Strong coupling between excitons in transition metal dichalcogenides and optical bound states in the continuum

Being motivated by recent achievements in the rapidly developing fields of optical bound states in the continuum (BICs) and excitons in monolayers of transition metal dichalcogenides, we analyze strong coupling between BICs in Ta 2 O 5 periodic photonic structures and excitons in WSe 2 monolayers. We demonstrate that giant radiative lifetime of BICs allows to engineer the exciton-polariton lifetime enhancing it three orders of magnitude compared to a bare exciton. We show that maximal lifetime of hybrid light-matter state can be achieved at any point of k-space by shaping the geometry of the photonic structure.This work was supported by the Russian Foundation for Basic Research (16-37-60064, 17-02- 01234), the Ministry of Education and Science of the Russian Federation (3.1668.2017/4.6), the President of Rus- sian Federation (MK-403.2018.2

Bound states in the continuum and Fano resonances in the strong mode coupling regime

The study of resonant dielectric nanostructures with a high refractive index is a new research direction in the nanoscale optics and metamaterial-inspired nanophotonics. Because of the unique optically induced electric and magnetic Mie resonances, high-index nanoscale structures are expected to complement or even replace different plasmonic components in a range of potential applications. We study a strong coupling between modes of a single subwavelength high-index dielectric resonator and analyze the mode transformation and Fano resonances when the resonator’s aspect ratio varies. We demonstrate that strong mode coupling results in resonances with high-quality factors, which are related to the physics of bound states in the continuum when the radiative losses are almost suppressed due to the Friedrich–Wintgen scenario of destructive interference. We explain the physics of these states in terms of multipole decomposition, and show that their appearance is accompanied by a drastic change in the far-field radiation pattern. We reveal a fundamental link between the formation of the high-quality resonances and peculiarities of the Fano parameter in the scattering cross-section spectra. Our theoretical findings are confirmed by microwave experiments for the scattering of high-index cylindrical resonators with a tunable aspect ratio. The proposed mechanism of the strong mode coupling in single subwavelength high-index resonators accompanied by resonances with high-quality factors helps to extend substantially functionalities of all-dielectric nanophotonics, which opens horizons for active and passive nanoscale metadevices.The numerical calculations were performed with support from the Ministry of Education and Science of the Russian Federation (Project 3.1500.2017/4.6) and the Australian Research Council. The experimental study of the cylinder SCS in the microwave frequency range was supported by the Russian Science Foundation (17-79-20379). The analytical calculations with resonant-state expansion method were performed with support from the Russian Science Foundation (17-12-01581). A. A. B., K. L. K. and Z. F. S. acknowledge support from the Foundation for the Advancement of Theoretical Physics and Mathematics “BASIS” (Russia)

Light-matter interaction between photonic bound states in the continuum and bright excitons in transition metal dichalcogenides

Being motivated by recent achievements in the rapidly developing fields of optical bound states in the continuum (BICs) and excitons in monolayers of transition metal dichalcogenides, we analyze strong coupling between BICs in Ta2O5 periodic photonic structures and excitons in WSe2 monolayers. We demonstrate that giant radiative lifetime of BICs allow to engineer the exciton-polariton lifetime enhancing it three orders of magnitude compared to a bare exciton.The work has been supported by the Ministry of Education and Science of the Russian Federation (3.1668.2017/4.6), the Russian Foundation for Basic Research (16-37-60064) and the President of Russian Federation (Grant MK-403.2018.2)

Formation of Gold Nanoparticle Self-Assembling Films in Various Polymer Matrices for SERS Substrates

