254 research outputs found

    Search for weak M1 transitions in 48^{48}Ca with inelastic proton scattering

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    The spinflip M1 resonance in the doubly magic nucleus 48^{48}Ca, dominated by a single transition, serves as a reference case for the quenching of spin-isospin modes in nuclei. The aim of the present work is a search for weak M1 transitions in 48^{48}Ca with a high-resolution (p,p') experiment at 295 MeV and forward angles including 0 degree and a comparison to results from a similar study using backward-angle electron scattering at low momentum transfers in order to estimate their contribution to the total B(M1) strength. M1 cross sections of individual peaks in the spectra are deduced with a multipole decomposition analysis. The corresponding reduced B(M1) transition strengths are extracted following the approach outlined in J. Birkhan et al., Phys. Rev. C 93, 041302(R) (2016). In total, 29 peaks containing a M1 contribution are found in the excitation energy region 7 - 13 MeV. The resulting B(M1) strength distribution compares well to the electron scattering results considering different factors limiting the sensitivity in both experiments and the enhanced importance of mechanisms breaking the proportionality of nuclear cross sections and electromagnetic matrix elements for weak transitions as studied here. The total strength of 1.19(6) μN2\mu_N^2 deduced assuming a non-quenched isoscalar part of the (p,p') cross sections agrees with the (e,e') result of 1.21(13) μN2\mu_N^2. A binwise analysis above 10 MeV provides an upper limit of 1.62(23) μN2\mu_N^2. The present results confirm that weak transitions contribute about 25% to the total B(M1) strength in 48^{48}Ca and the quenching factors of GT and spin-M1 strength are comparable in fp-shell nuclei. Thus, the role of of meson exchange currents seems to be neglible, in contrast to sd-shell nuclei.Comment: 11 pages, 9 figures, revised analysis with oxygen contamination remove

    GRIDKIT: Pluggable overlay networks for Grid computing

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    A `second generation' approach to the provision of Grid middleware is now emerging which is built on service-oriented architecture and web services standards and technologies. However, advanced Grid applications have significant demands that are not addressed by present-day web services platforms. As one prime example, current platforms do not support the rich diversity of communication `interaction types' that are demanded by advanced applications (e.g. publish-subscribe, media streaming, peer-to-peer interaction). In the paper we describe the Gridkit middleware which augments the basic service-oriented architecture to address this particular deficiency. We particularly focus on the communications infrastructure support required to support multiple interaction types in a unified, principled and extensible manner-which we present in terms of the novel concept of pluggable overlay networks

    Ultrafast optical nonlinearity in quasi-one-dimensional Mott-insulator Sr2CuO3{\rm Sr_2CuO_3}

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    We report strong instantaneous photoinduced absorption (PA) in the quasi-one-dimensional Mott insulator Sr2CuO3{\rm Sr_2CuO_3} in the IR spectral region. The observed PA is to an even-parity two-photon state that occurs immediately above the absorption edge. Theoretical calculations based on a two-band extended Hubbard model explains the experimental features and indicates that the strong two-photon absorption is due to a very large dipole-coupling between nearly degenerate one- and two-photon states. Room temperature picosecond recovery of the optical transparency suggests the strong potential of Sr2CuO3{\rm Sr_2CuO_3} for all-optical switching.Comment: 10 pages, 4 figure

    A theoretical investigation of the low lying electronic structure of poly(p-phenylene vinylene)

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    The two-state molecular orbital model of the one-dimensional phenyl-based semiconductors is applied to poly(p-phenylene vinylene). The energies of the low-lying excited states are calculated using the density matrix renormalization group method. Calculations of both the exciton size and the charge gap show that there are both Bu and Ag excitonic levels below the band threshold. The energy of the 1Bu exciton extrapolates to 2.60 eV in the limit of infinite polymers, while the energy of the 2Ag exciton extrapolates to 2.94 eV. The calculated binding energy of the 1Bu exciton is 0.9 eV for a 13 phenylene unit chain and 0.6 eV for an infinite polymer. This is expected to decrease due to solvation effects. The lowest triplet state is calculated to be at ca. 1.6 eV, with the triplet-triplet gap being ca. 1.6 eV. A comparison between theory, and two-photon absorption and electroabsorption is made, leading to a consistent picture of the essential states responsible for most of the third-order nonlinear optical properties. An interpretation of the experimental nonlinear optical spectroscopies suggests an energy difference of ca. 0.4 eV between the vertical energy and ca. 0.8 eV between the relaxed energy, of the 1Bu exciton and the band gap, respectively.Comment: LaTeX, 19 pages, 7 eps figures included using epsf. To appear in Physical Review B, 199

