13 research outputs found
Heavy fermion superconductivity in the filled skutterudite compound PrOsSb
The filled skutterudite compound \PrOsSb{} has been found to exhibit
superconductivity with a critical temperature K that
develops out of a heavy Fermi liquid with an effective mass . The current experimental situation regarding the heavy fermion
state, the superconducting state, and a high field, low temperature phase that
is apparently associated with magnetic or quadrupolar order in \PrOsSb{} is
briefly reviewed herein.Comment: 4 pages, 2 figures, presented at the LT23 23rd International
Conference on Low Temperature Physics, Hiroshima, Japa
Superconductivity and crystalline electric field effects in the filled skutterudite series Pr(OsRu)Sb
X-ray powder diffraction, magnetic susceptibility , and electrical
resistivity measurements were made on single crystals of the filled
skutterudite series Pr(OsRu)Sb. One end of the series
() is a heavy fermion superconductor with a superconducting critical
temperature K, while the other end () is a conventional
superconductor with K. The lattice constant decreases
approximately linearly with increasing Ru concentration . As Ru (Os) is
substituted for Os (Ru), decreases nearly linearly with substituent
concentration and exhibits a minimum with a value of K at , suggesting that the two types of superconductivity compete with one
another. Crystalline electric field (CEF) effects in and
due to the splitting of the Pr nine-fold degenerate Hund's
rule multiplet are observed throughout the series, with the splitting
between the ground state and the first excited state increasing monotonically
as increases. The fits to the and data are
consistent with a doublet ground state for all values of x,
although reasonable fits can be obtained for a ground state for
values near the end member compounds ( or ).Comment: 10 pages, 8 figures, submitted to Phys. Rev.
Unusual giant magnetostriction in the ferrimagnet GdCaMnO
We report an unusual giant linear magnetostrictive effect in the ferrimagnet
GdCaMnO (80 K). Remarkably, the
magnetostriction, negative at high temperature (), becomes
positive below 15 K when the magnetization of the Gd sublattice overcomes the
magnetization of the Mn sublattice. A rather simple model where the magnetic
energy competes against the elastic energy gives a good account of the observed
results and confirms that Gd plays a crucial role in this unusual observation.
Unlike previous works in manganites where only striction associated with 3
Mn orbitals is considered, our results show that the lanthanide 4 orbitals
related striction can be very important too and it cannot be disregarded.Comment: 6 pages, 3 figure
Heat capacity studies of Ce and Rh site substitution in the heavy fermion antiferromagnet CeRhIn_5;: Short-range magnetic interactions and non-Fermi-liquid behavior
In heavy fermion materials superconductivity tends to appear when long range
magnetic order is suppressed by chemical doping or applying pressure. Here we
report heat capacity measurements on diluted alloyes of the heavy fermion
superconductor CeRhIn_5;. Heat capacity measurements have been performed on
CeRh_{1-y}Ir_{y}In_5; (y <= 0.10) and Ce_{1-x}La_{x}Rh_{1-y}Ir_{y}In_5; (x <=
0.50) in applied fields up to 90 kOe to study the affect of doping and magnetic
field on the magnetic ground state. The magnetic phase diagram of
CeRh_{0.9}Ir_{0.1}In_5; is consistent with the magnetic structure of CeRhIn_5;
being unchanged by Ir doping. Doping of Ir in small concentrations is shown to
slightly increase the antiferromagnetic transition temperature T_{N} (T_{N}=3.8
K in the undoped sample). La doping which causes disorder on the Ce sublattice
is shown to lower T_{N} with no long range order observed above 0.34 K for
Ce_{0.50}La_{0.50}RhIn_5;. Measurements on Ce_{0.50}La_{0.50}RhIn_5; show a
coexistence of short range magnetic order and non-Fermi-liquid behavior. This
dual nature of the Ce 4f-electrons is very similar to the observed results on
CeRhIn_5; when long range magnetic order is suppressed at high pressure.Comment: 8 pages, 9 figure
Field-controlled magnetic order in the quantum spin-ladder system (Hpip)2CuBr4
International audienceNeutron diffraction is used to investigate the field-induced, antiferromagnetically ordered state in the two-leg spin-ladder material (Hpip)2CuBr4. This âclassicalâ phase, a consequence of weak interladder coupling, is nevertheless highly unconventional: its properties are influenced strongly by the spin Luttinger-liquid state of the ladder subunits. We determine directly the order parameter (transverse magnetization), the ordering temperature, the spin structure, and the critical exponents around the transition. We introduce a minimal microscopic model for the interladder coupling and calculate the quantum fluctuation corrections to the mean-field interaction
Magnetic structure of CeRhIn_5 as a function of pressure and temperature
We report magnetic neutron-diffraction and electrical resistivity studies on
single crystals of the heavy-fermion antiferromagnet CeRhIn at pressures
up to 2.3 GPa. These experiments show that the staggered moment of Ce and the
incommensurate magnetic structure change weakly with applied pressure up to
1.63 GPa, where resistivity, specific heat and NQR measurements confirm the
presence of bulk superconductivity. This work places new constraints on an
interpretation of the relationship between antiferromagnetism and
unconventional superconductivity in CeRhIn.Comment: 6 pages, 6 figures, submitted to Phys. Rev.
