128 research outputs found
Extended Magnetic Dome Induced by Low Pressures in Superconducting FeSeS
We report muon spin rotation (SR) and magnetization measurements under
pressure on FeSeS with x
.Above GPa we find microscopic coexistence of
superconductivity with an extended dome of long range magnetic order that spans
a pressure range between previously reported separated magnetic phases. The
magnetism initially competes on an atomic scale with the coexisting
superconductivity leading to a local maximum and minimum of the superconducting
. The maximum of corresponds to the onset of
magnetism while the minimum coincides with the pressure of strongest
competition. A shift of the maximum of for a series of single
crystals with x up to 0.14 roughly extrapolates to a putative magnetic and
superconducting state at ambient pressure for x .Comment: 10 pages, 6 figures, including supplemental materia
Gradual Enhancement of Stripe-Type Antiferromagnetism in Spin Ladder Material BaFeS Under Pressure
We report pressure-dependent neutron diffraction and muon spin
relaxation/rotation measurements combined with first-principles calculations to
investigate the structural, magnetic, and electronic properties of
BaFeS under pressure. The experimental results reveal a gradual
enhancement of the stripe-type ordering temperature with increasing pressure up
to 2.6 GPa and no observable change in the size of the ordered moment. The ab
initio calculations suggest that the magnetism is highly sensitive to the Fe-S
bond lengths and angles, clarifying discrepancies with previously published
results. In contrast to our experimental observations, the calculations predict
a monotonic reduction of the ordered moment with pressure. We suggest that the
robustness of the stripe-type antiferromagnetism is due to strong electron
correlations not fully considered in the calculations
Universal fluctuating regime in triangular chromate antiferromagnets
We report x-ray diffraction, magnetic susceptibility, heat capacity, H
nuclear magnetic resonance (NMR), and muon spin relaxation (SR)
measurements, as well as density-functional band-structure calculations for the
frustrated triangular lattice Heisenberg antiferromagnet (TLHAF)
-HCrO (trigonal, space group: ). This compound
undergoes a clear magnetic transition at ~K, as seen
from the drop in the muon paramagnetic fraction and concurrent anomalies in the
magnetic susceptibility and specific heat. Local probes (NMR and SR)
reveal a broad regime with slow fluctuations down to , this
temperature corresponding to the maximum in the SR relaxation rate and in
the NMR wipe-out. From the comparison with NaCrO and -KCrO,
the fluctuating regime and slow dynamics below appear to be
hallmarks of the TLHAF with stacking that leads to a frustration of
interlayer couplings between the triangular planes. This interlayer frustration
is a powerful lever to generate spin states with persistent dynamics and may
bear implications to spin-liquid candidates with the triangular geometry.Comment: 14 pages, 11 figures, 2 table
Disordered ground state in the spin-orbit coupled Jeff = 1/2 distorted honeycomb magnet BiYbGeO5
We delineate quantum magnetism in the strongly spin-orbit coupled distorted honeycomb lattice antiferromagnet BiYbGeO5. Our magnetization and heat capacity measurements reveal that its low-temperature behavior is well described by an effective Jeff=12 Kramers doublet of Yb3+. The ground state is nonmagnetic with a tiny spin gap. Temperature-dependent magnetic susceptibility, magnetization isotherm, and heat capacity can be modeled well assuming isolated spin dimers with anisotropic exchange interactions JZ≃2.6 K and JXY≃1.3 K. Heat capacity measurements backed by muon spin relaxation suggest the absence of magnetic long-range order down to at least 80 mK both in zero field and in applied fields. This sets BiYbGeO5 apart from Yb2Si2O7, with its unusual regime of magnon Bose-Einstein condensation, and suggests negligible interdimer couplings, despite only a weak structural deformation of the honeycomb lattice
Surgical site infection after gastrointestinal surgery in high-income, middle-income, and low-income countries: a prospective, international, multicentre cohort study
Background: Surgical site infection (SSI) is one of the most common infections associated with health care, but its importance as a global health priority is not fully understood. We quantified the burden of SSI after gastrointestinal surgery in countries in all parts of the world.
