80 research outputs found

    Gradual Enhancement of Stripe-Type Antiferromagnetism in Spin Ladder Material BaFe2_2S3_3 Under Pressure

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    We report pressure-dependent neutron diffraction and muon spin relaxation/rotation measurements combined with first-principles calculations to investigate the structural, magnetic, and electronic properties of BaFe2_2S3_3 under pressure. The experimental results reveal a gradual enhancement of the stripe-type ordering temperature with increasing pressure up to 2.6 GPa and no observable change in the size of the ordered moment. The ab initio calculations suggest that the magnetism is highly sensitive to the Fe-S bond lengths and angles, clarifying discrepancies with previously published results. In contrast to our experimental observations, the calculations predict a monotonic reduction of the ordered moment with pressure. We suggest that the robustness of the stripe-type antiferromagnetism is due to strong electron correlations not fully considered in the calculations

    Extended Magnetic Dome Induced by Low Pressures in Superconducting FeSe1-x_\mathrm{1\text{-}x}Sx_\mathrm{x}

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    We report muon spin rotation (μ\muSR) and magnetization measurements under pressure on Fe1+δ_{1+\delta}Se1-x_\mathrm{1\text{-}x}Sx_\mathrm{x} with x 0.11\approx 0.11.Above p0.6p\approx0.6 GPa we find microscopic coexistence of superconductivity with an extended dome of long range magnetic order that spans a pressure range between previously reported separated magnetic phases. The magnetism initially competes on an atomic scale with the coexisting superconductivity leading to a local maximum and minimum of the superconducting Tc(p)T_\mathrm{c}(p). The maximum of TcT_\mathrm{c} corresponds to the onset of magnetism while the minimum coincides with the pressure of strongest competition. A shift of the maximum of Tc(p)T_\mathrm{c}(p) for a series of single crystals with x up to 0.14 roughly extrapolates to a putative magnetic and superconducting state at ambient pressure for x 0.2\geq0.2.Comment: 10 pages, 6 figures, including supplemental materia

    Universal fluctuating regime in triangular chromate antiferromagnets

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    We report x-ray diffraction, magnetic susceptibility, heat capacity, 1^{1}H nuclear magnetic resonance (NMR), and muon spin relaxation (μ\muSR) measurements, as well as density-functional band-structure calculations for the frustrated S=3/2S=3/2 triangular lattice Heisenberg antiferromagnet (TLHAF) α\alpha-HCrO2_{2} (trigonal, space group: R3ˉmR\bar{3}m). This compound undergoes a clear magnetic transition at TN22.5T_{\rm N} \simeq 22.5~K, as seen from the drop in the muon paramagnetic fraction and concurrent anomalies in the magnetic susceptibility and specific heat. Local probes (NMR and μ\muSR) reveal a broad regime with slow fluctuations down to 0.7TN0.7\,T_{\rm N}, this temperature corresponding to the maximum in the μ\muSR relaxation rate and in the NMR wipe-out. From the comparison with NaCrO2_{2} and α\alpha-KCrO2_{2}, the fluctuating regime and slow dynamics below TNT_{\rm N} appear to be hallmarks of the TLHAF with ABCABC stacking that leads to a frustration of interlayer couplings between the triangular planes. This interlayer frustration is a powerful lever to generate spin states with persistent dynamics and may bear implications to spin-liquid candidates with the triangular geometry.Comment: 14 pages, 11 figures, 2 table

    Disordered ground state in the spin-orbit coupled Jeff = 1/2 distorted honeycomb magnet BiYbGeO5

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    We delineate quantum magnetism in the strongly spin-orbit coupled distorted honeycomb lattice antiferromagnet BiYbGeO5. Our magnetization and heat capacity measurements reveal that its low-temperature behavior is well described by an effective Jeff=12 Kramers doublet of Yb3+. The ground state is nonmagnetic with a tiny spin gap. Temperature-dependent magnetic susceptibility, magnetization isotherm, and heat capacity can be modeled well assuming isolated spin dimers with anisotropic exchange interactions JZ≃2.6 K and JXY≃1.3 K. Heat capacity measurements backed by muon spin relaxation suggest the absence of magnetic long-range order down to at least 80 mK both in zero field and in applied fields. This sets BiYbGeO5 apart from Yb2Si2O7, with its unusual regime of magnon Bose-Einstein condensation, and suggests negligible interdimer couplings, despite only a weak structural deformation of the honeycomb lattice