Non-Fermi Liquid Regimes and Superconductivity in the Low Temperature Phase Diagrams of Strongly Correlated d- and f-Electron Materials
Integrated chemiresistor and work function microsensor array with carbon black/polymer composite materials
An array of chemically-sensitive field-effect transistors (CHEMFETs) that measure both work function and bulk resistance changes in thin films was used to detect volatile organic compounds. Carbon black/organic polymer composite films were deposited onto the CHEMFETs using an automated microdispensing method
Evolution of the Kondo lattice electronic structure above the transport coherence temperature
The temperature-dependent evolution of the Kondo lattice is a long-standing topic of theoretical and experimental investigation and yet it lacks a truly microscopic description of the relation of the basic f-c hybridization processes to the fundamental temperature scales of Kondo screening and Fermi-liquid lattice coherence. Here, the temperature dependence of f-c hybridized band dispersions and Fermi-energy f spectral weight in the Kondo lattice system CeCoIn5 is investigated using f-resonant angle-resolved photoemission spectroscopy (ARPES) with sufficient detail to allow direct comparison to first-principles dynamical mean-field theory (DMFT) calculations containing full realism of crystalline electric-field states. The ARPES results, for two orthogonal (001) and (100) cleaved surfaces and three different f-c hybridization configurations, with additional microscopic insight provided by DMFT, reveal f participation in the Fermi surface at temperatures much higher than the lattice coherence temperature, T* approximate to 45 K, commonly believed to be the onset for such behavior. The DMFT results show the role of crystalline electric-field (CEF) splittings in this behavior and a T-dependent CEF degeneracy crossover below T* is specifically highlighted. A recent ARPES report of low T Luttinger theorem failure for CeCoIn5 is shown to be unjustified by current ARPES data and is not found in the theory.11Nsciescopu
Magnetization dynamics and frustration in the multiferroic double perovskite Lu2MnCoO6
We investigate the magnetic ordering and the magnetization dynamics (from kHz to THz time scales) of the double perovskite Lu2MnCoO6 using elastic neutron diffraction, muon spin relaxation, and micro-Hall magnetization measurements. This compound is known to be a type II multiferroic with the interesting feature that a ferromagneticlike magnetization hysteresis loop couples to an equally hysteretic electric polarization in the bulk of the material despite a zero-field magnetic ordering of the type ââââ along Co-Mn spin chains. Here we explore the unusual dynamics of this compound and find extremely strong fluctuations, consistent with the axial next-nearest-neighbor Ising (ANNNI) model for frustrated spin chains. We identify three temperature scales in Lu2MnCoO6 corresponding to the onset of highly fluctuating long-range order below TN=50±3 K identified from neutron scattering, the onset of magnetic and electric hysteresis, with change in kHz magnetic and electric dynamics below a 30 K temperature scale, and partial freezing of âŒMHz spin fluctuations in the muon spin relaxation data below 12±3 K. Our results provide a framework for understanding the multiferroic behavior of this compound and its hysteresis and dynamics