29 research outputs found
Nanocalorimetric Evidence for Nematic Superconductivity in the Doped Topological Insulator SrBiSe
Spontaneous rotational-symmetry breaking in the superconducting state of
doped has attracted significant attention as an
indicator for topological superconductivity. In this paper, high-resolution
calorimetry of the single-crystal
provides unequivocal evidence of a two-fold rotational symmetry in the
superconducting gap by a \emph{bulk thermodynamic} probe, a fingerprint of
nematic superconductivity. The extremely small specific heat anomaly resolved
with our high-sensitivity technique is consistent with the material's low
carrier concentration proving bulk superconductivity. The large basal-plane
anisotropy of is attributed to a nematic phase of a two-component
topological gap structure and caused by a
symmetry-breaking energy term .
A quantitative analysis of our data excludes more conventional sources of this
two-fold anisotropy and provides the first estimate for the symmetry-breaking
strength , a value that points to an onset transition of
the second order parameter component below 2K
Interplay of stripe and double-Q magnetism with superconductivity in under the influence of magnetic fields
At
undergoes a
novel first-order transition from a four-fold symmetric double-Q magnetic phase
to a two-fold symmetric single-Q phase, which was argued to occur
simultaneously with the onset of superconductivity (B\"ohmer et al., Nat. Comm.
6, 7911 (2015)). Here, by applying magnetic fields up to 10T, we investigate in
more detail the interplay of superconductivity with this magneto-structural
transition using a combination of high-resolution thermal-expansion and
heat-capacity measurements. We find that a magnetic field suppresses the
reentrance of the single-Q orthorhombic phase more strongly than the
superconducting transition, resulting in a splitting of the zero-field
first-order transition. The suppression rate of the orthorhombic reentrance
transition is stronger for out-of-plane than for in-plane fields and scales
with the anisotropy of the superconducting state. These effects are captured
within a phenomenological Ginzburg-Landau model, strongly suggesting that the
suppression of the reentrant orthorhombic single-Q phase is primarily linked to
the field-induced weakening of the superconducting order. Not captured by this
model is however a strong reduction of the orthorhombic distortion for
out-of-plane fields, which deserves further theoretical attention
Electronic nematicity in URu2Si2 revisited
The nature of the hidden-order (HO) state in URu2Si2 remains one of the major
unsolved issues in heavy-fermion physics. Recently, torque magnetometry, x-ray
diffraction and elastoresistivity data have suggested that the HO phase
transition at THO = 17.5 K is driven by electronic nematic effects. Here, we
search for thermodynamic signatures of this purported structural instability
using anisotropic thermal-expansion, Young\'s modulus, elastoresistivity and
specific-heat measurements. In contrast to the published results, we find no
evidence of a rotational symmetry-breaking in any of our data. Interestingly,
our elastoresistivity measurements, which are in full agreement with published
results, exhibit a Curie-Weiss divergence, which we however attribute to a
volume and not to a symmetry-breaking effect. Finally, clear evidence for
thermal fluctuations is observed in our heat-capacity data, from which we
estimate the HO correlation length.Comment: 4 Figures, 5 page
An electronic nematic liquid in BaNiAs
Understanding the organizing principles of interacting electrons and the emergence of novel electronic phases is a central endeavor of condensed matter physics. Electronic nematicity, in which the discrete rotational symmetry in the electron fluid is broken while the translational one remains unaffected, is a prominent example of such a phase. It has proven ubiquitous in correlated electron systems, and is of prime importance to understand Fe-based superconductors. Here, we find that fluctuations of such broken symmetry are exceptionally strong over an extended temperature range above phase transitions in BaNi(AsP), the nickel homologue to the Fe-based systems. This lends support to a type of electronic nematicity, dynamical in nature, which exhibits a particularly strong coupling to the underlying crystal lattice. Fluctuations between degenerate nematic configurations cause splitting of phonon lines, without lifting degeneracies nor breaking symmetries, akin to spin liquids in magnetic systems
Soft Phonon Mode Triggering Fast Ag Diffusion in Superionic Argyrodite AgGeSe
The structural coexistence of dual rigid and mobile sublattices in superionic Argyrodites yields ultralow lattice thermal conductivity along with decent electrical and ionic conductivities and therefore attracts intense interest for batteries, fuel cells, and thermoelectric applications. However, a comprehensive understanding of their underlying lattice and diffusive dynamics in terms of the interplay between phonons and mobile ions is missing. Herein, inelastic neutron scattering is employed to unravel that phonon softening on heating to T ≈ 350 K triggers fast Ag diffusion in the canonical superionic Argyrodite AgGeSe. Ab initio molecular dynamics simulations reproduce the experimental neutron scattering signals and identify the partially ultrafast Ag diffusion with a large diffusion coefficient of 10 cm s. The study illustrates the microscopic interconnection between soft phonons and mobile ions and provides a paradigm for an intertwined interaction of the lattice and diffusive dynamics in superionic materials
Charge density wave transitions, soft phonon, and possible electronic nematicity in BaNi₂(As₁₋ₓPₓ)₂