Surface-enhanced Raman spectroscopy (SERS) is regarded as a versatile tool for studying the composition and structure of matter. This work has studied the preparation of a SERS substrate based on a self-assembling plasmonic nanoparticle film (SPF) in a polymer matrix. Several synthesis parameters for the SPF are investigated, including the size of the particles making up the film and the concentration and type of the self-assembling agent. The result of testing systems with different characteristics is discussed using a model substance (pseudo isocyaniniodide). These models can be useful in the study of biology and chemistry. Research results contain the optimal parameters for SPF synthesis, maximizing the SERS signal. The optimal procedure for SPF assembly is determined and used for the synthesis of composite SPFs within different polymer matrices. SPF in a polymer matrix is necessary for the routine use of the SERS substrate for various types of analytes, including solid samples or those sensitive to contamination. Polystyrene, polyvinyl alcohol (PVA), and polyethylene are investigated to obtain a polymer matrix for SPF, and various methods of incorporating SPF into a polymer matrix are being explored. It is found that films with the best signal enhancement and reproducibility were obtained in polystyrene. The minimum detectable concentration for the SERS substrate obtained is equal to 10 10 M We prepared a SERS substrate with an analytical enhancement factor of 2.7 104, allowing an increase in the detection sensitivity of analyte solutions of five orders of magnitude

Centrality evolution of the charged-particle pseudorapidity density over a broad pseudorapidity range in Pb-Pb collisions at root s(NN)=2.76TeV

Peer reviewe

High-Q resonances with low azimuthal indices in all-dielectric high-index nanoparticles

Recently, a novel class of high-Q optical resonators based on all-dielectric subwavelength nanoparticles with high refractive index has been proposed [M. V. Rybin, et al, arXiv:1706.02099, 2017]. Here we study a complex spectrum of such nanoscale resonators by means of the resonant-state expansion, treating the problem as a nonHermitian eigenproblem. We show that the high-Q features can be described within the mechanism of external coupling of open channels via the continuum. For ceramic resonators with permittivity = 40, we demonstrate that the quality factor of a trapped mode with a low azimuthal index could reach the value Q = 104.This work has been supported by the Ministry of Education and Science of the Russian Federation (3.1668.2017/4.6) and the Russian Foundation for Basic Research (16-02-00461, 16-37-60064, 17-02-01234)

Effect of Reactive Ion Etching on the Luminescence of GeV Color Centers in CVD Diamond Nanocrystals

The negatively charged germanium-vacancy GeV− color centers in diamond nanocrystals are solid-state photon emitters suited for quantum information technologies, bio-sensing, and labeling applications. Due to the small Huang–Rhys factor, the GeV−-center zero-phonon line emission is expected to be very intensive and spectrally narrow. However, structural defects and the inhomogeneous distribution of local strains in the nanodiamonds result in the essential broadening of the ZPL. Therefore, clarification and elimination of the reasons for the broadening of the GeV− center ZPL is an important problem. We report on the effect of reactive ion etching in oxygen plasma on the structure and luminescence properties of nanodiamonds grown by hot filament chemical vapor deposition. Emission of GeV− color centers ensembles at about 602 nm in as-grown and etched nanodiamonds is probed using micro-photoluminescence and micro-Raman spectroscopy at room and liquid nitrogen temperature. We show that the etching removes the nanodiamond surface sp2-induced defects resulting in a reduction in the broad luminescence background and a narrowing of the diamond Raman band. The zero-phonon luminescence band of the ensemble of the GeV− centers is a superposition of narrow lines originated most likely from the GeV− center sub-ensembles under different uniaxial local strain conditions

Duo Emission of CVD Nanodiamonds Doped by SiV and GeV Color Centers: Effects of Growth Conditions

The investigation of the hot filament chemical vapor deposition nanodiamonds with simultaneously embedded luminescent GeV− and SiV− color centers from solid sources showed that both the absolute and relative intensities of their zero-phonon lines (at 602 and 738 nm) depend on nanodiamond growth conditions (a methane concentration in the CH4/H2 gas mixture, growth temperature, and time). It is shown that a controlled choice of parameters of hot filament chemical vapor deposition synthesis makes it possible to select the optimal synthesis conditions for tailoring bicolor fluorescence nanodiamond labels for imaging biological systems