191 research outputs found
Lifetime measurements in Co and Co
Lifetimes of the and states in Co and the
state in Co were measured using the recoil distance Doppler
shift and the differential decay curve methods. The nuclei were populated by
multi-nucleon transfer reactions in inverse kinematics. Gamma rays were
measured with the EXOGAM Ge array and the recoiling fragments were fully
identified using the large-acceptance VAMOS spectrometer. The E2 transition
probabilities from the and states to the ground
state could be extracted in Co as well as an upper limit for the
(E2) value in Co. The experimental
results were compared to large-scale shell-model calculations in the and
model spaces, allowing to draw conclusions on the single-particle
or collective nature of the various states.Comment: 8 pages, 8 figures, 1 table, accepted for publication in Physical
Review
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Statistical description of laser damage initiation in NIF and LMJ optics at 355 nm
Understanding the �extreme statistics� of failure at a weak link allows extrapolation of the results of small area laser damage tests to predict damage levels for the large areas pertinent to NIF/LMJ. Conceptually, it is important to focus on the fluence dependence of the surface density of damage sites. Results of different types of damage tests can be reported in terms of this sample characteristic property
First spectroscopy of Se and As: Investigating shape coexistence beyond the N = Z line
The experiment was performed at the National Superconducting Cyclotron Laboratory (NSCL), at Michigan State University (USA).We report on the first γ spectroscopy of 66Se and 65As from two-neutron removal at intermediate beam energies. The deduced excitation energies for the first-excited states in 66Se and 65As are compared to mean-field-based predictions within a collective Hamiltonian formalism using the Gogny D1S effective interaction and to state-of-the-art shell-model calculations restricted to the pf5/2 g9/2 valence space. The obtained Coulomb-energy differences for the first excited states in 66Se and 65As are discussed within the shell-model formalism to assess the shape-coexistence picture for both nuclei. Our results support a favored oblate ground-state deformation in 66Se and 65As. A shape transition for the ground state of even-odd As isotopes from oblate in 65As to prolate in 67,69,71As is suggested
Can Arginine Inhibit Insulin Aggregation? A Combined Protein Crystallography, Capillary Electrophoresis, and Molecular Simulation Study
The oligomeric state of the storage form of human insulin in the pancreas, which may be affected by several endogenous components of β-cell storage granules such as arginine, is not known. Here, the effect of arginine on insulin oligomerization is investigated independently by protein crystallography, molecular dynamics simulations, and capillary electrophoresis. The combined results point to a strong effect of ionic strength on insulin assembly. Molecular simulations and electrophoretic measurements at low/mM salt concentrations show no significant effect of arginine on insulin aggregation. In contrast, crystallographic data at high/molar ionic strength indicate inhibition of insulin hexamerization by arginine due to its binding at the site relevant for intermolecular contacts, which was also observed in MD simulations. Our results thus bracket the in vivo situation in pancreatic β-cell storage granules, where the ionic strength is estimated to be in the hundreds of millimolar to submolar range. The present findings add to a molecular understanding of in vivo insulin oligomerization and storage, with additional implications for insulin stability in arginine-rich injections
Character of particle-hole excitations in 94 Ru deduced from gamma-ray angular correlation and linear polarization measurements
Regulatory Trust in EU Free Movement Law Adopting the Level of Protection of the Other?
Noncovalent Interactions of Hydrated DNA and RNA Mapped by 2D-IR Spectroscopy
Biomolecules couple to their aqueous environment through a variety of
noncovalent interactions. Local structures at the surface of DNA and RNA are
frequently determined by hydrogen bonds with water molecules, complemented by
non-specific electrostatic and many-body interactions. Structural fluctuations
of the water shell result in fluctuating Coulomb forces on polar and/or ionic
groups of the biomolecular structure and in a breaking and reformation of
hydrogen bonds. Two-dimensional infrared (2D-IR) spectroscopy of vibrational
modes of DNA and RNA gives insight into local hydration geometries, elementary
molecular dynamics, and the mechanisms behind them. In this chapter, recent
results from 2D-IR spectroscopy of native and artificial DNA and RNA are
presented, together with theoretical calculations of molecular couplings and
molecular dynamics simulations. Backbone vibrations of DNA and RNA are
established as sensitive noninvasive probes of the complex behavior of hydrated
helices. The results reveal the femtosecond fluctuation dynamics of the water
shell, the short-range character of Coulomb interactions, and the strength and
fluctuation amplitudes of interfacial electric fields.Comment: To appear as Chapter 8 of Springer Series in Optical Sciences:
Coherent Multidimensional Spectroscopy -- Editors: Cho, Minhaeng (Ed.), 201
Isotopic fission-fragment distributions of U-238, Np-239, Pu-240, Cm-244, and Cf-250 produced through inelastic scattering, transfer, and fusion reactions in inverse kinematics
Transfer- and fusion-induced fission in inverse kinematics has proved to be a powerful tool to investigate nuclear fission, widening information on the fission fragments and access to unstable fissioning systems with respect to other experimental approaches. An experimental campaign is being carried out at GANIL with this technique since 2008. In these experiments, a beam of U-238, accelerated to 6.1 MeV/u, impinges on a C-12 target. Fissioning systems from U to Cf are populated through inelastic scattering, transfer, and fusion reactions, with excitation energies that range from a few MeV up to 46 MeV. The use of inverse kinematics, the SPIDER telescope, and the VAMOS spectrometer allow the characterization of the fissioning system in terms of mass, nuclear charge, and excitation energy, and the isotopic identification of the full fragment distribution. This work reports on new data from the second experiment of the campaign on fission-fragment yields of the heavy actinides U-238, Np-239, Pu-240, Cm-244, and Cf-250, which are of interest from both fundamental and application points of view
Evidence for a spin-aligned neutron-proton paired phase from the level structure of Pd
The general phenomenon of shell structure in atomic nuclei has been
understood since the pioneering work of Goeppert-Mayer, Haxel, Jensen and
Suess.They realized that the experimental evidence for nuclear magic numbers
could be explained by introducing a strong spin-orbit interaction in the
nuclear shell model potential. However, our detailed knowledge of nuclear
forces and the mechanisms governing the structure of nuclei, in particular far
from stability, is still incomplete. In nuclei with equal neutron and proton
numbers (), the unique nature of the atomic nucleus as an object
composed of two distinct types of fermions can be expressed as enhanced
correlations arising between neutrons and protons occupying orbitals with the
same quantum numbers. Such correlations have been predicted to favor a new type
of nuclear superfluidity; isoscalar neutron-proton pairing, in addition to
normal isovector pairing (see Fig. 1). Despite many experimental efforts these
predictions have not been confirmed. Here, we report on the first observation
of excited states in nucleus Pd. Gamma rays emitted
following the Ni(Ar,2)Pd fusion-evaporation reaction
were identified using a combination of state-of-the-art high-resolution
{\gamma}-ray, charged-particle and neutron detector systems. Our results reveal
evidence for a spin-aligned, isoscalar neutron-proton coupling scheme,
different from the previous prediction. We suggest that this coupling scheme
replaces normal superfluidity (characterized by seniority coupling) in the
ground and low-lying excited states of the heaviest N = Z nuclei. The strong
isoscalar neutron- proton correlations in these nuclei are predicted to
have a considerable impact on their level structures, and to influence the
dynamics of the stellar rapid proton capture nucleosynthesis process.Comment: 13 pages, 3 figure
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