A detailed investigation of BaNi2(As1−xPx)2 single crystals using high-resolution thermal-expansion, heat-capacity, Young\u27s-modulus, and resistivity measurements is presented. The phase diagram of BaNi2(As1−xPx)2 is shown to be much richer than suggested by the original data of Kudo et al. [Phys. Rev. Lett. 109, 097002 (2012)]. The transition to the commensurate charge density wave (C-CDW) is always preceded by a fourfold symmetry-breaking transition associated with the long-range ordering of a strongly fluctuating unidirectional incommensurate charge density wave (I-CDW). Significant precursors above the I-CDW and C-CDW transitions are seen in the thermal expansion and resistivity and are particularly evident in the temperature dependence of the c/a ratio of the lattice parameters. Heat-capacity measurements of the crystals with a higher P content and a higher critical temperature of 3.2 K uncover a Debye-like behavior of a soft-phonon mode with a very low ΘDebye of roughly 50 K. Associated with this soft phonon are unusually large thermal-expansion anomalies, resulting in logarithmically diverging uniaxial phonon Grüneisen parameters. Young\u27s-modulus data of these higher-Tc crystals exhibit a significant softening in both B1g and B2g channels, which is argued to be incompatible with nematic criticality and is rather associated with a broad phase transition to an hitherto unknown structure. Possible origins of the increase in the superconducting critical temperature with P substitution are discussed
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Amorphous-Like Ultralow Thermal Transport in Crystalline Argyrodite Cu7PS6
Due to their amorphous-like ultralow lattice thermal conductivity both below and above the superionic phase transition, crystalline Cu- and Ag-based superionic argyrodites have garnered widespread attention as promising thermoelectric materials. However, despite their intriguing properties, quantifying their lattice thermal conductivities and a comprehensive understanding of the microscopic dynamics that drive these extraordinary properties are still lacking. Here, an integrated experimental and theoretical approach is adopted to reveal the presence of Cu-dominated low-energy optical phonons in the Cu-based argyrodite Cu7PS6. These phonons yield strong acoustic-optical phonon scattering through avoided crossing, enabling ultralow lattice thermal conductivity. The Unified Theory of thermal transport is employed to analyze heat conduction and successfully reproduce the experimental amorphous-like ultralow lattice thermal conductivities, ranging from 0.43 to 0.58 W m−1 K−1, in the temperature range of 100–400 K. The study reveals that the amorphous-like ultralow thermal conductivity of Cu7PS6 stems from a significantly dominant wave-like conduction mechanism. Moreover, the simulations elucidate the wave-like thermal transport mainly results from the contribution of Cu-associated low-energy overlapping optical phonons. This study highlights the crucial role of low-energy and overlapping optical modes in facilitating amorphous-like ultralow thermal transport, providing a thorough understanding of the underlying complex dynamics of argyrodites
Reconstructing the Deep Population History of Central and South America
We report genome-wide ancient DNA from 49 individuals forming four parallel time transects in Belize, Brazil, the Central Andes, and the Southern Cone, each dating to at least 9,000 years ago. The common ancestral population radiated rapidly from just one of the two early branches that contributed to Native Americans today. We document two previously unappreciated streams of gene flow between North and South America. One affected the Central Andes by 4,200 years ago, while the other explains an affinity between the oldest North American genome associated with the Clovis culture and the oldest Central and South Americans from Chile, Brazil, and Belize. However, this was not the primary source for later South Americans, as the other ancient individuals derive from lineages without specific affinity to the Clovis-associated genome, suggesting a population replacement that began at least 9,000 years ago and was followed by substantial population continuity in multiple regions
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Ancestral diversity improves discovery and fine-mapping of genetic loci for anthropometric traits - the Hispanic/Latino Anthropometry Consortium
Hispanic/Latinos have been underrepresented in genome-wide association studies (GWAS) for anthropometric traits despite their notable anthropometric variability, ancestry proportions, and high burden of growth stunting and overweight/obesity. To address this knowledge gap, we analyzed densely-imputed genetic data in a sample of Hispanic/Latino adults to identify and fine-map genetic variants associated with body mass index (BMI), height, and BMI-adjusted waist-to-hip ratio (WHRadjBMI). We conducted a GWAS of 18 studies/consortia as part of the Hispanic/Latino Anthropometry (HISLA) Consortium (Stage 1, n=59,771) and generalized our findings in 9 additional studies (HISLA Stage 2, n=10,538). We conducted a trans-ancestral GWAS with summary statistics from HISLA Stage 1 and existing consortia of European and African ancestries. In our HISLA Stage 1+2 analyses, we discovered one BMI locus, as well as two BMI signals and another height signal each within established anthropometric loci. In our trans-ancestral meta-analysis, we discovered three BMI loci, one height locus, and one WHRadjBMI locus. We also identified three secondary signals for BMI, 28 for height, and two for WHRadjBMI in established loci. We show that 336 known BMI, 1,177 known height, and 143 known WHRadjBMI (combined) SNPs demonstrated suggestive transferability (nominal significance and effect estimate directional consistency) in Hispanic/Latino adults. Of these, 36 BMI, 124 height, and 11 WHRadjBMI SNPs were significant after trait-specific Bonferroni correction. Trans-ancestral meta-analysis of the three ancestries showed a small-to-moderate impact of uncorrected population stratification on the resulting effect size estimates. Our findings demonstrate that future studies may also benefit from leveraging diverse ancestries and differences in linkage disequilibrium patterns to discover novel loci and additional signals with less residual population stratification