Phonon Density of States and Anharmonicity of UO2

Phonon density of states (PDOS) measurements have been performed on polycrystalline UO2 at 295 and 1200 K using time-of-flight inelastic neutron scattering to investigate the impact of anharmonicity on the vibrational spectra and to benchmark ab initio PDOS simulations performed on this strongly correlated Mott-insulator. Time-of-flight PDOS measurements include anharmonic linewidth broadening inherently and the factor of ~ 7 enhancement of the oxygen spectrum relative to the uranium component by the neutron weighting increases sensitivity to the oxygen-dominated optical phonon modes. The first-principles simulations of quasi-harmonic PDOS spectra were neutron-weighted and anharmonicity was introduced in an approximate way by convolution with wavevector-weighted averages over our previously measured phonon linewidths for UO2 that are provided in numerical form. Comparisons between the PDOS measurements and the simulations show reasonable agreement overall, but they also reveal important areas of disagreement for both high and low temperatures. The discrepancies stem largely from an ~ 10 meV compression in the overall bandwidth (energy range) of the oxygen-dominated optical phonons in the simulations. A similar linewidth-convoluted comparison performed with the PDOS spectrum of Dolling et al. obtained by shell-model fitting to their historical phonon dispersion measurements shows excellent agreement with the time-of-flight PDOS measurements reported here. In contrast, we show by comparisons of spectra in linewidth-convoluted form that recent first-principles simulations for UO2 fail to account for the PDOS spectrum determined from the measurements of Dolling et al. These results demonstrate PDOS measurements to be stringent tests for ab initio simulations of phonon physics in UO2 and they indicate further the need for advances in theory to address lattice dynamics of UO2.Comment: Text slightly modified, results unchange

Large Scale Traces of Solar System Cold Dust on CMB Anisotropies

We explore the microwave anisotropies at large angular scales produced by the emission from cold and large dust grains, expected to exist in the outer parts of the Solar System, using a simple toy model for this diuse emission. Its amplitude is constrained in the Far-IR by the COBE data and is compatible with simulations found in the literature. We analyze the templates derived after subtracting our model from the WMAP ILC 7 yr maps and investigate on the cosmological implications of such a possible foreground. The anomalies related to the low quadrupole of the angular power spectrum, the two-point correlation function, the parity and the excess of signal found in the ecliptic plane are significantly alleviated. An impact of this foreground for some cosmological parameters characterizing the spectrum of primordial density perturbations, relevant for on-going and future CMB anisotropy experiments, is found.Comment: Issue 2.0, Accepted for pub. in MNRAS, Apr 8th, 2011, (sub. Oct 4th, 2010); 10 pages, 6 Figures, 1 table; pdflatex with mn2e, AMS, natbib, txfonts, graphic

Seven-Year Wilkinson Microwave Anisotropy Probe (WMAP) Observations: Power Spectra and WMAP-Derived Parameters

(Abridged) We present the angular power spectra derived from the 7-year maps and discuss the cosmological conclusions that can be inferred from WMAP data alone. The third acoustic peak in the TT spectrum is now well measured by WMAP. In the context of a flat LambdaCDM model, this improvement allows us to place tighter constraints on the matter density from WMAP data alone, and on the epoch of matter-radiation equality, The temperature-polarization (TE) spectrum is detected in the 7-year data with a significance of 20 sigma, compared to 13 sigma with the 5-year data. The low-l EE spectrum, a measure of the optical depth due to reionization, is detected at 5.5 sigma significance when averaged over l = 2-7. The BB spectrum, an important probe of gravitational waves from inflation, remains consistent with zero. The upper limit on tensor modes from polarization data alone is a factor of 2 lower with the 7-year data than it was using the 5-year data (Komatsu et al. 2010). We test the parameter recovery process for bias and find that the scalar spectral index, ns, is biased high, but only by 0.09 sigma, while the remaining parameters are biased by < 0.15 sigma. The improvement in the third peak measurement leads to tighter lower limits from WMAP on the number of relativistic degrees of freedom (e.g., neutrinos) in the early universe: Neff > 2.7 (95% CL). Also, using WMAP data alone, the primordial helium mass fraction is found to be YHe = 0.28+0.14-0.15, and with data from higher-resolution CMB experiments included, we now establish the existence of pre-stellar helium at > 3 sigma (Komatsu et al. 2010).Comment: 22 pages, 14 figures, version accepted to Astrophysical Journal Supplement Series, added high-l EE detection, consolidated parameter recovery simulation

Phonon Lifetime Investigation of Anharmonicity and Thermal Conductivity of UO₂ by Neutron Scattering and Theory

Inelastic neutron scattering measurements of individual phonon lifetimes and dispersion at 295 and 1200 K have been used to probe anharmonicity and thermal conductivity in UO2. They show that longitudinal optic phonon modes carry the largest amount of heat, in contrast to past simulations and that the total conductivity demonstrates a quantitative correspondence between microscopic and macroscopic phonon physics. We have further performed first-principles simulations for UO2 showing semiquantitative agreement with phonon lifetimes at 295 K, but larger anharmonicity than measured at 1200 K

Seven-Year Wilkinson Microwave Anisotropy Probe (WMAP) Observations: Are There Cosmic Microwave Background Anomalies?

