Laser-induced radial birefringence and spin-to-orbital optical angular momentum conversion in silver-doped glasses

Samples of Ag$^+$/Na$^{+}$ ion-exchanged glass that have been subject to intense laser irradiation may develop novel optical properties, as a consequence of the formation of patterns of silver nanoparticles and other structures. Here, we report the observation of a laser-induced permanent transverse birefringence, with the optical axis forming a radial pattern, as revealed by the spin-to-orbital angular momentum conversion occurring in a probe light beam. The birefringence pattern can be modeled well as resulting from thermally-induced stresses arising in the silver-doped glass during laser exposure, although the actual mechanism leading to the permanent anisotropy is probably more complex.Comment: 3 pages, 3 figure

Photonic polarization gears for ultra-sensitive angular measurements

Quantum metrology bears a great promise in enhancing measurement precision, but is unlikely to become practical in the near future. Its concepts can nevertheless inspire classical or hybrid methods of immediate value. Here, we demonstrate NOON-like photonic states of m quanta of angular momentum up to m=100, in a setup that acts as a "photonic gear", converting, for each photon, a mechanical rotation of an angle {\theta} into an amplified rotation of the optical polarization by m{\theta}, corresponding to a "super-resolving" Malus' law. We show that this effect leads to single-photon angular measurements with the same precision of polarization-only quantum strategies with m photons, but robust to photon losses. Moreover, we combine the gear effect with the quantum enhancement due to entanglement, thus exploiting the advantages of both approaches. The high "gear ratio" m boosts the current state-of-the-art of optical non-contact angular measurements by almost two orders of magnitude.Comment: 10 pages, 4 figures, + supplementary information (10 pages, 3 figures

Spin-orbit hybrid entanglement of photons and quantum contextuality

We demonstrate electromagnetic quantum states of single photons and of correlated photon pairs exhibiting "hybrid" entanglement between spin and orbital angular momentum. These states are obtained from entangled photon pairs emitted by spontaneous parametric down conversion, by employing a $q$-plate for coupling the spin and orbital degrees of freedom of a photon. Entanglement and contextual quantum behavior (that is also non-local, in the case of photon pairs) is demonstrated by the reported violation of the Clauser-Horne-Shimony-Holt inequality. In addition a classical analog of the hybrid spin-orbit photonic entanglement is reported and discussed.Comment: 5 pages, 3 figure

Heralded quantum steering over a high-loss channel

Entanglement is the key resource for many long-range quantum information tasks, including secure communication and fundamental tests of quantum physics. These tasks require robust verification of shared entanglement, but performing it over long distances is presently technologically intractable because the loss through an optical fiber or free-space channel opens up a detection loophole. We design and experimentally demonstrate a scheme that verifies entanglement in the presence of at least $14.8\pm0.1$ dB of added loss, equivalent to approximately $80$ km of telecommunication fiber. Our protocol relies on entanglement swapping to herald the presence of a photon after the lossy channel, enabling event-ready implementation of quantum steering. This result overcomes the key barrier in device-independent communication under realistic high-loss scenarios and in the realization of a quantum repeater.Comment: 8 pages, 5 figure

Light-induced surface sliding of the nematic director in liquid crystals

We report the effect of light-induced sliding of the nematic director over an isotropic boundary surface in an azo-dye doped liquid-crystal cell. We show that illumination of the cell with polarized laser light induces transient dynamic sliding followed by permanent reorientation of the director. The two effects are in competition and tend to orient the director along mutually orthogonal directions. The sliding can be controlled and even completely quenched by the amount of induced anchoring energy. A physical model is proposed which accounts for the experimental results. [S0031-9007(99) PACS numbers: 42.70. Df, 61.30.Cz Light-induced anchoring and reorientation effects in liquid crystals (LC) have been the subject of intense research interests in recent years Optical reorientation was originally concerned with light fields acting on the bulk of a liquid crystal cell, the aligning surface determining only the boundary conditions in the reorientation process. Gibbons et al. These results stimulated an interest to investigate the possibility of getting free surface sliding of the nematic director under the control of the incident light. In the paper of Marusii et al. [8], the authors interpreted the observed molecular reorientation close to the isotropic control surface as an effect of director sliding. However, the impossibility of changing the anchoring energy in their experiment did not allow one to establish definitively the actual nature of the phenomenon. In this paper we report the first clear demonstration of the effect of molecular director sliding over an isotropic surface endowed with very weak anchoring energy. We show that illumination with polarized laser light of an azo-dye doped LC cell induces both a transient dynamic sliding and a permanent reorientation of the molecular director. These two effects are regulated by different physical mechanisms and occur on different time scales. The key points of our experimental observations are (i) on a macroscopic scale, i.e., in the frame of the continuum theory, free director sliding over an isotropic boundary surface is possible, and (ii) this effect can be controlled and even completely quenched by the amount of anchoring energy induced on the surface. The scheme of the experimental setup is shown in The exciting polarized beam from He-Cd laser ͑l 0.442 mm; P 1 mW͒ was focused on the cell from the size of the control surface by the lens L 1 . The director reorientation over this surface was detected by checking the polarization state of a He-Ne laser probe beam ͑l 0.638 mm; P 0.1 mW͒ crossing the cell from the side of the reference surface. The electric field E p of the probe beam was set parallel to the initial director orientation n 0 , and the signal transmitted through an analyzer crossed to it was detected. In this geometry, any rotation of the molecular director (up to 90 ± ) over the control surface led to an increase of the transmitted signal. In fact, in our experimental conditions the Mauguin regime was 0031-9007͞99͞82(9)͞1855(4)$15.0

