52 research outputs found

    Comparison of 120Sn(6He,6He)120Sn and 120Sn(alpha,alpha)120Sn elastic scattering and signatures of the 6He neutron halo in the optical potential

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    Cross sections of 120^{120}Sn(α\alpha,α\alpha)120^{120}Sn elastic scattering have been extracted from the α\alpha particle beam contamination of a recent 120^{120}Sn(6^6He,6^6He)120^{120}Sn experiment. Both reactions are analyzed using systematic double folding potentials in the real part and smoothly varying Woods-Saxon potentials in the imaginary part. The potential extracted from the 120^{120}Sn(6^6He,6^6He)120^{120}Sn data may be used as the basis for the construction of a simple global 6^6He optical potential. The comparison of the 6^6He and α\alpha data shows that the halo nature of the 6^6He nucleus leads to a clear signature in the reflexion coefficients ηL\eta_L: the relevant angular momenta LL with ηL0\eta_L \gg 0 and ηL1\eta_L \ll 1 are shifted to larger LL with a broader distribution. This signature is not present in the α\alpha scattering data and can thus be used as a new criterion for the definition of a halo nucleus.Comment: 13 pages, 7 figures, accepted for publication in Phys. Rev.

    Rational Design of a Biocatalyst Based on Immobilized CALB onto Nanostructured SiO2

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    The adsorption of the lipase B from Candida antarctica (CALB) over nanostructured SiO2 (Ns SiO2 from now on) with and without the addition of polyols (sorbitol and glycerol) was investigated. The isotherms of adsorption made it possible to establish that the maximum dispersion limit was 0.029 µmol of protein per surface area unit of Ns SiO2 (29.4 mg per 100 mg of support), which was reached in 30 min of exposure. The studies through SDS-PAGE of the immobilization solutions and infrared spectroscopy of the prepared solids determined that CALB (from a commercial extract) is selectively adsorbed, and its secondary structure distribution is thus modified. Its biocatalytic activity was corroborated through the kinetic resolution of rac-ibuprofen. Conversions of up to 70% and 52% enantiomeric excess toward S-ibuprofen in 24 h of reaction at 45 °C were achieved. The biocatalytic performance increased with the increase in protein loading until it leveled off at 0.021 µmol.m−2, reaching 0.6 µmol.min−1. The biocatalyst containing the lipase at the maximum dispersion limit and co-adsorbed polyols presented the best catalytic performance in the kinetic resolution of rac-ibuprofen, an improved thermal resistance (up to 70 °C), and stability under long-term storage (more than 2 years).Fil: Llerena Suster, Carlos Rafael. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Centro de Investigación y Desarrollo en Ciencias Aplicadas "Dr. Jorge J. Ronco". Universidad Nacional de la Plata. Facultad de Ciencias Exactas. Centro de Investigación y Desarrollo en Ciencias Aplicadas; Argentina. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Departamento de Ciencias Biológicas. Laboratorio de Investigación de Proteínas Vegetales; ArgentinaFil: Toledo, María V.. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Centro de Investigación y Desarrollo en Ciencias Aplicadas "Dr. Jorge J. Ronco". Universidad Nacional de la Plata. Facultad de Ciencias Exactas. Centro de Investigación y Desarrollo en Ciencias Aplicadas; ArgentinaFil: Matkovic, Silvana Raquel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Centro de Investigación y Desarrollo en Ciencias Aplicadas "Dr. Jorge J. Ronco". Universidad Nacional de la Plata. Facultad de Ciencias Exactas. Centro de Investigación y Desarrollo en Ciencias Aplicadas; ArgentinaFil: Morcelle del Valle, Susana Raquel. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Departamento de Ciencias Biológicas. Laboratorio de Investigación de Proteínas Vegetales; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata; ArgentinaFil: Briand, Laura Estefania. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Centro de Investigación y Desarrollo en Ciencias Aplicadas "Dr. Jorge J. Ronco". Universidad Nacional de la Plata. Facultad de Ciencias Exactas. Centro de Investigación y Desarrollo en Ciencias Aplicadas; Argentin

    Two-neutron transfer in 7 Be + 9 Be collisions

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    Elastic scattering and transfer cross sections for the 7 Be + 9 Be system have been measured at E lab = 23.1 MeV using the 7 Be radioactive secondary beam produced at Radioactive Ion Beams in Brazil facility at the University of São Paulo. The elastic scattering has been measured by detecting the 7 Be scattered at forward angles in the laboratory system. The transfer reaction 9 Be ( 7 Be , 9 Be ) 7 Be was identified by detecting the 9 Be scattered at the same laboratory angles. The elastic angular distribution has been analyzed by optical model calculations using a Woods-Saxon form factor whose parameters have been varied to best reproduce the experimental data at forward angles. Coupled reaction channels calculations (CRC) have been performed to describe the transfer, considering the coupling to the transfer channel and including contributions to the ground state and to the first excited state of 7 Be ( 1 / 2 − ; 429 keV ) in the final state. The spectroscopic amplitudes used in the CRC calculation have been derived from shell-model calculations. Similar CRC calculations were applied to existing 9 Be ( p , t ) 7 Be data to check the consistency of our results results for the ( 7 Be , 9 Be ) transfer reaction.Conselho Nacional de Desenvolvimento Científico e Tecnológico (CNPq) de Brasil, Fundação de Amparo à Pesquisa do Estado do Rio de Janeiro (FAPERJ) de Brasil y Fundação de Amparo à Pesquisa do Estado de São Paulo (FAPESP) de Brasil. 2013/22100-7 y 2016/21434-

