Aerosol indirect effect in the thermal spectral range as seen from satellites

Insufficient knowledge about aerosol-cloud interactions has caused uncertainty in the Earth Radiation Budget. Lack of information about aerosol type, composition and concentration on global and regional scales also has restrained numerous efforts that have been made in the past to quantify the modulation of cloud properties by aerosols. Clouds, which cover more than half of the earth at any given time, have a key role in radiation budget. Most of the work has been done so far to understand modulation of cloud microphysical properties (invisible spectrum) by aerosols neglecting the thermal part. Satellites play unique role in improving knowledge about aerosol-cloud interactions through their ability to quantify spectral signatures of clouds and uniform, continuous sampling of the earth. Using long-term satellite data evaluations, this study reveals an entirely new aspect of these interactions and suggests that there exists indirect aerosol effect in the thermal spectrum. It suggests that anthropogenic aerosols, finer particles in particular, and cloud top temperature covary. This thermal effect could be equally important and hence cannot be neglected in radiation budget studies. First evidence of the impact of ship emissions on cloud properties over coastal waters is also presented

Impact of ship emissions on cloud properties over coastal areas

Although land based emissions in Europe are decreasing, ship emissions continue to grow. The main emissions from ships can modulate cloud properties of coastal areas and are of direct relevance to the earth radiation budget. In this context, satellite data from AVHRR onboard NOAA-14 are evaluated for six years (1997–02) in order to assess impact of ship emissions on cloud properties over coastal areas. Study area was chosen in such a way that it includes the English Channel and top three polluting harbours in Europe. Results present first evidence of possible impact of ship emissions on both cloud albedo and cloud top temperature over coastal areas using long-term satellite measurements. Increase in cloud albedo (with corresponding decrease in cloud top temperature) and higher variability are observed over coastal areas. This effect is more pronounced for areas over and around harbours and the English Channel. It also confirms indirect aerosol effects

Stratospheric aerosol - Observations, processes, and impact on climate

Interest in stratospheric aerosol and its role in climate have increased over the last decade due to the observed increase in stratospheric aerosol since 2000 and the potential for changes in the sulfur cycle induced by climate change. This review provides an overview about the advances in stratospheric aerosol research since the last comprehensive assessment of stratospheric aerosol was published in 2006. A crucial development since 2006 is the substantial improvement in the agreement between in situ and space-based inferences of stratospheric aerosol properties during volcanically quiescent periods. Furthermore, new measurement systems and techniques, both in situ and space based, have been developed for measuring physical aerosol properties with greater accuracy and for characterizing aerosol composition. However, these changes induce challenges to constructing a long-term stratospheric aerosol climatology. Currently, changes in stratospheric aerosol levels less than 20% cannot be confidently quantified. The volcanic signals tend to mask any nonvolcanically driven change, making them difficult to understand. While the role of carbonyl sulfide as a substantial and relatively constant source of stratospheric sulfur has been confirmed by new observations and model simulations, large uncertainties remain with respect to the contribution from anthropogenic sulfur dioxide emissions. New evidence has been provided that stratospheric aerosol can also contain small amounts of nonsulfate matter such as black carbon and organics. Chemistry-climate models have substantially increased in quantity and sophistication. In many models the implementation of stratospheric aerosol processes is coupled to radiation and/or stratospheric chemistry modules to account for relevant feedback processes

Black carbon fractal morphology and short-wave radiative impact: a modelling study

