193 research outputs found
Quasi Free 238U (e,e'f)-Cross Section in Macroscopic-Microscopic Approach
We present the result of a theoretical study of inclusive quasi free
electrofission of U. The off-shell cross sections for the quasi free
reaction stage have been calculated within the Plane Wave Impulse Approximation
(PWIA), using a Macroscopic -Microscopic description of the proton and neutron
single particle momentum distributions. Electron wave function distortion
corrections were included using the effective momentum approximation, and the
Final State Interaction (FSI) effects were calculated using an optical
potential. The fissility for the proton single hole excited states of the
residual nucleus Pa was calculated both without and with contributions
of the pre-equilibrium emission of the particles. The fissility for
residual nuclei was calculated within the compound nucleus model.
The cross sections thus obtained were compared with available
experimental data.Comment: 26 pages, 7 figure
Spectroscopy of Po
Prompt, in-beam rays following the reaction Yb + 142 MeV
Si were measured at the ATLAS facility using 10 Compton-suppressed Ge
detectors and the Fragment Mass Analyzer. Transitions in Po were
identified and placed using -ray singles and coincidence data gated on
the mass of the evaporation residues. A level spectrum up to
J10 was established. The structure of Po is more
collective than that observed in the heavier polonium isotopes and indicates
that the structure has started to evolve towards the more collective nature
expected for deformed nuclei.Comment: 8 pages, revtex 3.0, 4 figs. available upon reques
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Radiation imaging technology for nuclear materials safeguards
Gamma-ray and neutron imaging technology is emerging as a useful tool for nuclear materials safeguards. Principal applications include improvement in accuracy for nondestructive assay of heterogeneous material (e.g., residues) and wide-area imaging of nuclear material in facilities (e.g., holdup). Portable gamma cameras with gamma-ray spectroscopy are available commercially and are being applied to holdup measurements. The technology has the potential to significantly reduce effort and exposure in holdup campaigns; and, with imaging, some of the limiting assumptions required for conventional holdup analysis can be relaxed, resulting in a more general analysis. Methods to analyze spectroscopic-imaging data to assay plutonium and uranium in processing equipment are being development. Results of holdup measurements using a commercial, portable gamma-cameras are presented. The authors are also developing fast neutron imaging techniques for NDA, search, and holdup. Fast neutron imaging provides a direct measurement of the source of neutrons and is relatively insensitive to surroundings when compared to thermal or epithermal neutron imaging. The technology is well-suited for in-process inventory measurements and verification of materials in interim storage, for which gamma-ray measurements may be inadequate due to self-shielding. Results of numerical simulations to predict the performance of fast-neutron telescopes for safeguards applications are presented
Neutrino-induced neutron spallation and supernova r-process nucleosynthesis
In order to explore the consequences of the neutrino irradiation for the
supernova r-process nucleosynthesis, we calculate the rates of charged-current
and neutral-current neutrino reactions on neutron-rich heavy nuclei, and
estimate the average number of neutrons emitted in the resulting spallation.
Our results suggest that charged-current captures can be important in
breaking through the waiting-point nuclei at N=50 and 82, while still allowing
the formation of abundance peaks. Furthermore, after the r-process freezes out,
there appear to be distinctive neutral-current and charged-current
postprocessing effects. A subtraction of the neutrino postprocessing effects
from the observed solar r-process abundance distribution shows that two mass
regions, A=124-126 and 183-187, are inordinately sensitive to neutrino
postprocessing effects. This imposes very stringent bounds on the freeze-out
radii and dynamic timescales governing the r-process. Moreover, we find that
the abundance patterns within these mass windows are entirely consistent with
synthesis by neutrino interactions. This provides a strong argument that the
r-process must occur in the intense neutrino flux provided by a core-collapse
supernova.Comment: 34 pages, 4 PostScript figures, RevTe
Very high rotational frequencies and band termination in 73Br
Rotational bands in 73Br have been investigated up to spins of 65/2 using the
EUROBALL III spectrometer. One of the negative-parity bands displays the
highest rotational frequency 1.85 MeV reported to date in nuclei with mass
number greater than 25. At high frequencies, the experimental dynamic moment of
inertia for all bands decrease to very low values, indicating a loss of
collectivity. The bands are described in the configuration-dependent cranked
Nilsson-Strutinsky model. The calculations indicate that one of the
negative-parity bands is observed up to its terminating single-particle state
at spin 63/2. This result establishes the first band termination case in the A
= 70 mass region.Comment: 6 pages, 6 figures, submitted to Phys. Rev. C as a Rapid
Communicatio
Extended Hauser-Feshbach Method for Statistical Binary-Decay of Light-Mass Systems
An Extended Hauser-Feshbach Method (EHFM) is developed for light heavy-ion
fusion reactions in order to provide a detailed analysis of all the possible
decay channels by including explicitly the fusion-fission phase-space in the
description of the cascade chain. The mass-asymmetric fission component is
considered as a complex-fragment binary-decay which can be treated in the same
way as the light-particle evaporation from the compound nucleus in
statistical-model calculations. The method of the phase-space integrations for
the binary-decay is an extension of the usual Hauser-Feshbach formalism to be
applied to the mass-symmetric fission part. The EHFM calculations include
ground-state binding energies and discrete levels in the low excitation-energy
regions which are essential for an accurate evaluation of the phase-space
integrations of the complex-fragment emission (fission). In the present
calculations, EHFM is applied to the first-chance binary-decay by assuming that
the second-chance fission decay is negligible. In a similar manner to the
description of the fusion-evaporation process, the usual cascade calculation of
light-particle emission from the highly excited complex fragments is applied.
