"Synthesis and characterization of new SILVER(I) coordination polymers incorporating a BIS(TRIAZOLYL)-type ligand "

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Fragment properties of fragmenting heavy nuclei produced in central and semi-peripheral collisions

Fragment properties of hot fragmenting sources of similar sizes produced in central and semi-peripheral collisions are compared in the excitation energy range 5-10 AMeV. For semi-peripheral collisions a method for selecting compact quasi-projectiles sources in velocity space similar to those of fused systems (central collisions) is proposed. The two major results are related to collective energy. The weak radial collective energy observed for quasi-projectile sources is shown to originate from thermal pressure only. The larger fragment multiplicity observed for fused systems and their more symmetric fragmentation are related to the extra radial collective energy due to expansion following a compression phase during central collisions. A first attempt to locate where the different sources break in the phase diagram is proposed.Comment: 23 pages submitted to NP

Freeze-out volume in multifragmentation - dynamical simulations

Stochastic mean-field simulations for multifragmenting sources at the same excitation energy per nucleon have been performed. The freeze-out volume, a concept which needs to be precisely defined in this dynamical approach, was shown to increase as a function of three parameters: freeze-out instant, fragment multiplicity and system size.Comment: Submitted to Eur. Phys. J. A - march 200

Yield scaling, size hierarchy and fluctuations of observables in fragmentation of excited heavy nuclei

Multifragmentation properties measured with INDRA are studied for single sources produced in Xe+Sn reactions in the incident energy range 32-50 A MeV and quasiprojectiles from Au+Au collisions at 80 A MeV. A comparison for both types of sources is presented concerning Fisher scaling, Zipf law, fragment size and fluctuation observables. A Fisher scaling is observed for all the data. The pseudo-critical energies extracted from the Fisher scaling are consistent between Xe+Sn central collisions and Au quasi-projectiles. In the latter case it also corresponds to the energy region at which fluctuations are maximal. The critical energies deduced from the Zipf analysis are higher than those from the Fisher analysis.Comment: 30 pages, accepted for publication in Nuclear Physics A, references correcte

Multifragmentation of a very heavy nuclear system (II): bulk properties and spinodal decomposition

The properties of fragments and light charged particles emitted in multifragmentation of single sources formed in central 36AMeV Gd+U collisions are reviewed. Most of the products are isotropically distributed in the reaction c.m. Fragment kinetic energies reveal the onset of radial collective energy. A bulk effect is experimentally evidenced from the similarity of the charge distribution with that from the lighter 32AMeV Xe+Sn system. Spinodal decomposition of finite nuclear matter exhibits the same property in simulated central collisions for the two systems, and appears therefore as a possible mechanism at the origin of multifragmentation in this incident energy domain.Comment: 28 pages including 14 figures; submitted to Nucl. Phys.

Evidence for Spinodal Decomposition in Nuclear Multifragmentation

Multifragmentation of a ``fused system'' was observed for central collisions between 32 MeV/nucleon 129Xe and natSn. Most of the resulting charged products were well identified thanks to the high performances of the INDRA 4pi array. Experimental higher-order charge correlations for fragments show a weak but non ambiguous enhancement of events with nearly equal-sized fragments. Supported by dynamical calculations in which spinodal decomposition is simulated, this observed enhancement is interpreted as a ``fossil'' signal of spinodal instabilities in finite nuclear systems.Comment: 4 pages, 4 figures, to be published in Phys. Rev. Letter

Multifragmentation of a very heavy nuclear system (I): Selection of single-source events

A sample of `single-source' events, compatible with the multifragmentation of very heavy fused systems, are isolated among well-measured 155Gd+natU 36AMeV reactions by examining the evolution of the kinematics of fragments with Z>=5 as a function of the dissipated energy and loss of memory of the entrance channel. Single-source events are found to be the result of very central collisions. Such central collisions may also lead to multiple fragment emission due to the decay of excited projectile- and target-like nuclei and so-called `neck' emission, and for this reason the isolation of single-source events is very difficult. Event-selection criteria based on centrality of collisions, or on the isotropy of the emitted fragments in each event, are found to be inefficient to separate the two mechanisms, unless they take into account the redistribution of fragments' kinetic energies into directions perpendicular to the beam axis. The selected events are good candidates to look for bulk effects in the multifragmentation process.Comment: 39 pages including 15 figures; submitted to Nucl. Phys.

Source shape determination with directional fragment-fragment velocity correlations

Correlation functions, constructed from directional projections of the relative velocities of fragments, are used to determine the shape of the breakup volume in coordinate space. For central collisions of 129Xe + natSn at 50 MeV per nucleon incident energy, measured with the 4pi multi-detector INDRA at GSI, a prolate shape aligned along the beam direction with an axis ratio of 1:0.7 is deduced. The sensitivity of the method is discussed in comparison with conventional fragment-fragment velocity correlations.Comment: 12 pages, 5 figures, subm. to Phys. Lett.

Nuclear multifragmentation and phase transition for hot nuclei

This review article is focused on the tremendous progress realized during the last fifteen years in the understanding of multifragmentation and its relationship to the liquid-gas phase diagram of nuclei and nuclear matter. The explosion of the whole nucleus, early predicted by Bohr [N. Bohr, Nature 137 (1936) 351], is a very complex and rich subject which continues to fascinate nuclear physicists as well as theoreticians who extend the thermodynamics of phase transitions to finite systems