Decay of the key 92-keV resonance in the 25Mg(p,γ) reaction to the ground and isomeric states of the cosmic γ-ray emitter 26Al

The 92-keV resonance in the 25Mg(p,γ)26Al reaction plays a key role in the production of 26Al at astrophysical burning temperatures of ≈100 MK in the Mg-Al cycle. However, the state can decay to feed either the ground, 26gAl, or isomeric state, 26mAl. It is the ground state that is critical as the source of cosmic γ rays. It is therefore important to precisely determine the ground-state branching fraction f0 of this resonance. Here we report on the identification of four γ-ray transitions from the 92-keV resonance, and determine the spin of the state and its ground-state branching fraction f0=0.52(2)stat(6)syst. The f0 value is the most precise reported to date, and at the lower end of the range of previously adopted values, implying a lower production rate of 26gAl and its cosmic 1809-keV γ rays.peerReviewe

Structure of resonances in the Gamow burning window for the Al 25 (p,γ) Si 26 reaction in novae

A γ-ray spectroscopy study of excited states in Si26 has been performed by using the Mg24(3He,n) reaction at a beam energy of 10 MeV. In particular, states have been studied above the proton threshold relevant for burning in the Al25(p,γ)Si26 reaction in novae. This reaction influences the amount of Al26 injected into the interstellar medium by novae, which contributes to the overall flux of cosmic γ-ray emission from Al26 observed in satellite missions. The present results point strongly to the existence of a 0+ state at an excitation energy of 5890 keV lying within the Gamow burning window, which raises questions about the existence and properties of another, higher-lying state reported in previous experimental work. The existence of two such states within this excitation energy region cannot be understood within the framework of sd-shell-model calculations. © 2015 American Physical Society

Decay of the key 92-keV resonance in the 25Mg(p,γ) reaction to the ground and isomeric states of the cosmic γ-ray emitter 26Al

The 92-keV resonance in the 25Mg(p,γ)26Al reaction plays a key role in the production of 26Al at astrophysical burning temperatures of ≈100 MK in the Mg-Al cycle. However, the state can decay to feed either the ground, 26gAl, or isomeric state, 26mAl. It is the ground state that is critical as the source of cosmic γ rays. It is therefore important to precisely determine the ground-state branching fraction f0 of this resonance. Here we report on the identification of four γ-ray transitions from the 92-keV resonance, and determine the spin of the state and its ground-state branching fraction f0=0.52(2)stat(6)syst. The f0 value is the most precise reported to date, and at the lower end of the range of previously adopted values, implying a lower production rate of 26gAl and its cosmic 1809-keV γ rays

Time-of-flight and activation experiments on 147Pm and 171Tm for astrophysics

The neutron capture cross section of several key unstable isotopes acting as branching points in the s-process are crucial for stellar nucleosynthesis studies, but they are very challenging to measure due to the difficult production of sufficient sample material, the high activity of the resulting samples, and the actual (n,γ) measurement, for which high neutron fluxes and effective background rejection capabilities are required. As part of a new program to measure some of these important branching points, radioactive targets of 147Pm and 171Tm have been produced by irradiation of stable isotopes at the ILL high flux reactor. Neutron capture on 146Nd and 170Er at the reactor was followed by beta decay and the resulting matrix was purified via radiochemical separation at PSI. The radioactive targets have been used for time-of-flight measurements at the CERN n-TOF facility using the 19 and 185 m beam lines during 2014 and 2015. The capture cascades were detected using a set of four C6D6 scintillators, allowing to observe the associated neutron capture resonances. The results presented in this work are the first ever determination of the resonance capture cross section of 147Pm and 171Tm. Activation experiments on the same 147Pm and 171Tm targets with a high-intensity 30 keV quasi-Maxwellian flux of neutrons will be performed using the SARAF accelerator and the Liquid-Lithium Target (LiLiT) in order to extract the corresponding Maxwellian Average Cross Section (MACS). The status of these experiments and preliminary results will be presented and discussed as well