    Quantum flutter of supersonic particles in one-dimensional quantum liquids

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    The non-equilibrium dynamics of strongly correlated many-body systems exhibits some of the most puzzling phenomena and challenging problems in condensed matter physics. Here we report on essentially exact results on the time evolution of an impurity injected at a finite velocity into a one-dimensional quantum liquid. We provide the first quantitative study of the formation of the correlation hole around a particle in a strongly coupled many-body quantum system, and find that the resulting correlated state does not come to a complete stop but reaches a steady state which propagates at a finite velocity. We also uncover a novel physical phenomenon when the impurity is injected at supersonic velocities: the correlation hole undergoes long-lived coherent oscillations around the impurity, an effect we call quantum flutter. We provide a detailed understanding and an intuitive physical picture of these intriguing discoveries, and propose an experimental setup where this physics can be realized and probed directly.Comment: 13 pages, 9 figure

    Three Essential Ribonucleases—RNase Y, J1, and III—Control the Abundance of a Majority of Bacillus subtilis mRNAs

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    Bacillus subtilis possesses three essential enzymes thought to be involved in mRNA decay to varying degrees, namely RNase Y, RNase J1, and RNase III. Using recently developed high-resolution tiling arrays, we examined the effect of depletion of each of these enzymes on RNA abundance over the whole genome. The data are consistent with a model in which the degradation of a significant number of transcripts is dependent on endonucleolytic cleavage by RNase Y, followed by degradation of the downstream fragment by the 5′–3′ exoribonuclease RNase J1. However, many full-size transcripts also accumulate under conditions of RNase J1 insufficiency, compatible with a model whereby RNase J1 degrades transcripts either directly from the 5′ end or very close to it. Although the abundance of a large number of transcripts was altered by depletion of RNase III, this appears to result primarily from indirect transcriptional effects. Lastly, RNase depletion led to the stabilization of many low-abundance potential regulatory RNAs, both in intergenic regions and in the antisense orientation to known transcripts

    Theory of excited state absorptions in phenylene-based π\pi-conjugated polymers

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    Within a rigid-band correlated electron model for oligomers of poly-(paraphenylene) (PPP) and poly-(paraphenylenevinylene) (PPV), we show that there exist two fundamentally different classes of two-photon Ag_g states in these systems to which photoinduced absorption (PA) can occur. At relatively lower energies there occur Ag_g states which are superpositions of one electron - one hole (1e--1h) and two electron -- two hole (2e--2h) excitations, that are both comprised of the highest delocalized valence band and the lowest delocalized conduction band states only. The dominant PA is to one specific member of this class of states (the mAg_g). In addition to the above class of Ag_g states, PA can also occur to a higher energy kAg_g state whose 2e--2h component is {\em different} and has significant contributions from excitations involving both delocalized and localized bands. Our calculated scaled energies of the mAg_g and the kAg_g agree reasonably well to the experimentally observed low and high energy PAs in PPV. The calculated relative intensities of the two PAs are also in qualitative agreement with experiment. In the case of ladder-type PPP and its oligomers, we predict from our theoretical work a new intense PA at an energy considerably lower than the region where PA have been observed currently. Based on earlier work that showed that efficient charge--carrier generation occurs upon excitation to odd--parity states that involve both delocalized and localized bands, we speculate that it is the characteristic electronic nature of the kAg_g that leads to charge generation subsequent to excitation to this state, as found experimentally.Comment: Revtex4 style, 2 figures inserted in the text, three tables, 10 page

    Electromagnetic properties of 21O for benchmarking nuclear Hamiltonians

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    The structure of exotic nuclei provides valuable tests for state-of-the-art nuclear theory. In particular electromagnetic transition rates are more sensitive to aspects of nuclear forces and many-body physics than excitation energies alone. We report the first lifetime measurement of excited states in 21^{21}O, finding τ1/2+=42032+35(stat)12+34(sys)\tau_{1/2^+}=420^{+35}_{-32}\text{(stat)}^{+34}_{-12}\text{(sys)}\,ps. This result together with the deduced level scheme and branching ratio of several γ\gamma-ray decays are compared to both phenomenological shell-model and ab initio calculations based on two- and three-nucleon forces derived from chiral effective field theory. We find that the electric quadrupole reduced transition probability of $\rm B(E2;1/2^+ \rightarrow 5/2^+_{g.s.}) = 0.71^{+0.07\ +0.02}_{-0.06\ -0.06} e~e^2fmfm^4,derivedfromthelifetimeofthe, derived from the lifetime of the 1/2^+$ state, is smaller than the phenomenological result where standard effective charges are employed, suggesting the need for modifications of the latter in neutron-rich oxygen isotopes. We compare this result to both large-space and valence-space ab initio calculations, and by using multiple input interactions we explore the sensitivity of this observable to underlying details of nuclear forces.Comment: 23 pages, 3 figure

    In Vivo Methods for the Assessment of Topical Drug Bioavailability

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    This paper reviews some current methods for the in vivo assessment of local cutaneous bioavailability in humans after topical drug application. After an introduction discussing the importance of local drug bioavailability assessment and the limitations of model-based predictions, the focus turns to the relevance of experimental studies. The available techniques are then reviewed in detail, with particular emphasis on the tape stripping and microdialysis methodologies. Other less developed techniques, including the skin biopsy, suction blister, follicle removal and confocal Raman spectroscopy techniques are also described
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