Supercurrent Spectroscopy of Andreev States

We measure the excitation spectrum of a superconducting atomic contact. In addition to the usual continuum above the superconducting gap, the single particle excitation spectrum contains discrete, spin-degenerate Andreev levels inside the gap. Quasiparticle excitations are induced by a broadband on-chip microwave source and detected by measuring changes in the supercurrent flowing through the atomic contact. Since microwave photons excite quasiparticles in pairs, two types of transitions are observed: Andreev transitions, which consists of putting two quasiparticles in an Andreev level, and transitions to odd states with a single quasiparticle in an Andreev level and the other one in the continuum. In contrast to absorption spectroscopy, supercurrent spectroscopy allows detection of long-lived odd states.Comment: typos correcte

Exciting Andreev pairs in a superconducting atomic contact

The Josephson effect describes the flow of supercurrent in a weak link, such as a tunnel junction, nanowire, or molecule, between two superconductors. It is the basis for a variety of circuits and devices, with applications ranging from medicine to quantum information. Currently, experiments using Josephson circuits that behave like artificial atoms are revolutionizing the way we probe and exploit the laws of quantum physics. Microscopically, the supercurrent is carried by Andreev pair states, which are localized at the weak link. These states come in doublets and have energies inside the superconducting gap. Existing Josephson circuits are based on properties of just the ground state of each doublet and so far the excited states have not been directly detected. Here we establish their existence through spectroscopic measurements of superconducting atomic contacts. The spectra, which depend on the atomic configuration and on the phase difference between the superconductors, are in complete agreement with theory. Andreev doublets could be exploited to encode information in novel types of superconducting qubits.Comment: Submitted to Natur

Theory of microwave spectroscopy of Andreev bound states with a Josephson junction

We present a microscopic theory for the current through a tunnel Josephson junction coupled to a non-linear environment, which consists of an Andreev two-level system coupled to a harmonic oscillator. It models a recent experiment [Bretheau, Girit, Pothier, Esteve, and Urbina, Nature (London) 499, 312 (2013)] on photon spectroscopy of Andreev bound states in a superconducting atomic-size contact. We find the eigenenergies and eigenstates of the environment and derive the current through the junction due to inelastic Cooper pair tunneling. The current-voltage characteristic reveals the transitions between the Andreev bound states, the excitation of the harmonic mode that hybridizes with the Andreev bound states, as well as multi-photon processes. The calculated spectra are in fair agreement with the experimental data.Comment: 8 pages, 6 figure

Evidence for long-lived quasiparticles trapped in superconducting point contacts

We have observed that the supercurrent across phase-biased, highly transmitting atomic size contacts is strongly reduced within a broad phase interval around {\pi}. We attribute this effect to quasiparticle trapping in one of the discrete sub-gap Andreev bound states formed at the contact. Trapping occurs essentially when the Andreev energy is smaller than half the superconducting gap {\Delta}, a situation in which the lifetime of trapped quasiparticles is found to exceed 100 \mus. The origin of this sharp energy threshold is presently not understood.Comment: Article (5 pages) AND Supplemental material (14 pages). To be published in Physical Review Letter

Dynamics of quasiparticle trapping in Andreev levels

We present a theory describing the trapping and untrapping of quasiparticles in the Andreev bound level of a single-channel weak link between two superconductors. We calculate the rates of the transitions between even and odd occupations of the Andreev level induced by absorption and emission of both photons and phonons. We apply the theory to a recent experiment [Phys. Rev. Lett. 106, 257003 (2011)] in which the dynamics of the trapping of quasiparticles in the Andreev levels of superconducting atomic contacts coupled to a Josephson junction was measured. We show that the plasma energy $h\nu_p$ of the Josephson junction defines a rather abrupt transition between a fast relaxation regime dominated by coupling to photons and a slow relaxation regime dominated by coupling to phonons. With realistic parameters the theory provides a semi-quantitative description of the experimental results.Comment: 11 pages, 9 figures. Accepted for publication in Physical Review