    Robust block magnetism in the spin ladder compound BaFe2_2Se3_3 under hydrostatic pressure

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    The majority of the iron-based superconductors (FeSCs) exhibit a two-dimensional square lattice structure. Recent reports of pressure-induced superconductivity in the spin-ladder system, BaFe2_2X3_3 (X =S,Se), introduce a quasi-one-dimensional prototype and an insulating parent compound to the FeSCs. Here we report X-ray, neutron diffraction and muon spin relaxation experiments on BaFe2_2Se3_3 under hydrostatic pressure to investigate its magnetic and structural properties across the pressure-temperature phase diagram. A structural phase transition was identified at a pressure of 3.7(3) GPa. Neutron diffraction measurements at 6.8(3) GPa and 120 K show that the block magnetism persists even at these high pressures. A steady increase and then fast drop of the magnetic transition temperature TNT\rm_N and greatly reduced moment above the pressure PsP_s indicate potentially rich and competing phases close to the superconducting phase in this ladder system

    Antimicrobial resistance among migrants in Europe: a systematic review and meta-analysis

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    BACKGROUND: Rates of antimicrobial resistance (AMR) are rising globally and there is concern that increased migration is contributing to the burden of antibiotic resistance in Europe. However, the effect of migration on the burden of AMR in Europe has not yet been comprehensively examined. Therefore, we did a systematic review and meta-analysis to identify and synthesise data for AMR carriage or infection in migrants to Europe to examine differences in patterns of AMR across migrant groups and in different settings. METHODS: For this systematic review and meta-analysis, we searched MEDLINE, Embase, PubMed, and Scopus with no language restrictions from Jan 1, 2000, to Jan 18, 2017, for primary data from observational studies reporting antibacterial resistance in common bacterial pathogens among migrants to 21 European Union-15 and European Economic Area countries. To be eligible for inclusion, studies had to report data on carriage or infection with laboratory-confirmed antibiotic-resistant organisms in migrant populations. We extracted data from eligible studies and assessed quality using piloted, standardised forms. We did not examine drug resistance in tuberculosis and excluded articles solely reporting on this parameter. We also excluded articles in which migrant status was determined by ethnicity, country of birth of participants' parents, or was not defined, and articles in which data were not disaggregated by migrant status. Outcomes were carriage of or infection with antibiotic-resistant organisms. We used random-effects models to calculate the pooled prevalence of each outcome. The study protocol is registered with PROSPERO, number CRD42016043681. FINDINGS: We identified 2274 articles, of which 23 observational studies reporting on antibiotic resistance in 2319 migrants were included. The pooled prevalence of any AMR carriage or AMR infection in migrants was 25·4% (95% CI 19·1-31·8; I2 =98%), including meticillin-resistant Staphylococcus aureus (7·8%, 4·8-10·7; I2 =92%) and antibiotic-resistant Gram-negative bacteria (27·2%, 17·6-36·8; I2 =94%). The pooled prevalence of any AMR carriage or infection was higher in refugees and asylum seekers (33·0%, 18·3-47·6; I2 =98%) than in other migrant groups (6·6%, 1·8-11·3; I2 =92%). The pooled prevalence of antibiotic-resistant organisms was slightly higher in high-migrant community settings (33·1%, 11·1-55·1; I2 =96%) than in migrants in hospitals (24·3%, 16·1-32·6; I2 =98%). We did not find evidence of high rates of transmission of AMR from migrant to host populations. INTERPRETATION: Migrants are exposed to conditions favouring the emergence of drug resistance during transit and in host countries in Europe. Increased antibiotic resistance among refugees and asylum seekers and in high-migrant community settings (such as refugee camps and detention facilities) highlights the need for improved living conditions, access to health care, and initiatives to facilitate detection of and appropriate high-quality treatment for antibiotic-resistant infections during transit and in host countries. Protocols for the prevention and control of infection and for antibiotic surveillance need to be integrated in all aspects of health care, which should be accessible for all migrant groups, and should target determinants of AMR before, during, and after migration. FUNDING: UK National Institute for Health Research Imperial Biomedical Research Centre, Imperial College Healthcare Charity, the Wellcome Trust, and UK National Institute for Health Research Health Protection Research Unit in Healthcare-associated Infections and Antimictobial Resistance at Imperial College London
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