Complete experimental toolbox for alignment-free quantum communication

Quantum communication employs the counter-intuitive features of quantum physics to perform tasks that are im- possible in the classical world. It is crucial for testing the foundations of quantum theory and promises to rev- olutionize our information and communication technolo- gies. However, for two or more parties to execute even the simplest quantum transmission, they must establish, and maintain, a shared reference frame. This introduces a considerable overhead in communication resources, par- ticularly if the parties are in motion or rotating relative to each other. We experimentally demonstrate how to circumvent this problem with the efficient transmission of quantum information encoded in rotationally invariant states of single photons. By developing a complete toolbox for the efficient encoding and decoding of quantum infor- mation in such photonic qubits, we demonstrate the fea- sibility of alignment-free quantum key-distribution, and perform a proof-of-principle alignment-free entanglement distribution and violation of a Bell inequality. Our scheme should find applications in fundamental tests of quantum mechanics and satellite-based quantum communication.Comment: Main manuscript: 7 pages, 3 figures; Supplementary Information: 7 pages, 3 figure

High speed switching between arbitrary spatial light profiles

Complex images, inscribed into the spatial profile of a laser beam or even a single photon, offer a highly efficient method of data encoding. Here we present a prototype system which can quickly modulate between arbitrary images. We display an array of holograms, each defined by its phase and intensity profile, on a spatial light modulator. The input beam is then steered by an acousto-optic modulator to one of these holograms, where it is converted into the desired light mode. We demonstrate switching between characters within three separate alphabets at a switching rate of up to10 kHz. This rate is limited by our detection system, and we anticipate that the system is capable of far higher rates. Furthermore our system is not limited in efficiency by channel number, making it ideal for quantum communication applications

Optical orbital angular momentum analogy to the Stern-Gerlach experiment

Symmetry breaking has been shown to reveal interesting phenomena in physical systems. A notable example is the fundamental work of Otto Stern and Walther Gerlach [Stern and Zerlach, Z. Physik 9, 349 (1922)] nearly 100 years ago demonstrating a spin angular momentum (SAM) deflection that differed from classical theory. Here we use non-separable states of SAM and orbital angular momentum (OAM), known as vector vortex modes, to demonstrate how a classical optics analogy can be used to reveal this nonseparability, reminiscent of the work carried out by Stern and Gerlach. We show that by implementing a polarization insensitive device to measure the OAM, the SAM states can be deflected to spatially resolved positions

Challenging local realism with human choices

A Bell test is a randomized trial that compares experimental observations against the philosophical worldview of local realism 1, in which the properties of the physical world are independent of our observation of them and no signal travels faster than light. A Bell test requires spatially distributed entanglement, fast and high-efficiency detection and unpredictable measurement settings 2,3 . Although technology can satisfy the first two of these requirements 4-7, the use of physical devices to choose settings in a Bell test involves making assumptions about the physics that one aims to test. Bell himself noted this weakness in using physical setting choices and argued that human 'free will' could be used rigorously to ensure unpredictability in Bell tests 8 . Here we report a set of local-realism tests using human choices, which avoids assumptions about predictability in physics. We recruited about 100,000 human participants to play an online video game that incentivizes fast, sustained input of unpredictable selections and illustrates Bell-test methodology 9 . The participants generated 97,347,490 binary choices, which were directed via a scalable web platform to 12 laboratories on five continents, where 13 experiments tested local realism using photons 5,6, single atoms 7, atomic ensembles 10 and superconducting devices 11 . Over a 12-hour period on 30 November 2016, participants worldwide provided a sustained data flow of over 1,000 bits per second to the experiments, which used different human-generated data to choose each measurement setting. The observed correlations strongly contradict local realism and other realistic positions in bipartite and tripartite 12 scenarios. Project outcomes include closing the 'freedom-of-choice loophole' (the possibility that the setting choices are influenced by 'hidden variables' to correlate with the particle properties 13 ), the utilization of video-game methods 14 for rapid collection of human-generated randomness, and the use of networking techniques for global participation in experimental science

Challenging local realism with human choices

A Bell test is a randomized trial that compares experimental observations against the philosophical worldview of local realism. A Bell test requires spatially distributed entanglement, fast and high-efficiency detection and unpredictable measurement settings. Although technology can satisfy the first two of these requirements, the use of physical devices to choose settings in a Bell test involves making assumptions about the physics that one aims to test. Bell himself noted this weakness in using physical setting choices and argued that human `free will' could be used rigorously to ensure unpredictability in Bell tests. Here we report a set of local-realism tests using human choices, which avoids assumptions about predictability in physics. We recruited about 100,000 human participants to play an online video game that incentivizes fast, sustained input of unpredictable selections and illustrates Bell-test methodology. The participants generated 97,347,490 binary choices, which were directed via a scalable web platform to 12 laboratories on five continents, where 13 experiments tested local realism using photons, single atoms, atomic ensembles, and superconducting devices. Over a 12-hour period on 30 November 2016, participants worldwide provided a sustained data flow of over 1,000 bits per second to the experiments, which used different human-generated data to choose each measurement setting. The observed correlations strongly contradict local realism and other realistic positions in bipartite and tripartite scenarios. Project outcomes include closing the `freedom-of-choice loophole' (the possibility that the setting choices are influenced by `hidden variables' to correlate with the particle properties), the utilization of video-game methods for rapid collection of human generated randomness, and the use of networking techniques for global participation in experimental science.Comment: This version includes minor changes resulting from reviewer and editorial input. Abstract shortened to fit within arXiv limit