A stable, single-photon emitter in a thin organic crystal for application to quantum-photonic devices

Single organic molecules offer great promise as bright, reliable sources of identical single photons on demand, capable of integration into solid-state devices. It has been proposed that such molecules in a crystalline organic matrix might be placed close to an optical waveguide for this purpose, but so far there have been no demonstrations of sufficiently thin crystals, with a controlled concentration of suitable dopant molecules. Here we present a method for growing very thin anthracene crystals from super-saturated vapour, which produces crystals of extreme flatness and controlled thickness. We show how this crystal can be doped with a widely adjustable concentration of dibenzoterrylene (DBT) molecules and we examine the optical properties of these molecules to demonstrate their suitability as quantum emitters in nanophotonic devices. Our measurements show that the molecules are available in the crystal as single quantum emitters, with a well-defined polarisation relative to the crystal axes, making them amenable to alignment with optical nanostructures. We find that the radiative lifetime and saturation intensity vary little within the crystal and are not in any way compromised by the unusual matrix environment. We show that a large fraction of these emitters are able to deliver more than $10^{12}$ photons without photo-bleaching, making them suitable for real applications.Comment: 12 pages, 10 figures, comments welcom

Interferometric mapping of the 3.3-mm continuum emission of comet 17P/Holmes after its 2007 outburst

Comet 17P/Holmes underwent a dramatic outburst in October 2007, caused by the sudden fragmentation of its nucleus and the production of a large quantity of grains scattering sunlight. We report on 90 GHz continuum observations carried out with the IRAM Plateau de Bure interferometer on 27.1 and 28.2 October 2007 UT, i.e., 4-5 days after the outburst. These observations probed the thermal radiation of large dust particles, and therefore provide the best constraints on the mass in the ejecta debris. The thermal emission of the debris was modelled and coupled to a time-dependent description of their expansion after the outburst. The analysis was performed in the Fourier plane. Visibilities were computed for the two observing dates and compared to the data to measure their velocity and mass. Optical data and 250-GHz continuum measurements published in the literature were used to further constrain the dust kinematics and size distribution. Two distinct dust components in terms of kinematic properties are identified in the data. The large-velocity component, with typical velocities V0 of 50-100 m/s for 1 mm particles, displays a steep size distribution with a size index estimated to q = -3.7 (\pm0.1), assuming a minimum grain size of 0.1 \mum. It corresponds to the fast expanding shell observed in optical images. The slowly-moving "core" component (V0 = 7-9 m/s) detected near the nucleus has a size index |q| < 3.4 and contains a higher proportion of large particles than the shell. The dust mass in the core is in the range 0.1-1 that of the shell. Using optical constants pertaining to porous grains (50% porosity) made of astronomical silicates mixed with water ice (48% in mass), the total dust mass Mdust injected by the outburst is estimated to 4-14 x 10**11 kg, corresponding to 3-9% the nucleus mass.Comment: 15 pages with 11 figures and 7 tables. Accepted for publication in Astronomy & Astrophysic

Star formation history of galaxies from z=0 to z=0.7 A backward approach to the evolution of star-forming galaxies

We investigate whether the mean star formation activity of star-forming galaxies from z=0 to z=0.7 in the GOODS-S field can be reproduced by simple evolution models of these systems. In this case, such models might be used as first order references for studies at higher z to decipher when and to what extent a secular evolution is sufficient to explain the star formation history in galaxies. We selected star-forming galaxies at z=0 and at z=0.7 in IR and in UV to have access to all the recent star formation. We focused on galaxies with a stellar mass ranging between 10^{10} and 10^{11} M_sun for which the results are not biased by the selections. We compared the data to chemical evolution models developed for spiral galaxies and originally built to reproduce the main characteristics of the Milky Way and nearby spirals without fine-tuning them for the present analysis. We find a shallow decrease in the specific star formation rate (SSFR) when the stellar mass increases. The evolution of the SSFR characterizing both UV and IR selected galaxies from z=0 to z=0.7 is consistent with the models built to reproduce the present spiral galaxies. There is no need to strongly modify of the physical conditions in galaxies to explain the average evolution of their star formation from z=0 to z=0.7. We use the models to predict the evolution of the star formation rate and the metallicity on a wider range of redshift and we compare these predictions with the results of semi-analytical models.Comment: 14 pages, 10 figures. accepted for publication in Astronomy & Astrophysic

