Colloquium: Beta delayed fission of atomic nuclei

This Colloquium reviews the studies of exotic type of low-energy nuclear fission, the beta-delayed fission (bDF). Emphasis is made on the new data from very neutron-deficient nuclei in the lead region, previously scarcely studied as far as fission is concerned. These data establish the new region of asymmetric fission in addition to the previously known one in the transuranium nuclei. New production and identification techniques, which emerged in the last two decades, such as the wider use of electromagnetic separators and the application of selective laser ionization to produce intense isotopically or even isomerically pure radioactive beams are highlighted. A critical analysis of presently available DF data is presented and the importance of detailed quantitative DF studies, which become possible now, is stressed, along with the recent theory efforts in the domain of low-energy fission

Advancing Radiation-Detected Resonance Ionization towards Heavier Elements and More Exotic Nuclides

RAdiation-Detected Resonance Ionization Spectroscopy (RADRIS) is a versatile method for highly sensitive laser spectroscopy studies of the heaviest actinides. Most of these nuclides need to be produced at accelerator facilities in fusion-evaporation reactions and are studied immediately after their production and separation from the primary beam due to their short half-lives and low production rates of only a few atoms per second or less. Only recently, the first laser spectroscopic investigation of nobelium (Z=102) was performed by applying the RADRIS technique in a buffer-gas-filled stopping cell at the GSI in Darmstadt, Germany. To expand this technique to other nobelium isotopes and for the search for atomic levels in the heaviest actinide element, lawrencium (Z=103), the sensitivity of the RADRIS setup needed to be further improved. Therefore, a new movable double-detector setup was developed, which enhances the overall efficiency by approximately 65% compared to the previously used single-detector setup. Further development work was performed to enable the study of longer-lived (t₁/₂>1 h) and shorter-lived nuclides (t₁/₂<1 s) with the RADRIS method. With a new rotatable multi-detector design, the long-lived isotope 254Fm (t₁/₂=3.2 h) becomes within reach for laser spectroscopy. Upcoming experiments will also tackle the short-lived isotope 251No (t₁/₂=0.8 s) by applying a newly implemented short RADRIS measurement cycle

High-resolution laser system for the S3-Low Energy Branch

In this paper we present the first high-resolution laser spectroscopy results obtained at the GISELE laser laboratory of the GANIL-SPIRAL2 facility, in preparation for the first experiments with the S$^3$-Low Energy Branch. Studies of neutron-deficient radioactive isotopes of erbium and tin represent the first physics cases to be studied at S$^3$. The measured isotope-shift and hyperfine structure data are presented for stable isotopes of these elements. The erbium isotopes were studied using the $4f^{12}6s^2$ $^3H_6 \rightarrow 4f^{12}(^3 H)6s6p$ $J = 5$ atomic transition (415 nm) and the tin isotopes were studied by the $5s^25p^2 (^3P_0) \rightarrow 5s^25p6s (^3P_1)$ atomic transition (286.4 nm), and are used as a benchmark of the laser setup. Additionally, the tin isotopes were studied by the $5s^25p6s (^3P_1) \rightarrow 5s^25p6p (^3P_2)$ atomic transition (811.6 nm), for which new isotope-shift data was obtained and the corresponding field-shift $F_{812}$ and mass-shift $M_{812}$ factors are presented

Shape staggering of midshell mercury isotopes from in-source laser spectroscopy compared with density-functional-theory and Monte Carlo shell-model calculations

Neutron-deficient 177−185Hg isotopes were studied using in-source laser resonance-ionization spectroscopy at the CERN-ISOLDE radioactive ion-beam facility in an experiment combining different detection methods tailored to the studied isotopes. These include either α-decay tagging or multireflection time-of-flight gating for isotope identification. The endpoint of the odd-even nuclear shape staggering in mercury was observed directly by measuring for the first time the isotope shifts and hyperfine structures of 177−180Hg. Changes in the mean-square charge radii for all mentioned isotopes, magnetic dipole, and electric quadrupole moments of the odd-A isotopes and arguments in favor of I=7/2 spin assignment for 177,179Hg were deduced. Experimental results are compared with density functional theory (DFT) and Monte Carlo shell model (MCSM) calculations. DFT calculations using Skyrme parametrizations predict a jump in the charge radius around the neutron N=104 midshell, with an odd-even staggering pattern related to the coexistence of nearly degenerate oblate and prolate minima. This near-degeneracy is highly sensitive to many aspects of the effective interaction, a fact that renders perfect agreement with experiments out of reach for current functionals. Despite this inherent difficulty, the SLy5s1 and a modified UNEDF1SO parametrization predict a qualitatively correct staggering that is off by two neutron numbers. MCSM calculations of states with the experimental spins and parities show good agreement for both electromagnetic moments and the observed charge radii. A clear mechanism for the origin of shape staggering within this context is identified: a substantial change in occupancy of the proton πh9/2 and neutron νi13/2 orbitals

Alpha Decay and Beta-Delayed Fission: Tools for Nuclear Physics Studies

α decay and β-delayed fission are two important decay modes of heavy exotic nuclei. Experimental α decay and β-delayed fission studies deliver significant nuclear-structure information in regions of the nuclear chart with limited accessibility. This information is important to improve the predictability of contemporary nuclear models used for e.g. nuclear astrophysics calculations. The basic principles and the current understanding of α and β-delayed fission decay are introduced. Examples of recent experiments and their impact on the understanding of heavy nuclei are presented

ISOLDE Workshop and Users meeting 2014 "50th Anniversary Edition"

Soon after the commissioning of ISOLDE at the PS-Booster facility, first experiments took place. This contribution will discuss highlights from the 1993-1995 period with a special focus on the preparatory work for the proposal to post-accelerate the ISOLDE beams. This lead eventually to the approval of the "Radioactive beam EXperiments at ISOLDE: Coulomb excitation and neutron transfer reactions of exotic nuclei" proposal under IS347

Physics with REX-ISOLDE: from experiment to facility

The REX-ISOLDE project and its physics program are presented. The innovative approach used to post-accelerate essentially all existing radioactive beams available at ISOLDE to 3 MeV u^−1 is presented and beam properties are discussed. Isotopes as light as 8Li and as heavy as 224Ra have been used for Coulomb excitation, few-nucleon transfer reaction or fusion evaporation studies. Selected examples of the physics program, primarily utilizing the Miniball detector and segmented silicon detector arrays, are presented emphasizing some unique features of REX-ISOLDE. Finally, the HIE-ISOLDE project aiming at, amongst other goals, increasing the beam energy to 5.5 MeV u^−1 and above, will be briefly discussed.status: publishe