This complete calculation is then defined as EHFM+CASCADE. Calculated
quantities such as charge-, mass- and kinetic-energy distributions are compared
with inclusive and/or exclusive data for the S+Mg and
Cl+C reactions which have been selected as typical examples.
Finally, the missing charge distributions extracted from exclusive measurements
are also successfully compared with the EHFM+CASCADE predictions.Comment: 34 pages, 6 Figures available upon request, Phys. Rev. C (to be
published
Highly deformed Ca configurations in Si + C
The possible occurrence of highly deformed configurations in the Ca
di-nuclear system formed in the Si + C reaction is investigated
by analyzing the spectra of emitted light charged particles. Both inclusive and
exclusive measurements of the heavy fragments (A 10) and their
associated light charged particles (protons and particles) have been
made at the IReS Strasbourg {\sc VIVITRON} Tandem facility at bombarding
energies of Si) = 112 MeV and 180 MeV by using the {\sc ICARE}
charged particle multidetector array. The energy spectra, velocity
distributions, and both in-plane and out-of-plane angular correlations of light
charged particles are compared to statistical-model calculations using a
consistent set of parameters with spin-dependent level densities. The analysis
suggests the onset of large nuclear deformation in Ca at high spin.Comment: 33 pages, 11 figure
Fission fragments mass distributions of nuclei populated by the multinucleon transfer channels of the 18O + 232Th reaction
It is shown that the multinucleon transfer reactions is a powerful tool to study fission of exotic neutron-rich actinide nuclei, which cannot be accessed by particle-capture or heavy-ion fusion reactions. In this work, multinucleon transfer channels of the 18OÂ +Â 232Th reaction are used to study fission of fourteen nuclei 231,232,233,234Th, 232,233,234,235,236Pa, and 234,235,236,237,238U. Identification of fissioning nuclei and of their excitation energy is performed on an event-by-event basis, through the measurement of outgoing ejectile particle in coincidence with fission fragments. Fission fragment mass distributions are measured for each transfer channel, in selected bins of excitation energy. In particular, the mass distributions of 231,234Th and 234,235,236Pa are measured for the first time. Predominantly asymmetric fission is observed at low excitation energies for all studied cases, with a gradual increase of the symmetric mode towards higher excitation energy. The experimental distributions are found to be in general agreement with predictions of the fluctuationâdissipation model
Fission Hindrance in Hot Nuclei
The role of dynamics in fission has attracted much interest since the discovery of this process over fifty years ago. However, the study of the dynamical aspects of fission was for many years hampered by the lack of suitable experimental observables against which theoretical calculations could be tested. For example, it was found that the total kinetic energy release in fission can be described equally well by very different dissipation mechanisms, namely the wall formula, that is based on the collisions of the nucleons with the moving wall of the system, as well as a bulk viscosity of the nuclear matter. Although early theoretical work suggested that the fission process may be described as a diffusion process over the fission barrier, this was largely forgotten because of the success of a purely statistical model which instead of enumerating the ultimate final states of the process argues that the fission rate is determined at the {open_quote}transition state{close_quote} as the system traverses the fission saddle point. It was therefore significant when Gavron showed that the transition state model was unable to describe the number of neutrons emitted prior to scission at high excitation energy in reactions of {sup 16}O+{sup 142}Nd. Subsequent experimental work using different methods to measure the fission dissipation/viscosity has confirmed these initial observations. It was therefore very surprising when Moretto in recent publications concluded that their analysis of fission excitation functions obtained with a and {alpha} and {sup 3}He induced projectiles was perfectly in accord with the transition state model and left no room for fission viscosity. In this paper we`ll show that Moretto`s analysis is flawed by assuming first chance fission only (in direct contradiction to the experimental observation of pre-scission neutron emission in heavy-ion induced fission), and reveal why the systematics presented by Moretto looked so convincing despite these flaws
Response of AGATA Segmented HPGe Detectors to Gamma Rays up to 15.1 MeV
The response of AGATA segmented HPGe detectors to gamma rays in the energy
range 2-15 MeV was measured. The 15.1 MeV gamma rays were produced using the
reaction d(11B,ng)12C at Ebeam = 19.1 MeV, while gamma-rays between 2 to 9 MeV
were produced using an Am-Be-Fe radioactive source. The energy resolution and
linearity were studied and the energy-to-pulse-height conversion resulted to be
linear within 0.05%. Experimental interaction multiplicity distributions are
discussed and compared with the results of Geant4 simulations. It is shown that
the application of gamma-ray tracking allows a suppression of background
radiation following neutron capture by Ge nuclei. Finally the Doppler
correction for the 15.1 MeV gamma line, performed using the position
information extracted with Pulse-shape Analysis, is discussed.Comment: 10 pages, 11 figure
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