Methods: This international, prospective, multicentre cohort study included consecutive patients undergoing elective or emergency gastrointestinal resection within 2-week time periods at any health-care facility in any country. Countries with participating centres were stratified into high-income, middle-income, and low-income groups according to the UN's Human Development Index (HDI). Data variables from the GlobalSurg 1 study and other studies that have been found to affect the likelihood of SSI were entered into risk adjustment models. The primary outcome measure was the 30-day SSI incidence (defined by US Centers for Disease Control and Prevention criteria for superficial and deep incisional SSI). Relationships with explanatory variables were examined using Bayesian multilevel logistic regression models. This trial is registered with ClinicalTrials.gov, number NCT02662231.
Findings: Between Jan 4, 2016, and July 31, 2016, 13 265 records were submitted for analysis. 12 539 patients from 343 hospitals in 66 countries were included. 7339 (58·5%) patient were from high-HDI countries (193 hospitals in 30 countries), 3918 (31·2%) patients were from middle-HDI countries (82 hospitals in 18 countries), and 1282 (10·2%) patients were from low-HDI countries (68 hospitals in 18 countries). In total, 1538 (12·3%) patients had SSI within 30 days of surgery. The incidence of SSI varied between countries with high (691 [9·4%] of 7339 patients), middle (549 [14·0%] of 3918 patients), and low (298 [23·2%] of 1282) HDI (p < 0·001). The highest SSI incidence in each HDI group was after dirty surgery (102 [17·8%] of 574 patients in high-HDI countries; 74 [31·4%] of 236 patients in middle-HDI countries; 72 [39·8%] of 181 patients in low-HDI countries). Following risk factor adjustment, patients in low-HDI countries were at greatest risk of SSI (adjusted odds ratio 1·60, 95% credible interval 1·05–2·37; p=0·030). 132 (21·6%) of 610 patients with an SSI and a microbiology culture result had an infection that was resistant to the prophylactic antibiotic used. Resistant infections were detected in 49 (16·6%) of 295 patients in high-HDI countries, in 37 (19·8%) of 187 patients in middle-HDI countries, and in 46 (35·9%) of 128 patients in low-HDI countries (p < 0·001).
Interpretation: Countries with a low HDI carry a disproportionately greater burden of SSI than countries with a middle or high HDI and might have higher rates of antibiotic resistance. In view of WHO recommendations on SSI prevention that highlight the absence of high-quality interventional research, urgent, pragmatic, randomised trials based in LMICs are needed to assess measures aiming to reduce this preventable complication
Engineering phase competition between stripe order and superconductivity in LaSrCuO
Unconventional superconductivity often couples to other electronic orders in a cooperative or competing fashion. Identifying external stimuli that tune between these two limits is of fundamental interest. Here, we show that strain perpendicular to the copper-oxide planes couples directly to the competing interaction between charge stripe order and superconductivity in LaSrCuO (LSCO). Compressive c-axis pressure amplifies stripe order within the superconducting state, while having no impact on the normal state. By contrast, strain dramatically diminishes the magnetic field enhancement of stripe order in the superconducting state. These results suggest that c-axis strain acts as tuning parameter of the competing interaction between charge stripe order and superconductivity. This interpretation implies a uniaxial pressure-induced ground state in which the competition between charge order and superconductivity is reduced
Robust block magnetism in the spin ladder compound BaFeSe under hydrostatic pressure
The majority of the iron-based superconductors (FeSCs) exhibit a
two-dimensional square lattice structure. Recent reports of pressure-induced
superconductivity in the spin-ladder system, BaFeX (X =S,Se), introduce
a quasi-one-dimensional prototype and an insulating parent compound to the
FeSCs. Here we report X-ray, neutron diffraction and muon spin relaxation
experiments on BaFeSe under hydrostatic pressure to investigate its
magnetic and structural properties across the pressure-temperature phase
diagram. A structural phase transition was identified at a pressure of 3.7(3)
GPa. Neutron diffraction measurements at 6.8(3) GPa and 120 K show that the
block magnetism persists even at these high pressures. A steady increase and
then fast drop of the magnetic transition temperature and greatly
reduced moment above the pressure indicate potentially rich and competing
phases close to the superconducting phase in this ladder system
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