120 research outputs found
Electron-nuclei spin dynamics in II-VI semiconductor quantum dots
We report on the dynamics of optically induced nuclear spin polarization in
individual CdTe/ZnTe quantum dots loaded with one electron by modulation
doping. The fine structure of the hot trion (charged exciton with an
electron in the -shell) is identified in photoluminescence excitation
spectra. A negative polarisation rate of the photoluminescence, optical pumping
of the resident electron and the built-up of dynamic nuclear spin polarisation
(DNSP) are observed in time-resolved optical pumping experiments when the
quantum dot is excited at higher energy than the hot trion triplet state. The
time and magnetic field dependence of the polarisation rate of the
emission allows to probe the dynamics of formation of the DNSP in the optical
pumping regime. We demonstrate using time-resolved measurements that the
creation of a DNSP at B=0T efficiently prevents longitudinal spin relaxation of
the electron caused by fluctuations of the nuclear spin bath. The DNSP is built
in the microsecond range at high excitation intensity. A relaxation time of the
DNSP in about 10 microseconds is observed at and significantly increases
under a magnetic field of a few milli-Tesla. We discuss mechanisms responsible
for the fast initialisation and relaxation of the diluted nuclear spins in this
system
Phase diagrams of magnetopolariton gases
The magnetic field effect on phase transitions in electrically neutral
bosonic systems is much less studied than those in fermionic systems, such as
superconducting or ferromagnetic phase transitions. Nevertheless, composite
bosons are strongly sensitive to magnetic fields: both their internal structure
and motion as whole particles may be affected. A joint effort of ten
laboratories has been focused on studies of polariton lasers, where
non-equilibrium Bose-Einstein condensates of bosonic quasiparticles,
exciton-polaritons, may appear or disappear under an effect of applied magnetic
fields. Polariton lasers based on pillar or planar microcavities were excited
both optically and electrically. In all cases a pronounced dependence of the
onset to lasing on the magnetic field has been observed. For the sake of
comparison, photon lasing (lasing by an electron-hole plasma) in the presence
of a magnetic field has been studied on the same samples as polariton lasing.
The threshold to photon lasing is essentially governed by the excitonic Mott
transition which appears to be sensitive to magnetic fields too. All the
observed experimental features are qualitatively described within a uniform
model based on coupled diffusion equations for electrons, holes and excitons
and the Gross-Pitaevskii equation for exciton-polariton condensates. Our
research sheds more light on the physics of non-equilibrium Bose-Einstein
condensates and the results manifest high potentiality of polariton lasers for
spin-based quantum logic applications.Comment: 21 pages, 11 figure
Picosecond Nonlinear Relaxation of Photoinjected Carriers in a Single GaAs/AlGaAs Quantum Dot
Photoemission from a single self-organized GaAs/AlGaAs quantum dot (QD) is
temporally resolved with picosecond time resolution. The emission spectra
consisting of the multiexciton structures are observed to depend on the delay
time and the excitation intensity. Quantitative agreement is found between the
experimental data and the calculation based on a model which characterizes the
successive relaxation of multiexcitons. Through the analysis we can determine
the carrier relaxation time as a function of population of photoinjected
carriers. Enhancement of the intra-dot carrier relaxation is demonstrated to be
due to the carrier-carrier scattering inside a single QD.Comment: 4 pages, 4 figures, to be published in Phys. Rev. B, Rapid
Polarized emission of GaN/AlN quantum dots : single dot spectroscopy and symmetry-based theory
We report micro-photoluminescence studies of single GaN/AlN quantum dots
grown along the (0001) crystal axis by molecular beam epitaxy on Si(111)
substrates. The emission lines exhibit a linear polarization along the growth
plane, but with varying magnitudes of the polarization degree and with
principal polarization axes that do not necessarily correspond to
crystallographic directions. Moreover, we could not observe any splitting of
polarized emission lines, at least within the spectral resolution of our setup
(1 meV). We propose a model based on the joint effects of electron-hole
exchange interaction and in-plane anisotropy of strain and/or quantum dot
shape, in order to explain the quantitative differences between our
observations and those previously reported on, e.g. CdTe- or InAs-based quantum
dots
Evaluation of the density and absorption properties of generated organonitrate particles (pON)
Evaluation of receptor and chemical transport models for PM10 source apportionment
In this study, the performance of two types of source apportionment models was evaluated by assessing the results provided by 40 different groups in the framework of an intercomparison organised by FAIRMODE WG3 (Forum for air quality modelling in Europe, Working Group 3). The evaluation was based on two performance indicators: z-scores and the root mean square error weighted by the reference uncertainty (RMSEu), with pre-established acceptability criteria. By involving models based on completely different and independent input data, such as receptor models (RMs) and chemical transport models (CTMs), the intercomparison provided a unique opportunity for their cross-validation. In addition, comparing the CTM chemical profiles with those measured directly at the source contributed to corroborate the consistency of the tested model results. The most commonly used RM was the US EPA- PMF version 5. RMs showed very good performance for the overall dataset (91% of z-scores accepted) while more difficulties were observed with the source contribution time series (72% of RMSEu accepted). Industrial activities proved to be the most difficult sources to be quantified by RMs, with high variability in the estimated contributions. In the CTMs, the sum of computed source contributions was lower than the measured gravimetric PM10 mass concentrations. The performance tests pointed out the differences between the two CTM approaches used for source apportionment in this study: brute force (or emission reduction impact) and tagged species methods. The sources meeting the z-score and RMSEu acceptability criteria tests were 50% and 86%, respectively. The CTM source contributions to PM10 were in the majority of cases lower than the RM averages for the corresponding source. The CTMs and RMs source contributions for the overall dataset were more comparable (83% of the z-scores accepted) than their time series (successful RMSEu in the range 25% - 34%). The comparability between CTMs and RMs varied depending on the source: traffic/exhaust and industry were the source categories with the best results in the RMSEu tests while the most critical ones were soil dust and road dust. The differences between RMs and CTMs source reconstructions confirmed the importance of cross validating the results of these two families of models
Unbound states in quantum heterostructures
We report in this review on the electronic continuum states of semiconductor Quantum Wells and Quantum Dots and highlight the decisive part played by the virtual bound states in the optical properties of these structures. The two particles continuum states of Quantum Dots control the decoherence of the excited electron â hole states. The part played by Auger scattering in Quantum Dots is also discussed
Polarization-dependent Rabi oscillations in single InGaAs quantum dots
Measurements of optical Rabi oscillations in the excited states of individual InGaAs are presented. Under pulsed resonant excitation we observe Rabi oscillations with increasing pulse area, which are damped after the first maximum and minimum. We show that the observed damping comes from an additional non-resonant generation of carriers in the quantum dot. The observation of Rabi oscillations provides an efficient way of directly measuring the excitonic transitions' dipole moments. A polarization anisotropy of the dipole moment is resolved in some of the quantum dots
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