŃ€ĐŸĐČŃ–ĐŽĐœĐžĐșĐŸĐČĐŸĐłĐŸ тĐČĐ”Ń€ĐŽĐŸĐłĐŸ Ń€ĐŸĐ·Ń‡ĐžĐœŃƒ Zr1-xVxNiSn (х=0–0.10) ĐČ Ń–ĐœŃ‚Đ”Ń€ĐČалі Ń‚Đ”ĐŒĐżĐ”Ń€Đ°Ń‚ŃƒŃ€ 80–400 К. ĐŸĐŸĐșĐ°Đ·Đ°ĐœĐŸ, Ń‰ĐŸ уĐČĐ”ĐŽĐ”ĐœĐœŃ Đ°Ń‚ĐŸĐŒŃ–ĐČ V (rV=0.134 ĐœĐŒ) у струĐșтуру ŃĐżĐŸĐ»ŃƒĐșĐž ZrNiSn ŃˆĐ»ŃŃ…ĐŸĐŒ Đ·Đ°ĐŒŃ–Ń‰Đ”ĐœĐœŃ Zr (rZr=0.160 ĐœĐŒ) ŃŃƒĐżŃ€ĐŸĐČĐŸĐŽĐ¶ŃƒŃ”Ń‚ŃŒŃŃ ĐœĐ”ĐŸŃ‡Ń–ĐșуĐČĐ°ĐœĐžĐŒ Đ·Đ±Ń–Đ»ŃŒŃˆĐ”ĐœĐœŃĐŒ Đ·ĐœĐ°Ń‡Đ”ĐœŃŒ ĐżĐ”Ń€Ń–ĐŸĐŽŃƒ Đ”Đ»Đ”ĐŒĐ”ĐœŃ‚Đ°Ń€ĐœĐŸŃ— ĐșĐŸĐŒŃ–Ń€ĐșĐž&nbsp;Đ°(х) Zr1-xVxNiSn, ĐČĐșĐ°Đ·ŃƒŃŽŃ‡Đž ĐœĐ° ĐœĐ”ĐżŃ€ĐŸĐłĐœĐŸĐ·ĐŸĐČĐ°ĐœŃ– струĐșŃ‚ŃƒŃ€ĐœŃ– Đ·ĐŒŃ–ĐœĐž. На ĐŸŃĐœĐŸĐČі Đ°ĐœĐ°Đ»Ń–Đ·Ńƒ шĐČОЎĐșĐŸŃŃ‚Ń– руху ріĐČĐœŃ Đ€Đ”Ń€ĐŒŃ– ΔΔF/Δх&nbsp;Zr1-xVxNiSn у ĐœĐ°ĐżŃ€ŃĐŒŃ– Đ·ĐŸĐœĐž ĐżŃ€ĐŸĐČŃ–ĐŽĐœĐŸŃŃ‚Ń– Đ·Ń€ĐŸĐ±Đ»Đ”ĐœĐŸ ĐČĐžŃĐœĐŸĐČĐŸĐș ĐżŃ€ĐŸ ĐŸĐŽĐœĐŸŃ‡Đ°ŃĐœĐ” ĐłĐ”ĐœĐ”Ń€ŃƒĐČĐ°ĐœĐœŃ у ĐșрОсталі струĐșŃ‚ŃƒŃ€ĐœĐžŃ… ЎДфДĐșтіĐČ ĐŽĐŸĐœĐŸŃ€ĐœĐŸŃ— та Đ°ĐșŃ†Đ”ĐżŃ‚ĐŸŃ€ĐœĐŸŃ— ĐżŃ€ĐžŃ€ĐŸĐŽĐž (ĐŽĐŸĐœĐŸŃ€ĐœĐŸ-Đ°ĐșŃ†Đ”ĐżŃ‚ĐŸŃ€ĐœŃ– паро) Đ·Đ° ĐœĐ”ĐČŃ–ĐŽĐŸĐŒĐžĐŒ ĐŒĐ”Ń…Đ°ĐœŃ–Đ·ĐŒĐŸĐŒ, яĐșі ĐżĐŸŃ€ĐŸĐŽĐ¶ŃƒŃŽŃ‚ŃŒ ĐČŃ–ĐŽĐżĐŸĐČŃ–ĐŽĐœŃ– Đ”ĐœĐ”Ń€ĐłĐ”Ń‚ĐžŃ‡ĐœŃ– ріĐČĐœŃ– у Đ·Đ°Đ±ĐŸŃ€ĐŸĐœĐ”ĐœŃ–Đč Đ·ĐŸĐœŃ– ĐœĐ°ĐżŃ–ĐČĐżŃ€ĐŸĐČŃ–ĐŽĐœĐžĐș

    Peculiarities of structural, electrokinetic, energetic, and magnetic properties semiconductive solid solution Lu1-xVxNiSb

