Planar Rayleigh scattering results in helium-air mixing experiments in a Mach-6 wind tunnel

Planar Rayleigh scattering measurements with an argon—fluoride excimer laser are performed to investigate helium mixing into air at supersonic speeds. The capability of the Rayleigh scattering technique for flow visualization of a turbulent environment is demonstrated in a large-scale, Mach-6 facility. The detection limit obtained with the present setup indicates that planar, quantitative measurements of density can be made over a large cross-sectional area (5 cm × 10 cm) of the flow field in the absence of clusters

Search for isotope effects in projectile and target ionization in swift He+^+ on H2_2 or D2_2 collisions

Using the cold target recoil ion momentum spectroscopy (COLTRIMS) technique, we have measured the simultaneous projectile and target ionization in collisions of He$^+$ projectiles with a mixture of gaseous H$_2$ and D$_2$ for an incident projectile energy of 650 keV. Motivated by Cooper et al. [Phys. Rev. Lett. 100, 043204 (2008)], we look for differences in the ionization cross section of the two isotopes with the highest resolution and statistical significance. Contributions of the electron-electron and electron-nucleus interactions have been clearly separated kinematically by measuring the longitudinal and transverse momentum of the recoiling ion. We find no significant isotope effect in any of our momentum distributions.Comment: 13 pages, 6 figure

Ion impact induced Interatomic Coulombic Decay in neon and argon dimers

We investigate the contribution of Interatomic Coulombic Decay induced by ion impact in neon and argon dimers (Ne$_2$ and Ar$_2$) to the production of low energy electrons. Our experiments cover a broad range of perturbation strengths and reaction channels. We use 11.37 MeV/u S$^{14+}$, 0.125 MeV/u He$^{1+}$, 0.1625 MeV/u He$^{1+}$ and 0.150 MeV/u He$^{2+}$ as projectiles and study ionization, single and double electron transfer to the projectile as well as projectile electron loss processes. The application of a COLTRIMS reaction microscope enables us to retrieve the three-dimensional momentum vectors of the ion pairs of the fragmenting dimer into Ne$^{q+}$/Ne$^{1+}$ and Ar$^{q+}$/Ar$^{1+}$ (q = 1, 2, 3) in coincidence with at least one emitted electron

Interatomic-Coulombic-decay-induced recapture of photoelectrons in helium dimers

We investigate the onset of photoionization shakeup induced interatomic Coulombic decay (ICD) in He2 at the He+*(n = 2) threshold by detecting two He+ ions in coincidence. We find this threshold to be shifted towards higher energies compared to the same threshold in the monomer. The shifted onset of ion pairs created by ICD is attributed to a recapture of the threshold photoelectron after the emission of the faster ICD electron.Comment: 5 Pages, 2 Figure

Vibrationally Resolved Decay Width of Interatomic Coulombic Decay in HeNe

We investigate the ionization of HeNe from below the He 1s3p excitation to the He ionization threshold. We observe HeNe$^+$ ions with an enhancement by more than a factor of 60 when the He side couples resonantly to the radiation field. These ions are an experimental proof of a two-center resonant photoionization mechanism predicted by Najjari et al. [Phys. Rev. Lett. 105, 153002 (2010)]. Furthermore, our data provide electronic and vibrational state resolved decay widths of interatomic Coulombic decay (ICD) in HeNe dimers. We find that the ICD lifetime strongly increases with increasing vibrational state.Comment: 7 pages, 5 figure

A measurement of the evolution of Interatomic Coulombic Decay in the time domain

During the last 15 years a novel decay mechanism of excited atoms has been discovered and investigated. This so called ''Interatomic Coulombic Decay'' (ICD) involves the chemical environment of the electronically excited atom: the excitation energy is transferred (in many cases over long distances) to a neighbor of the initially excited particle usually ionizing that neighbor. It turned out that ICD is a very common decay route in nature as it occurs across van-der-Waals and hydrogen bonds. The time evolution of ICD is predicted to be highly complex, as its efficiency strongly depends on the distance of the atoms involved and this distance typically changes during the decay. Here we present the first direct measurement of the temporal evolution of ICD using a novel experimental approach.Comment: 6 pages, 4 figures, submitted to PR

Two-particle interference of electron pairs on a molecular level

We investigate the photo-doubleionization of $H_2$ molecules with 400 eV photons. We find that the emitted electrons do not show any sign of two-center interference fringes in their angular emission distributions if considered separately. In contrast, the quasi-particle consisting of both electrons (i.e. the "dielectron") does. The work highlights the fact that non-local effects are embedded everywhere in nature where many-particle processes are involved

Contrail altitude estimation using GOES-16 ABI data and deep learning

The climate impact of persistent aircraft contrails is currently estimated to be comparable to that due to aviation-emitted CO2. A potential near-term and low-cost mitigation option is contrail avoidance, which involves rerouting aircraft around ice-supersaturated regions, preventing the formation of persistent contrails. Current forecasting methods for these regions of ice supersaturation have been found to be inaccurate when compared to in situ measurements. Further assessment and improvements of the quality of these predictions can be realized by comparison with observations of persistent contrails, such as those found in satellite imagery. In order to further enable comparison between these observations and contrail predictions, we develop a deep learning algorithm to estimate contrail altitudes based on GOES-16 Advanced Baseline Imager (ABI) infrared imagery. This algorithm is trained using a dataset of 3267 contrails found within Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) data and achieves a root mean square error (RMSE) of 570 m. The altitude estimation algorithm outputs probability distributions for the contrail top altitude in order to represent predictive uncertainty. The 95 % confidence intervals constructed using these distributions, which are shown to contain approximately 95 % of the contrail data points, are found to be 2.2 km thick on average. These intervals are found to be 34.1 % smaller than the 95 % confidence intervals constructed using flight altitude information alone, which are 3.3 km thick on average. Furthermore, we show that the contrail altitude estimates are consistent in time and, in combination with contrail detections, can be used to observe the persistence and three-dimensional (3D) evolution of contrail-forming regions from satellite images alone

Aristotle’s assertoric syllogistic and modern relevance logic

This paper sets out to evaluate the claim that Aristotle’s Assertoric Syllogistic is a relevance logic or shows significant similarities with it. I prepare the grounds for a meaningful comparison by extracting the notion of relevance employed in the most influential work on modern relevance logic, Anderson and Belnap’s Entailment. This notion is characterized by two conditions imposed on the concept of validity: first, that some meaning content is shared between the premises and the conclusion, and second, that the premises of a proof are actually used to derive the conclusion. Turning to Aristotle’s Prior Analytics, I argue that there is evidence that Aristotle’s Assertoric Syllogistic satisfies both conditions. Moreover, Aristotle at one point explicitly addresses the potential harmfulness of syllogisms with unused premises. Here, I argue that Aristotle’s analysis allows for a rejection of such syllogisms on formal grounds established in the foregoing parts of the Prior Analytics. In a final section I consider the view that Aristotle distinguished between validity on the one hand and syllogistic validity on the other. Following this line of reasoning, Aristotle’s logic might not be a relevance logic, since relevance is part of syllogistic validity and not, as modern relevance logic demands, of general validity. I argue that the reasons to reject this view are more compelling than the reasons to accept it and that we can, cautiously, uphold the result that Aristotle’s logic is a relevance logic