82 research outputs found
Doppler-free Two-Photon Electronic Spectra of Large Molecules with Resolution Near the Natural Linewidth
Damagnetization cooling of a gas
We demonstrate demagnetization cooling of a gas of ultracold Cr atoms.
Demagnetization is driven by inelastic dipolar collisions which couple the
motional degrees of freedom to the spin degree. By that kinetic energy is
converted into magnetic work with a consequent temperature reduction of the
gas. Optical pumping is used to magnetize the system and drive continuous
demagnetization cooling. Applying this technique, we can increase the phase
space density of our sample by one order of magnitude, with nearly no atom
loss. This method can be in principle extended to every dipolar system and
could be used to achieve quantum degeneracy via optical means.Comment: 10 pages, 5 figure
Precision measurements and test of molecular theory in highly excited vibrational states of H2 (v = 11)
High-fidelity quantum driving
The ability to accurately control a quantum system is a fundamental
requirement in many areas of modern science such as quantum information
processing and the coherent manipulation of molecular systems. It is usually
necessary to realize these quantum manipulations in the shortest possible time
in order to minimize decoherence, and with a large stability against
fluctuations of the control parameters. While optimizing a protocol for speed
leads to a natural lower bound in the form of the quantum speed limit rooted in
the Heisenberg uncertainty principle, stability against parameter variations
typically requires adiabatic following of the system. The ultimate goal in
quantum control is to prepare a desired state with 100% fidelity. Here we
experimentally implement optimal control schemes that achieve nearly perfect
fidelity for a two-level quantum system realized with Bose-Einstein condensates
in optical lattices. By suitably tailoring the time-dependence of the system's
parameters, we transform an initial quantum state into a desired final state
through a short-cut protocol reaching the maximum speed compatible with the
laws of quantum mechanics. In the opposite limit we implement the recently
proposed transitionless superadiabatic protocols, in which the system perfectly
follows the instantaneous adiabatic ground state. We demonstrate that
superadiabatic protocols are extremely robust against parameter variations,
making them useful for practical applications.Comment: 17 pages, 4 figure
Frequency comb transferred by surface plasmon resonance
Frequency combs, millions of narrow-linewidth optical modes referenced to an atomic clock, have shown remarkable potential in time/frequency metrology, atomic/molecular spectroscopy and precision LIDARs. Applications have extended to coherent nonlinear Raman spectroscopy of molecules and quantum metrology for entangled atomic qubits. Frequency combs will create novel possibilities in nano-photonics and plasmonics; however, its interrelation with surface plasmons is unexplored despite the important role that plasmonics plays in nonlinear spectroscopy and quantum optics through the manipulation of light on a sub-wavelength scale. Here, we demonstrate that a frequency comb can be transformed to a plasmonic comb in plasmonic nanostructures and reverted to the original frequency comb without noticeable degradation of <6.51 x 10(-19) in absolute position, 2.92 x 10(-19) in stability and 1Hz in linewidth. The results indicate that the superior performance of a well-defined frequency comb can be applied to nanoplasmonic spectroscopy, quantum metrology and subwavelength photonic circuits.open
Resolved Sideband Cooling of a Micromechanical Oscillator
Micro- and nanoscale opto-mechanical systems provide radiation pressure
coupling of optical and mechanical degree of freedom and are actively pursued
for their ability to explore quantum mechanical phenomena of macroscopic
objects. Many of these investigations require preparation of the mechanical
system in or close to its quantum ground state. Remarkable progress in ground
state cooling has been achieved for trapped ions and atoms confined in optical
lattices. Imperative to this progress has been the technique of resolved
sideband cooling, which allows overcoming the inherent temperature limit of
Doppler cooling and necessitates a harmonic trapping frequency which exceeds
the atomic species' transition rate. The recent advent of cavity back-action
cooling of mechanical oscillators by radiation pressure has followed a similar
path with Doppler-type cooling being demonstrated, but lacking inherently the
ability to attain ground state cooling as recently predicted. Here we
demonstrate for the first time resolved sideband cooling of a mechanical
oscillator. By pumping the first lower sideband of an optical microcavity,
whose decay rate is more than twenty times smaller than the eigen-frequency of
the associated mechanical oscillator, cooling rates above 1.5 MHz are attained.
Direct spectroscopy of the motional sidebands reveals 40-fold suppression of
motional increasing processes, which could enable reaching phonon occupancies
well below unity (<0.03). Elemental demonstration of resolved sideband cooling
as reported here should find widespread use in opto-mechanical cooling
experiments. Apart from ground state cooling, this regime allows realization of
motion measurement with an accuracy exceeding the standard quantum limit.Comment: 13 pages, 5 figure
An Integrated-Photonics Optical-Frequency Synthesizer
Integrated-photonics microchips now enable a range of advanced
functionalities for high-coherence applications such as data transmission,
highly optimized physical sensors, and harnessing quantum states, but with
cost, efficiency, and portability much beyond tabletop experiments. Through
high-volume semiconductor processing built around advanced materials there
exists an opportunity for integrated devices to impact applications cutting
across disciplines of basic science and technology. Here we show how to
synthesize the absolute frequency of a lightwave signal, using integrated
photonics to implement lasers, system interconnects, and nonlinear frequency
comb generation. The laser frequency output of our synthesizer is programmed by
a microwave clock across 4 THz near 1550 nm with 1 Hz resolution and
traceability to the SI second. This is accomplished with a heterogeneously
integrated III/V-Si tunable laser, which is guided by dual
dissipative-Kerr-soliton frequency combs fabricated on silicon chips. Through
out-of-loop measurements of the phase-coherent, microwave-to-optical link, we
verify that the fractional-frequency instability of the integrated photonics
synthesizer matches the reference-clock instability for a 1
second acquisition, and constrain any synthesis error to while
stepping the synthesizer across the telecommunication C band. Any application
of an optical frequency source would be enabled by the precision optical
synthesis presented here. Building on the ubiquitous capability in the
microwave domain, our results demonstrate a first path to synthesis with
integrated photonics, leveraging low-cost, low-power, and compact features that
will be critical for its widespread use.Comment: 10 pages, 6 figure
Spatial and Spectral Coherent Control with Frequency Combs
Quantum coherent control (1-3) is a powerful tool for steering the outcome of
quantum processes towards a desired final state, by accurate manipulation of
quantum interference between multiple pathways. Although coherent control
techniques have found applications in many fields of science (4-9), the
possibilities for spatial and high-resolution frequency control have remained
limited. Here, we show that the use of counter-propagating broadband pulses
enables the generation of fully controlled spatial excitation patterns. This
spatial control approach also provides decoherence reduction, which allows the
use of the high frequency resolution of an optical frequency comb (10,11). We
exploit the counter-propagating geometry to perform spatially selective
excitation of individual species in a multi-component gas mixture, as well as
frequency determination of hyperfine constants of atomic rubidium with
unprecedented accuracy. The combination of spectral and spatial coherent
control adds a new dimension to coherent control with applications in e.g
nonlinear spectroscopy, microscopy and high-precision frequency metrology.Comment: 12 page
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