We investigate the impact of the morphological properties of freshly emitted black carbon aerosols on optical properties and on radiative forcing. To this end, we model the optical properties of fractal black carbon aggregates by use of numerically exact solutions to Maxwell's equations within a spectral range from the UVC to the mid-IR. The results are coupled to radiative transfer computations, in which we consider six realistic case studies representing different atmospheric pollution conditions and surface albedos. The spectrally integrated radiative impacts of black carbon are compared for two different fractal morphologies, which brace the range of recently reported experimental observations of black carbon fractal structures. We also gauge our results by performing corresponding calculations based on the homogeneous sphere approximation, which is commonly employed in climate models. We find that at top of atmosphere the aggregate models yield radiative impacts that can be as much as 2 times higher than those based on the homogeneous sphere approximation. An aggregate model with a low fractal dimension can predict a radiative impact that is higher than that obtained with a high fractal dimension by a factor ranging between 1.1–1.6. Although the lower end of this scale seems like a rather small effect, a closer analysis reveals that the single scattering optical properties of more compact and more lacy aggregates differ considerably. In radiative flux computations there can be a partial cancellation due to the opposing effects of different error sources. However, this cancellation effect can strongly depend on atmospheric conditions and is therefore quite unpredictable. We conclude that the fractal morphology of black carbon aerosols and their fractal parameters can have a profound impact on their radiative forcing effect, and that the use of the homogeneous sphere model introduces unacceptably high biases in radiative impact studies. We emphasise that there are other potentially important morphological features that have not been addressed in the present study, such as sintering and coating of freshly emitted black carbon by films of organic material. Finally, we found that the spectral variation of the absorption cross section of black carbon significantly deviates from a simple 1/λ scaling law. We therefore discourage the use of single-wavelength absorption measurements in conjunction with a 1/λ scaling relation in broadband radiative forcing simulations of black carbon

Dependence of frequency of convective cloud occurrence on the orbital drift of satellites

Deriving accurate time-series of cloud cover from satellite sensor data still remains a challenging task. The instruments onboard polar orbiting NOAA satellites offer the opportunity to prepare cloud climatology on a global scale; however, the orbital drifts of these satellites can introduce uncertainty when deriving such cloud climatology. The aim of this letter is to point out the importance and to estimate the impact of orbital drift on long-term time-series of the observation of convective cloud frequency of occurrence. The 20 years of daytime AVHRR data from over the Indian subcontinent for the summer monsoon season is used in this study. All four AVHRRs onboard NOAA-7, -9, -11, and -14 satellites show positive correlation between increased cloud frequency and the delay in equator crossing-times during their lifetime. This increase is significant over land, but over the ocean, there is no discernible effect. This effect should be considered to avoid spurious trends in cloud cover. Further in-depth investigations are needed to make possible corrections. [References: 17

Change in cloud-top temperatures over Europe

Long-term measurements from Advanced Very High Resolution Radtiometer (AVHRR) onboard the National Oceanic and Atmospheric Administration satellites were evaluated to assess variability in cloud-top temperatures over central and eastern Europe that saw radical infrastructural changes after the fall of the East Bloc in 1989 that has affected the pollution levels and hence cloud albedo. Four years in the late 1980s (1985-1988) and in the late 1990s (1997-2000) were chosen, as these are distinctively marked as episodes of very high and lower air pollution (sulphates and particulate matter). During the late 1980s, low- and medium-level clouds were colder by more than 2 K and convective clouds even by 4 K. Cloud-tops over and around polluted regions are higher, and their temperatures showed stronger variability, suggesting an indirect aerosol effect in the thermal spectral range as well

Correcting orbital drift signal in the time series of AVHRR derived convective cloud fraction using rotated empirical orthogonal function

The Advanced Very High Resolution Radiometer (AVHRR) instruments onboard the series of National Oceanic and Atmospheric Administration (NOAA) satellites offer the longest available meteorological data records from space. These satellites have drifted in orbit resulting in shifts in the local time sampling during the life span of the sensors onboard. Depending upon the amplitude of the diurnal cycle of the geophysical parameters derived, orbital drift may cause spurious trends in their time series. We investigate tropical deep convective clouds, which show pronounced diurnal cycle amplitude, to estimate an upper bound of the impact of orbital drift on their time series. We carry out a rotated empirical orthogonal function analysis (REOF) and show that the REOFs are useful in delineating orbital drift signal and, more importantly, in subtracting this signal in the time series of convective cloud amount. These results will help facilitate the derivation of homogenized data series of cloud amount from NOAA satellite sensors and ultimately analyzing trends from them. However, we suggest detailed comparison of various methods and rigorous testing thereof applying final orbital drift corrections