Chemical evolution of the Milky Way: the origin of phosphorus

Context. Recently, for the first time the abundance of P has been measured in disk stars. This provides the opportunity of comparing the observed abundances with predictions from theoretical models. Aims. We aim at predicting the chemical evolution of P in the Milky Way and compare our results with the observed P abundances in disk stars in order to put constraints on the P nucleosynthesis. Methods. To do that we adopt the two-infall model of galactic chemical evolution, which is a good model for the Milky Way, and compute the evolution of the abundances of P and Fe. We adopt stellar yields for these elements from different sources. The element P should have been formed mainly in Type II supernovae. Finally, Fe is mainly produced by Type Ia supernovae. Results. Our results confirm that to reproduce the observed trend of [P/Fe] vs. [Fe/H] in disk stars, P is formed mainly in massive stars. However, none of the available yields for P can reproduce the solar abundance of this element. In other words, to reproduce the data one should assume that massive stars produce more P than predicted by a factor of ~ 3. Conclusions. We conclude that all the available yields of P from massive stars are largely underestimated and that nucleosynthesis calculations should be revised. We also predict the [P/Fe] expected in halo stars.Comment: Accepted for publication in A&A (minor changes with respect to the submitted version

The origin of abundance gradients in the Milky Way: the predictions of different models

We aim at studying the abundance gradients along the Galactic disk and their dependence upon several parameters: a threshold in the surface gas density regulating star formation, the star formation efficiency, the timescale for the formation of the thin disk and the total surface mass density of the stellar halo. We test a model which considers a cosmological infall law. This law does not predict an inside-out disk formation, but it allows to well fit the properties of the solar vicinity. We study several cases. We find that to reproduce at the same time the abundance, star formation rate and surface gas density gradients along the Galactic disk it is necessary to assume an inside-out formation for the disk. The threshold in the gas density is not necessary and the same effect could be reached by assuming a variable star formation efficiency. A cosmologically derived infall law with an inside-out process for the disk formation and a variable star formation efficiency can indeed well reproduce all the properties of the disk. However, the cosmological model presented here does not have sufficient resolution to capture the requested inside-out formation for the disk.Comment: 13 pages, 17 figures and 2 tables. Accepted for publication in Astronomy & Astrophysic

Stellar Kinematics and Structural Properties of Virgo Cluster Dwarf Early-Type Galaxies from the SMAKCED Project. I. Kinematically Decoupled Cores and Implications for Infallen Groups in Clusters

We present evidence for kinematically decoupled cores (KDCs) in two dwarf early-type (dE) galaxies in the Virgo cluster, VCC 1183 and VCC 1453, studied as part of the SMAKCED stellar absorption-line spectroscopy and imaging survey. These KDCs have radii of 1.8'' (0.14 kpc) and 4.2'' (0.33 kpc), respectively. Each of these KDCs is distinct from the main body of its host galaxy in two ways: (1) inverted sense of rotation; and (2) younger (and possibly more metal-rich) stellar population. The observed stellar population differences are probably associated with the KDC, although we cannot rule out the possibility of intrinsic radial gradients in the host galaxy. We describe a statistical analysis method to detect, quantify the significance of, and characterize KDCs in long-slit rotation curve data. We apply this method to the two dE galaxies presented in this paper and to five other dEs for which KDCs have been reported in the literature. Among these seven dEs, there are four significant KDC detections, two marginal KDC detections, and one dE with an unusual central kinematic anomaly that may be an asymmetric KDC.The frequency of occurence of KDCs and their properties provide important constraints on the formation history of their host galaxies. We discuss different formation scenarios for these KDCs in cluster environments and find that dwarf-dwarf wet mergers or gas accretion can explain the properties of these KDCs. Both of these mechanisms require that the progenitor had a close companion with a low relative velocity. This suggests that KDCs were formed in galaxy pairs residing in a poor group environment or in isolation whose subsequent infall into the cluster quenched star formation.Comment: 14 pages, accepted for publication in Ap

The GALEX Ultraviolet Virgo Cluster Survey (GUViCS). II. Constraints on star formation in ram-pressure stripped gas