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    The structural, electrokinetic, energetic, and magnetic properties of the new semiconductive solid solution Lu1-xVxNiSb, х=0–0.10, were studied. It was shown that V atoms could simultaneously occupy different crystallographic positions in different ratios, generating structural defects of acceptor and donor nature. This creates corresponding acceptor and donor bands in the bandgap Δg of Lu1-xVxNiSb. The mechanism of the formation of two acceptor bands with different depths of occurrence has been established: a small acceptor band ΔА2, formed by defects due to the substitution of Ni atoms by V ones in the 4c position, and band ΔА1, generated by vacancies in the LuNiSb structure. The ratio of the concentrations of generated defects determines the position of the Fermi level ΔF and the conduction mechanisms. The investigated solid solution Lu1-xVxNiSb is a promising thermoelectric material

    Measurement of the cross-section and charge asymmetry of WW bosons produced in proton-proton collisions at s=8\sqrt{s}=8 TeV with the ATLAS detector

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    This paper presents measurements of the W+→Ό+ÎœW^+ \rightarrow \mu^+\nu and W−→Ό−ΜW^- \rightarrow \mu^-\nu cross-sections and the associated charge asymmetry as a function of the absolute pseudorapidity of the decay muon. The data were collected in proton--proton collisions at a centre-of-mass energy of 8 TeV with the ATLAS experiment at the LHC and correspond to a total integrated luminosity of 20.2~\mbox{fb^{-1}}. The precision of the cross-section measurements varies between 0.8% to 1.5% as a function of the pseudorapidity, excluding the 1.9% uncertainty on the integrated luminosity. The charge asymmetry is measured with an uncertainty between 0.002 and 0.003. The results are compared with predictions based on next-to-next-to-leading-order calculations with various parton distribution functions and have the sensitivity to discriminate between them.Comment: 38 pages in total, author list starting page 22, 5 figures, 4 tables, submitted to EPJC. All figures including auxiliary figures are available at https://atlas.web.cern.ch/Atlas/GROUPS/PHYSICS/PAPERS/STDM-2017-13

    Search for chargino-neutralino production with mass splittings near the electroweak scale in three-lepton final states in √s=13 TeV pp collisions with the ATLAS detector

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    A search for supersymmetry through the pair production of electroweakinos with mass splittings near the electroweak scale and decaying via on-shell W and Z bosons is presented for a three-lepton final state. The analyzed proton-proton collision data taken at a center-of-mass energy of √s=13  TeV were collected between 2015 and 2018 by the ATLAS experiment at the Large Hadron Collider, corresponding to an integrated luminosity of 139  fb−1. A search, emulating the recursive jigsaw reconstruction technique with easily reproducible laboratory-frame variables, is performed. The two excesses observed in the 2015–2016 data recursive jigsaw analysis in the low-mass three-lepton phase space are reproduced. Results with the full data set are in agreement with the Standard Model expectations. They are interpreted to set exclusion limits at the 95% confidence level on simplified models of chargino-neutralino pair production for masses up to 345 GeV

    Search for new phenomena in final states with an energetic jet and large missing transverse momentum in pp collisions at √ s = 8 TeV with the ATLAS detector

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    Results of a search for new phenomena in final states with an energetic jet and large missing transverse momentum are reported. The search uses 20.3 fb−1 of √ s = 8 TeV data collected in 2012 with the ATLAS detector at the LHC. Events are required to have at least one jet with pT > 120 GeV and no leptons. Nine signal regions are considered with increasing missing transverse momentum requirements between Emiss T > 150 GeV and Emiss T > 700 GeV. Good agreement is observed between the number of events in data and Standard Model expectations. The results are translated into exclusion limits on models with either large extra spatial dimensions, pair production of weakly interacting dark matter candidates, or production of very light gravitinos in a gauge-mediated supersymmetric model. In addition, limits on the production of an invisibly decaying Higgs-like boson leading to similar topologies in the final state are presente

    Selection of the silicon sensor thickness for the Phase-2 upgrade of the CMS Outer Tracker

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    During the operation of the CMS experiment at the High-Luminosity LHC the silicon sensors of the Phase-2 Outer Tracker will be exposed to radiation levels that could potentially deteriorate their performance. Previous studies had determined that planar float zone silicon with n-doped strips on a p-doped substrate was preferred over p-doped strips on an n-doped substrate. The last step in evaluating the optimal design for the mass production of about 200 m2^{2} of silicon sensors was to compare sensors of baseline thickness (about 300 ÎŒm) to thinned sensors (about 240 ÎŒm), which promised several benefits at high radiation levels because of the higher electric fields at the same bias voltage. This study provides a direct comparison of these two thicknesses in terms of sensor characteristics as well as charge collection and hit efficiency for fluences up to 1.5 × 1015^{15} neq_{eq}/cm2^{2}. The measurement results demonstrate that sensors with about 300 ÎŒm thickness will ensure excellent tracking performance even at the highest considered fluence levels expected for the Phase-2 Outer Tracker
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