(Abridged) A simple six-parameter LCDM model provides a successful fit to WMAP data, both when the data are analyzed alone and in combination with other cosmological data. Even so, it is appropriate to search for any hints of deviations from the now standard model of cosmology, which includes inflation, dark energy, dark matter, baryons, and neutrinos. The cosmological community has subjected the WMAP data to extensive and varied analyses. While there is widespread agreement as to the overall success of the six-parameter LCDM model, various "anomalies" have been reported relative to that model. In this paper we examine potential anomalies and present analyses and assessments of their significance. In most cases we find that claimed anomalies depend on posterior selection of some aspect or subset of the data. Compared with sky simulations based on the best fit model, one can select for low probability features of the WMAP data. Low probability features are expected, but it is not usually straightforward to determine whether any particular low probability feature is the result of the a posteriori selection or of non-standard cosmology. We examine in detail the properties of the power spectrum with respect to the LCDM model. We examine several potential or previously claimed anomalies in the sky maps and power spectra, including cold spots, low quadrupole power, quadropole-octupole alignment, hemispherical or dipole power asymmetry, and quadrupole power asymmetry. We conclude that there is no compelling evidence for deviations from the LCDM model, which is generally an acceptable statistical fit to WMAP and other cosmological data.Comment: 19 pages, 17 figures, also available with higher-res figures on http://lambda.gsfc.nasa.gov; accepted by ApJS; (v2) text as accepte

`Standard' Cosmological model & beyond with CMB

Observational Cosmology has indeed made very rapid progress in the past decade. The ability to quantify the universe has largely improved due to observational constraints coming from structure formation Measurements of CMB anisotropy and, more recently, polarization have played a very important role. Besides precise determination of various parameters of the `standard' cosmological model, observations have also established some important basic tenets that underlie models of cosmology and structure formation in the universe -- `acausally' correlated initial perturbations in a flat, statistically isotropic universe, adiabatic nature of primordial density perturbations. These are consistent with the expectation of the paradigm of inflation and the generic prediction of the simplest realization of inflationary scenario in the early universe. Further, gravitational instability is the established mechanism for structure formation from these initial perturbations. The signature of primordial perturbations observed as the CMB anisotropy and polarization is the most compelling evidence for new, possibly fundamental, physics in the early universe. The community is now looking beyond the estimation of parameters of a working `standard' model of cosmology for subtle, characteristic signatures from early universe physics.Comment: 16 pages, 6 figures, Plenary talk, Proc. of GR-19, Mexico City, Mexico (Jul 5-9, 2010). To appear in a special issue in Class. Q. Gra

Seven-Year Wilkinson Microwave Anisotropy Probe (WMAP) Observations: Sky Maps, Systematic Errors, and Basic Results

(Abridged) New full sky temperature and polarization maps based on seven years of data from WMAP are presented. The new results are consistent with previous results, but have improved due to reduced noise from the additional integration time, improved knowledge of the instrument performance, and improved data analysis procedures. The improvements are described in detail. The seven year data set is well fit by a minimal six-parameter flat Lambda-CDM model. The parameters for this model, using the WMAP data in conjunction with baryon acoustic oscillation data from the Sloan Digital Sky Survey and priors on H_0 from Hubble Space Telescope observations, are: Omega_bh^2 = 0.02260 +-0.00053, Omega_ch^2 = 0.1123 +-0.0035, Omega_Lambda = 0.728 +0.015 -0.016, n_s = 0.963 +-0.012, tau = 0.087 +-0.014 and sigma_8 = 0.809 +-0.024 (68 % CL uncertainties). The temperature power spectrum signal-to-noise ratio per multipole is greater that unity for multipoles < 919, allowing a robust measurement of the third acoustic peak. This measurement results in improved constraints on the matter density, Omega_mh^2 = 0.1334 +0.0056 -0.0055, and the epoch of matter- radiation equality, z_eq = 3196 +134 -133, using WMAP data alone. The new WMAP data, when combined with smaller angular scale microwave background anisotropy data, results in a 3 sigma detection of the abundance of primordial Helium, Y_He = 0.326 +-0.075.The power-law index of the primordial power spectrum is now determined to be n_s = 0.963 +-0.012, excluding the Harrison-Zel'dovich-Peebles spectrum by >3 sigma. These new WMAP measurements provide important tests of Big Bang cosmology.Comment: 42 pages, 9 figures, Submitted to Astrophysical Journal Supplement Serie