    Experimental study of He6+Be9 elastic scattering at low energies

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    New data for the He6+Be9 reaction at Elab=16.2 and 21.3 MeV have been taken and analyzed. The effect of the collective couplings to the excited states of the target has been studied by means of coupled-channels calculations, using a double-folding potential for the bare interaction between the colliding nuclei, supplemented with a phenomenological imaginary part of Woods-Saxon type. In addition, three- and four-body continuum-discretized coupled-channels calculations have been performed to investigate the effect of the projectile breakup on the elastic scattering. Both effects, the coupling to target and projectile excited states, are found to affect significantly the elastic scattering. The trivial local polarization potential extracted from the continuum-discretized coupled-channels calculations indicates that continuum couplings produce a repulsive real part and a long-range imaginary part in the projectile-target interaction. © 2011 American Physical Society.This work has been partially supported by the Spanish Ministerio de Ciencia e Innovacion´ under Projects FPA2009-07653 and PCI2006-A7-0654 and by the Spanish Consolider-Ingenio 2010 Programme CPAN (CSD2007-00042).Peer Reviewe

    Study of the 6He+9Be and 7Be+9Be collisions

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    We present elastic scattering angular distributions of the 6He+9Be and 7Be+9Be reactions at Elab =16.2 MeV and Elab =23.7 MeV respectively. The 6He+9Be measurements have been performed at the Pelletron Laboratory of the Institute of Physics of the University of Sao Paulo, Brazil, using the Radioactive Ion Beams in Brasil (RIBRAS) facility and the 7Be+9Be system has beenmeasured at CRC Radioactive Beam Facility at Louvain-la-Neuve,Belgium. An OpticalModel analysis has been performed to obtain the nuclear potentials for both systems. A coupled-channel calculation was performed for the 7Be+9Be system taking into account the coupling to the first excited state and breakup channels of the 7Be nucleus. Keywords: Radioctive Beams. Exotic Nuclei. Nuclear Halo. Long range absorption. Elastic Scattering. Optical potential. Coupled channels calculations. PACS: 25.60.-t,25.60.Bx,25.70.Bc,29.38.-c,24.10.E

    Ionization and Fragmentation of a Global Warming Gas by EUV and X-Ray Photons

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    An experimental investigation of the processes leading tothe fragmentation of the singly ionized 1,1,1,2-tetrafluoroethane (HFC-134a, CH2FCF3) by EUV and soft X-rays is presented. HFC-134ais taken into consideration as the most convenient replacement for CFC-12 in refrigeration applications due to the fact that it has null ozone depletion factor. Dissociation of the singly ionized HFC-134amolecule was induced by valence, direct and indirect C 1s core photoionization or photoexcitation and the ionic fragments were detected in coincidence (PEPICO mode) with the ejected electrons without energy analysis. The singly ionized parent ion CF4CH2+can be detected even at photon energies above the C 1s threshold

    Nuclear astrophysics with radioactive ions at FAIR

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    The nucleosynthesis of elements beyond iron is dominated by neutron captures in the s and r processes. However, 32 stable, proton-rich isotopes cannot be formed during those processes, because they are shielded from the s-process flow and r-process, β-decay chains. These nuclei are attributed to the p and rp process. For all those processes, current research in nuclear astrophysics addresses the need for more precise reaction data involving radioactive isotopes. Depending on the particular reaction, direct or inverse kinematics, forward or time-reversed direction are investigated to determine or at least to constrain the desired reaction cross sections. The Facility for Antiproton and Ion Research (FAIR) will offer unique, unprecedented opportunities to investigate many of the important reactions. The high yield of radioactive isotopes, even far away from the valley of stability, allows the investigation of isotopes involved in processes as exotic as the r or rp processes

    Photofissility at 1 GeV for nuclei throughout the periodic table

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    A new approach to evaluate nuclear photofissilities at incident photon energies above the pion photoproduction threshold has been recently developed and proved to describe successfully the fissilities of natPb and 232Th target nuclei at energies ~0.2-4.0 GeV. The method is merely a simple, semiempirical description of the photofission reactions in which fissility, f, is governed by two basic quantities, namely, i) the first-chance fission probability, fˉ1\bar{f}_1, for the average cascade residual, and ii) the slope, sˉ\bar{s}, of the chance-fission probability associated with the average evaporative sequence of fissionable residuals. In the present work we have extended this approach to analyse photofissity data that have been accumulated over the past fourty years or so, measured at 1 GeV, for nearly fourty target nuclei extending from Ti up to Np. Results have shown that the variation of fissility with Z²/A could be described quite satisfactorily by the proposed model
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