127 research outputs found
Electronic and magnetic properties of the ionic Hubbard model on the striped triangular lattice at 3/4 filling
We report a detailed study of a model Hamiltonian which exhibits a rich
interplay of geometrical spin frustration, strong electronic correlations, and
charge ordering. The character of the insulating phase depends on the magnitude
of Delta/|t| and on the sign of t. We find a Mott insulator for Delta >> U >>
|t|; a charge transfer insulator for U >> \Delta >> |t|; and a correlated
covalent insulator for U >> \Delta ~ |t|. The charge transfer insulating state
is investigated using a strong coupling expansion. The frustration of the
triangular lattice can lead to antiferromagnetism or ferromagnetism depending
on the sign of the hopping matrix element, t. We identify the "ring" exchange
process around a triangular plaquette which determines the sign of the magnetic
interactions. Exact diagonalization calculations are performed on the model for
a wide range of parameters and compared to the strong coupling expansion. The
regime U >> \Delta ~ |t| and t<0 is relevant to Na05CoO2. The calculated
optical conductivity and the spectral density are discussed in the light of
recent experiments on Na05CoO2.Comment: 15 pages, 15 figure
Direct comparison between potential landscape and local density of states in a disordered two-dimensional electron system
The local density of states (LDOS) of the adsorbate induced two-dimensional
electron system (2DES) on n-InAs(110) is studied by low-temperature scanning
tunneling spectroscopy. The LDOS exhibits irregular structures with fluctuation
lengths decreasing with increasing energy. Fourier transformation reveals that
the k-values of the unperturbed 2DES dominate the LDOS, but additional lower
k-values contribute significantly. To clarify the origin of the additional
k-space intensity, we measure the potential landscape of the same 2DES area
with the help of the tip induced quantum dot. This allows to calculate the
expected LDOS from the single particle Schroedinger equation and to directly
compare it with the measured one. Reasonable correspondance between calculated
and measured LDOS is found.Comment: 7 pages, 4 figures, submitted to PR
Correlation between magnetic interactions and domain structure in A1 FePt ferromagnetic thin films
We have investigated the relationship between the domain structure and the
magnetic interactions in a series of FePt ferromagnetic thin films of varying
thickness. As-made films grow in the magnetically soft and chemically
disordered A1 phase that may have two distinct domain structures. Above a
critical thickness nm the presence of an out of plane
anisotropy induces the formation of stripes, while for planar
domains occur.
Magnetic interactions have been characterized using the well known DCD-IRM
remanence protocols, plots, and magnetic viscosity measurements. We
have observed a strong correlation between the domain configuration and the
sign of the magnetic interactions. Planar domains are associated with positive
exchange-like interactions, while stripe domains have a strong negative
dipolar-like contribution. In this last case we have found a close correlation
between the interaction parameter and the surface dipolar energy of the stripe
domain structure. Using time dependent magnetic viscosity measurements, we have
also estimated an average activation volume for magnetic reversal, nm which is approximately
independent of the film thickness or the stripe period.Comment: 25 pages, 11 figure
Orientation and substrate interaction of adsorbed CO and NO molecules probed by circular dichroism in the angular distribution of photoelectrons
The sensitivity and utility of circular dichroism in the angular distribution of photoelectrons (CDAD) as a probe of molecular orientation is demonstrated for adsorbed CO and NO molecules. A comparison between measured CDAD spectra and calculated values for spatially oriented CO and NiCO clearly confirms the well-known perpendicular adsorption for CO on Ni(100), whereas for CO adsorbed on Fe(100) a tilted adsorption geometry was found. For NO/Ni(100) and for NO on the oxygen-preadsorbed Ni(100) surface, an average tilt angle of α=40±10° was observed. In the case of the oxygen-preadsorbed Ni(100) surface, a higher fraction of NO molecules was found to be in a tilted orientation than on the clean surface
Electronic transport through domain walls in ferromagnetic nanowires: Co-existence of adiabatic and non-adiabatic spin dynamics
We study the effect of a domain wall on the electronic transport in
ferromagnetic quantum wires. Due to the transverse confinement, conduction
channels arise. In the presence of a domain wall, spin up and spin down
electrons in these channels become coupled. For very short domain walls or at
high longitudinal kinetic energy, this coupling is weak, leads to very few spin
flips, and a perturbative treatment is possible. For very long domain wall
structures, the spin follows adiabatically the local magnetization orientation,
suppressing the effect of the domain wall on the total transmission, but
reversing the spin of the electrons. In the intermediate regime, we numerically
investigate the spin-dependent transport behavior for different shapes of the
domain wall. We find that the knowledge of the precise shape of the domain wall
is not crucial for determining the qualitative behavior. For parameters
appropriate for experiments, electrons with low longitudinal energy are
transmitted adiabatically while the electrons at high longitudinal energy are
essentially unaffected by the domain wall. Taking this co-existence of
different regimes into account is important for the understanding of recent
experiments.Comment: 10 pages, 6 figure
Femtosecond nonlinear ultrasonics in gold probed with ultrashort surface plasmons
Fundamental interactions induced by lattice vibrations on ultrafast time
scales become increasingly important for modern nanoscience and technology.