Context: Several galaxies in the Virgo cluster are known to have large HI gas tails related to a recent ram-pressure stripping event. The Virgo cluster has been extensively observed at 1539 A in the far-ultraviolet for the GALEX Ultraviolet Virgo Cluster Survey (GUViCS), and in the optical for the Next Generation Virgo Survey (NGVS), allowing a study of the stellar emission potentially associated with the gas tails of 8 cluster members. On the theoretical side, models of ram-pressure stripping events have started to include the physics of star formation. Aim: We aim to provide quantitative constraints on the amount of star formation taking place in the ram-pressure stripped gas, mainly on the basis of the far-UV emission found in the GUViCS images in relation with the gas content of the tails. Methods: We have performed three comparisons of the young stars emission with the gas column density: visual, pixel-by-pixel and global. We have compared our results to other observational and theoretical studies. Results: We find that the level of star formation taking place in the gas stripped from galaxies by ram-pressure is low with respect to the available amount of gas. Star formation is lower by at least a factor 10 compared to the predictions of the Schmidt Law as determined in regular spiral galaxy disks. It is also lower than measured in dwarfs galaxies and the outer regions of spirals, and than predicted by some numerical simulations. We provide constraints on the star formation efficiency in the ram-pressure stripped gas tails, and compare these with current models.Comment: Accepted in A&A, 17 pages (including the appendix and "on-line" figures of the paper

Hydrogen Isocyanide in Comet 73P/Schwassmann-Wachmann (Fragment B)

We present a sensitive 3-sigma upper limit of 1.1% for the HNC/HCN abundance ratio in comet 73P/Schwassmann-Wachmann (Fragment B), obtained on May 10-11, 2006 using Caltech Submillimeter Observatory (CSO). This limit is a factor of ~7 lower than the values measured previously in moderately active comets at 1 AU from the Sun. Comet 73P/Schwassmann-Wachmann was depleted in most volatile species, except of HCN. The low HNC/HCN ratio thus argues against HNC production from polymers produced from HCN. However, thermal degradation of macromolecules, or polymers, produced from ammonia and carbon compounds, such as acetylene, methane, or ethane appears a plausible explanation for the observed variations of the HNC/HCN ratio in moderately active comets, including the very low ratio in comet 73P/Schwassmann-Wachmann reported here. Similar polymers have been invoked previously to explain anomalous 14N/15N ratios measured in cometary CN.Comment: 6 pages, 5 figures, 2 table

Detection of CO and HCN in Pluto's atmosphere with ALMA

Observations of the Pluto-Charon system, acquired with the ALMA interferometer on June 12-13, 2015, have yielded a detection of the CO(3-2) and HCN(4-3) rotational transitions from Pluto, providing a strong confirmation of the presence of CO, and the first observation of HCN, in Pluto's atmosphere. The CO and HCN lines probe Pluto's atmosphere up to ~450 km and ~900 km altitude, respectively. The CO detection yields (i) a much improved determination of the CO mole fraction, as 515+/-40 ppm for a 12 ubar surface pressure (ii) clear evidence for a well-marked temperature decrease (i.e., mesosphere) above the 30-50 km stratopause and a best-determined temperature of 70+/-2 K at 300 km, in agreement with recent inferences from New Horizons / Alice solar occultation data. The HCN line shape implies a high abundance of this species in the upper atmosphere, with a mole fraction >1.5x10-5 above 450 km and a value of 4x10-5 near 800 km. The large HCN abundance and the cold upper atmosphere imply supersaturation of HCN to a degree (7-8 orders of magnitude) hitherto unseen in planetary atmospheres, probably due to the slow kinetics of condensation at the low pressure and temperature conditions of Pluto's upper atmosphere. HCN is also present in the bottom ~100 km of the atmosphere, with a 10-8 - 10-7 mole fraction; this implies either HCN saturation or undersaturation there, depending on the precise stratopause temperature. The HCN column is (1.6+/-0.4)x10^14 cm-2, suggesting a surface-referred net production rate of ~2x10^7 cm-2s-1. Although HCN rotational line cooling affects Pluto's atmosphere heat budget, the amounts determined in this study are insufficient to explain the well-marked mesosphere and upper atmosphere's ~70 K temperature. We finally report an upper limit on the HC3N column density (< 2x10^13 cm-2) and on the HC15N / HC14N ratio (< 1/125).Comment: Revised version. Icarus, in press, Oct. 11, 2016. 57 pages, including 13 figures and 4 table

Efficient excitation of dye molecules for single photon generation

A reliable photon source is required for many aspects of quantum technology. Organic molecules are attractive for this application because they can have high quantum yield and can be photostable, even at room temperature. To generate a photon with high probability, a laser must excite the molecule efficiently. We develop a simple model for that efficiency and discuss how to optimise it. We demonstrate the validity of our model through experiments on a single dibenzoterrylene (DBT) molecule in an anthracene crystal. We show that the excitation probability cannot exceed 75\% at room temperature, but can increase to over 99\% if the sample is cooled to liquid nitrogen temperature. The possibility of high photon generation efficiency with only modest cooling is a significant step towards a reliable photon source that is simple and practical.Comment: Main article (8 pages), Supplementary material (4 pages). Comments welcom