Observing quantum state diffusion by heterodyne detection of fluorescence

A qubit can relax by fluorescence, which prompts the release of a photon into its electromagnetic environment. By counting the emitted photons, discrete quantum jumps of the qubit state can be observed. The succession of states occupied by the qubit in a single experiment, its quantum trajectory, depends in fact on the kind of detector. How are the quantum trajectories modified if one measures continuously the amplitude of the fluorescence field instead? Using a superconducting parametric amplifier, we have performed heterodyne detection of the fluorescence of a superconducting qubit. For each realization of the measurement record, we can reconstruct a different quantum trajectory for the qubit. The observed evolution obeys quantum state diffusion, which is characteristic of quantum measurements subject to zero point fluctuations. Independent projective measurements of the qubit at various times provide a quantitative validation of the reconstructed trajectories. By exploring the statistics of quantum trajectories, we demonstrate that the qubit states span a deterministic surface in the Bloch sphere at each time in the evolution. Additionally, we show that when monitoring fluorescence, coherent superpositions are generated during the decay from excited to ground state. Counterintuitively, measuring light emitted during relaxation can give rise to trajectories with increased excitation probability.Comment: Supplementary material can be found in the ancillary sectio

Using Spontaneous Emission of a Qubit as a Resource for Feedback Control

Persistent control of a transmon qubit is performed by a feedback protocol based on continuous heterodyne measurement of its fluorescence. By driving the qubit and cavity with microwave signals whose amplitudes depend linearly on the instantaneous values of the quadratures of the measured fluorescence field, we show that it is possible to stabilize permanently the qubit in any targeted state. Using a Josephson mixer as a phase-preserving amplifier, it was possible to reach a total measurement efficiency $\eta$=35%, leading to a maximum of 59% of excitation and 44% of coherence for the stabilized states. The experiment demonstrates multiple-input multiple-output analog Markovian feedback in the quantum regime.Comment: Supplementary material can be found as an ancillary objec

Coherent manipulation of Andreev states in superconducting atomic contacts

Coherent control of quantum states has been demonstrated in a variety of superconducting devices. In all these devices, the variables that are manipulated are collective electromagnetic degrees of freedom: charge, superconducting phase, or flux. Here, we demonstrate the coherent manipulation of a quantum system based on Andreev bound states, which are microscopic quasiparticle states inherent to superconducting weak links. Using a circuit quantum electrodynamics setup we perform single-shot readout of this "Andreev qubit". We determine its excited state lifetime and coherence time to be in the microsecond range. Quantum jumps and parity switchings are observed in continuous measurements. In addition to possible quantum information applications, such Andreev qubits are a testbed for the physics of single elementary excitations in superconductors.Comment: Supplementary Materials at the end of the fil

Superconducting Quantum Point Contacts

We review our experiments on the electronic transport properties of atomic contacts between metallic electrodes, in particular superconducting ones. Despite ignorance of the exact atomic configuration, these ultimate quantum point contacts can be manipulated and well characterized in-situ. They allow performing fundamental tests of the scattering theory of quantum transport. In particular, we discuss the case of the Josephson effect

Determining the Quantum Expectation Value by Measuring a Single Photon

Quantum mechanics, one of the keystones of modern physics, exhibits several peculiar properties, differentiating it from classical mechanics. One of the most intriguing is that variables might not have definite values. A complete quantum description provides only probabilities for obtaining various eigenvalues of a quantum variable. These and corresponding probabilities specify the expectation value of a physical observable, which is known to be a statistical property of an ensemble of quantum systems. In contrast to this paradigm, we demonstrate a unique method allowing to measure the expectation value of a physical variable on a single particle, namely, the polarisation of a single protected photon. This is the first realisation of quantum protective measurements.Comment: Nature Physics, in press (this version corresponds to the one initially submitted to Nature Physics