Experimental access to the physical properties of acoustic phonons in the THz
frequency range and over the entire Brillouin zone is crucial for understanding
electric and thermal transport in solids and their compounds. Here, we report
on the generation and nonlinear propagation of giant (1 percent) acoustic
strain pulses in hybrid gold/cobalt bilayer structures probed with ultrafast
surface plasmon interferometry. This new technique allows for unambiguous
characterization of arbitrary ultrafast acoustic transients. The giant acoustic
pulses experience substantial nonlinear reshaping already after a propagation
distance of 100 nm in a crystalline gold layer. Excellent agreement with the
Korteveg-de Vries model points to future quantitative nonlinear femtosecond
THz-ultrasonics at the nano-scale in metals at room temperature
Regional Imprints of Changes in the Atlantic Meridional Overturning Circulation in the Eddy-rich Ocean Model VIKING20X
A hierarchy of global 1/4° (ORCA025) and Atlantic Ocean 1/20° nested (VIKING20X) ocean/sea-ice models is described. It is shown that the eddy-rich configurations performed in hindcasts of the past 50â60 years under CORE and JRA55-do atmospheric forcings realistically simulate the large-scale horizontal circulation, the distribution of the mesoscale, overflow and convective processes, and the representation of regional current systems in the North and South Atlantic. The representation, and in particular the long-term temporal evolution, of the Atlantic Meridional Overturning Circulation (AMOC) strongly depends on numerical choices for the application of freshwater fluxes. The interannual variability of the AMOC instead is highly correlated among the model experiments and also with observations, including the 2010 minimum observed by RAPID at 26.5° N pointing at a dominant role of the forcing. Regional observations in western boundary current systems at 53° N, 26.5° N and 11° S are explored in respect to their ability to represent the AMOC and to monitor the temporal evolution of the AMOC. Apart from the basin-scale measurements at 26.5° N, it is shown that in particular the outflow of North Atlantic Deepwater at 53° N is a good indicator of the subpolar AMOC trend during the recent decades, if the latter is provided in density coordinates. The good reproduction of observed AMOC and WBC trends in the most reasonable simulations indicate that the eddy-rich VIKING20X is capable in representing realistic forcing-related and ocean-intrinsic trends
Silicon isotopes in an EMIC's ocean: Sensitivity to runoff, iron supply, and climate
The isotopic composition of Si in biogenic silica (BSi), such as opal buried in the oceans' sediments, has changed over time. Paleorecords suggest that the isotopic composition, described in terms of ÎŽ30Si, was generally much lower during glacial times than today. There is consensus that this variability is attributable to differing environmental conditions at the respective time of BSi production and sedimentation. The detailed links between environmental conditions and the isotopic composition of BSi in the sediments remain, however, poorly constrained. In this study, we explore the effects of a suite of offset boundary conditions during the Last Glacial Maximum (LGM) on the isotopic composition of BSi archived in sediments in an Earth System Model of intermediate complexity (EMIC). Our model results suggest that a change in the isotopic composition of Si supply to the glacial ocean is sufficient to explain the observed overall low(er) glacial ÎŽ30Si in BSi. All other processes explored trigger model responses of either wrong sign or magnitude or are inconsistent with a recent estimate of bottom water oxygenation in the Atlantic Sector of the Southern Ocean. Caveats, mainly associated with generic uncertainties in today's pelagic biogeochemical modules, remain.publishedVersio
Theory of magnetization precession induced by a picosecond strain pulse in ferromagnetic semiconductor (Ga,Mn)As
A theoretical model of the coherent precession of magnetization excited by a
picosecond acoustic pulse in a ferromagnetic semiconductor layer of (Ga,Mn)As
is developed. The short strain pulse injected into the ferromagnetic layer
modifies the magnetocrystalline anisotropy resulting in a tilt of the
equilibrium orientation of magnetization and subsequent magnetization
precession. We derive a quantitative model of this effect using the
Landau-Lifshitz equation for the magnetization that is precessing in the
time-dependent effective magnetic field. After developing the general
formalism, we then provide a numerical analysis for a certain structure and two
typical experimental geometries in which an external magnetic field is applied
either along the hard or the easy magnetization axis. As a result we identify
three main factors, which determine the precession amplitude: the
magnetocrystalline anisotropy of the ferromagnetic layer, its thickness, and
the strain pulse parameters
Zonal circulation across 52°W in the North Atlantic
Author Posting. © American Geophysical Union, 2004. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Journal of Geophysical Research 109 (2004): C11008, doi:10.1029/2003JC002103.In JulyâAugust 1997, a hydrographic/Acoustic Doppler Current Profiler (ADCP)/tracer section was occupied along 52°W in the North Atlantic as part of the World Ocean Circulation Experiment Hydrographic Program. Underway and lowered ADCP (LADCP) data have been used to reference geostrophic velocities calculated from the hydrographic data; additional (small) velocity adjustments provided by an inverse model, constraining mass and silicate transports in 17 neutral density layers, yield the absolute zonal velocity field for 52°W. We find a vigorous circulation throughout the entire section, with an unusually strong Gulf Stream (169 Sv) and southern Deep Western Boundary Current (DWBC; 64 Sv) at the time of the cruise. At the northern boundary, on the west side of the Grand Banks of Newfoundland, we find the westward flowing Labrador Current (8.6 Sv), whose continuity from the Labrador Sea, east of our section, has been disputed. Directly to the south we identify the slopewater current (12.5 Sv eastward) and northern DWBC (12.5 Sv westward). Strong departures from strictly zonal flow in the interior, which are found in the LADCP data, make it difficult to diagnose the circulation there. Isolated deep property extrema in the southern portion, associated with alternating bands of eastward and westward flow, are consistent with the idea that the rough topography of the Mid-Atlantic Ridge, directly east of our section, causes enhanced mixing of Antarctic Bottom Water properties into overlying waters with distinctly different properties. We calculate heat and freshwater fluxes crossing 52°W that exceed estimates based on air-sea exchanges by a factor of 1.7.This work was supported by NSF grants
OCE95-29607, OCE 95-31864, OCE98-18266, and OCE-0219644
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