Characterization of the n-TOF EAR-2 neutron beam

The experimental area 2 (EAR-2) at CERNs neutron time-of-flight facility (n-TOF), which is operational since 2014, is designed and built as a short-distance complement to the experimental area 1 (EAR-1). The Parallel Plate Avalanche Counter (PPAC) monitor experiment was performed to characterize the beam prole and the shape of the neutron 'ux at EAR-2. The prompt γ-flash which is used for calibrating the time-of-flight at EAR-1 is not seen by PPAC at EAR-2, shedding light on the physical origin of this γ-flash

New measurement of the 242Pu(n,γ) cross section at n-TOF-EAR1 for MOX fuels : Preliminary results in the RRR

The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with 238U to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. The use of MOX fuels in thermal and fast reactors requires accurate capture and fission cross sections. For the particular case of 242Pu, the previous neutron capture cross section measurements were made in the 70's, providing an uncertainty of about 35% in the keV region. In this context, the Nuclear Energy Agency recommends in its "High Priority Request List" and its report WPEC-26 that the capture cross section of 242Pu should be measured with an accuracy of at least 7-12% in the neutron energy range between 500 eV and 500 keV. This work presents a brief description of the measurement performed at n-TOF-EAR1, the data reduction process and the first ToF capture measurement on this isotope in the last 40 years, providing preliminary individual resonance parameters beyond the current energy limits in the evaluations, as well as a preliminary set of average resonance parameters

The measurement programme at the neutron time-of-flight facility n-TOF at CERN

Neutron-induced reaction cross sections are important for a wide variety of research fields ranging from the study of nuclear level densities, nucleosynthesis to applications of nuclear technology like design, and criticality and safety assessment of existing and future nuclear reactors, radiation dosimetry, medical applications, nuclear waste transmutation, accelerator-driven systems and fuel cycle investigations. Simulations and calculations of nuclear technology applications largely rely on evaluated nuclear data libraries. The evaluations in these libraries are based both on experimental data and theoretical models. CERN's neutron time-of-flight facility n-TOF has produced a considerable amount of experimental data since it has become fully operational with the start of its scientific measurement programme in 2001. While for a long period a single measurement station (EAR1) located at 185 m from the neutron production target was available, the construction of a second beam line at 20 m (EAR2) in 2014 has substantially increased the measurement capabilities of the facility. An outline of the experimental nuclear data activities at n-TOF will be presented

Determination of luminosity for in-ring reactions:A new approach for the low-energy domain

Luminosity is a measure of the colliding frequency between beam and target and it is a crucial parameter for the measurement of absolute values, such as reaction cross sections. In this paper, we make use of experimental data from the ESR storage ring to demonstrate that the luminosity can be precisely determined by modelling the measured Rutherford scattering distribution. The obtained results are in good agreement with an independent measurement based on the x-ray normalization method. Our new method provides an alternative way to precisely measure the luminosity in low-energy stored-beam configurations. This can be of great value in particular in dedicated low-energy storage rings where established methods are difficult or impossible to apply.Comment: 8 pages, 5 figure

Solving the Puzzles of the Decay of the Heaviest Known Proton-Emitting Nucleus Bi 185

Two long-standing puzzles in the decay of Bi185, the heaviest known proton-emitting nucleus are revisited. These are the nonobservation of the 9/2- state, which is the ground state of all heavier odd-A Bi isotopes, and the hindered nature of proton and α decays of its presumed 60-μs 1/2+ ground state. The Bi185 nucleus has now been studied with the Mo95(Nb93,3n) reaction in complementary experiments using the Fragment Mass Analyzer and Argonne Gas-Filled Analyzer at Argonne National Laboratory's ATLAS facility. The experiments have established the existence of two states in Bi185; the short-lived T1/2=2.8-1.0+2.3 μs, proton- and α-decaying ground state, and a 58(2)-μs γ-decaying isomer, the half-life of which was previously attributed to the ground state. The reassignment of the ground-state lifetime results in a proton-decay spectroscopic factor close to unity and represents the only known example of a ground-state proton decay to a daughter nucleus (Pb184) with a major shell closure. The data also demonstrate that the ordering of low- and high-spin states in Bi185 is reversed relative to the heavier odd-A Bi isotopes, with the intruder-based 1/2+ configuration becoming the ground, similar to the lightest At nuclides