79 research outputs found
Isomer shift and magnetic moment of the long-lived 1/2 isomer in Zn: signature of shape coexistence near Ni
Collinear laser spectroscopy has been performed on the Zn
isotope at ISOLDE-CERN. The existence of a long-lived isomer with a few hundred
milliseconds half-life was confirmed, and the nuclear spins and moments of the
ground and isomeric states in Zn as well as the isomer shift were
measured. From the observed hyperfine structures, spins and
are firmly assigned to the ground and isomeric states. The magnetic moment
(Zn) = 1.1866(10) , confirms the spin-parity
with a shell-model configuration, in excellent
agreement with the prediction from large scale shell-model theories. The
magnetic moment (Zn) = 1.0180(12) supports a
positive parity for the isomer, with a wave function dominated by a 2h-1p
neutron excitation across the shell gap. The large isomer shift
reveals an increase of the intruder isomer mean square charge radius with
respect to that of the ground state:
= +0.204(6) fm, providing first evidence of shape coexistence.Comment: 5 pages, 4 figures, 1 table, Accepeted by Phys. Rev. Lett. (2016
The nuclear magnetic moment of ÂČâ°âžBi and its relevance for a test of bound-state strong-field QED
The hyperfine structure splitting in the 6p2 4S3/2 -> 6p27s 4P1/2 transition at 307 nm in atomic 208Bi was measured with collinear laser spectroscopy at ISOLDE, CERN. The hyperfine A and B factors of both states were determined with an order of magnitude improved accuracy. Based on these measurements, theoretical input for the hyperfine structure anomaly, and results from hyperfine measurements on hydrogen-like and lithium-like 209Bi80+,82+, the nuclear magnetic moment of 208Bi has been determined to ÎŒ(208Bi) =+4.570(10) ÎŒN . Using this value, the transition energy of the ground-state hyperfine splitting in hydrogen-like and lithium-like 208Bi80+,82+ and their specific difference of â67.491(5)(148) meV are predicted. This provides a means for an experimental confirmation of the cancellation of nuclear structure effects in the specific difference in order to exclude such contributions as the cause of the hyperfine puzzle, the recently reported 7-Ï discrepancy between experiment and bound-state strong-field QED calculations of the specific difference in the hyperfine structure splitting of 209Bi80+,82+
Evolution of nuclear structure in neutron-rich odd-Zn isotopes and isomers
Collinear laser spectroscopy was performed on Zn (Z=30) isotopes at ISOLDE, CERN. The study of hyperfine spectra of nuclei across the Zn isotopic chain, N=33â49, allowed the measurement of nuclear spins for the ground and isomeric states in odd-A neutron-rich nuclei up to N=50. Exactly one long-lived (>10 ms) isomeric state has been established in each 69â79Zn isotope. The nuclear magnetic dipole moments and spectroscopic quadrupole moments are well reproduced by large-scale shellâmodel calculations in the f5pg9 and fpg9d5 model spaces, thus establishing the dominant term in their wave function. The magnetic moment of the intruder IÏ=1/2+ isomer in 79Zn is reproduced only if the Îœs1/2 orbital is added to the valence space, as realized in the recently developed PFSDG-U interaction. The spin and moments of the low-lying isomeric state in 73Zn suggest a strong onset of deformation at N=43, while the progression towards 79Zn points to the stability of the Z=28 and N=50 shell gaps, supporting the magicity of 78Ni
Competing particleâhole excitations in Âłâ°Na: Constraining state-of-the-art effective interactions
The oddâodd nucleus Âłâ°Na is studied via a one-proton, one-protonâone-neutron and one-neutron removal reaction using an intermediate-energy ÂłÂčMg, ÂłÂČMg and ÂłÂčNa radioactive ion beam, respectively. Combining high-resolution Îł-ray spectroscopy with the selectivity of the three reaction mechanisms, we are able to distinguish multiple particleâhole configurations. Negative-parity states in Âłâ°Na are observed for the first time, providing an important measure of the excitation of the 1p1h/3p3h configuration and hence the sdâpf shell gap. The extracted band structures and level energies serve as invaluable input for the theoretical refinement of the effective interactions used in this region
Laser Spectroscopy of Neutron-Rich Tin Isotopes: A Discontinuity in Charge Radii across the N=82 Shell Closure
The change in mean-square nuclear charge radii ÎŽâšr2â© along the even-A tin isotopic chain 108â134Sn has been investigated by means of collinear laser spectroscopy at ISOLDE/CERN using the atomic transitions 5p2â1S0â5p6âs1P1 and 5p2â3P0â5p6sâ3P1. With the determination of the charge radius of 134Sn and corrected values for some of the neutron-rich isotopes, the evolution of the charge radii across the N=82 shell closure is established. A clear kink at the doubly magic 132Sn is revealed, similar to what has been observed at N=82 in other isotopic chains with larger proton numbers, and at the N=126 shell closure in doubly magic 208Pb. While most standard nuclear density functional calculations struggle with a consistent explanation of these discontinuities, we demonstrate that a recently developed Fayans energy density functional provides a coherent description of the kinks at both doubly magic nuclei, 132Sn and 208Pb, without sacrificing the overall performance. A multiple correlation analysis leads to the conclusion that both kinks are related to pairing and surface effects
Nuclear charge radius of Al and its implication for V in the quark-mixing matrix
Collinear laser spectroscopy was performed on the isomer of the aluminium
isotope Al. The measured isotope shift to Al in the
3s^{2}3p\;^{2}\!P^\circ_{3/2} \rightarrow 3s^{2}4s\;^{2}\!S_{1/2} atomic
transition enabled the first experimental determination of the nuclear charge
radius of Al, resulting in =\qty{3.130\pm.015}{\femto\meter}. This
differs by 4.5 standard deviations from the extrapolated value used to
calculate the isospin-symmetry breaking corrections in the superallowed
decay of Al. Its corrected value, important for the
estimation of in the CKM matrix, is thus shifted by one standard
deviation to \qty{3071.4\pm1.0}{\second}.Comment: 5 pages, 2 figures, submitted to Phys. Rev. Let
Structural trends in atomic nuclei from laser spectroscopy of tin
Tin is the chemical element with the largest number of stable isotopes. Its complete proton shell, comparable with the closed electron shells in the chemically inert noble gases, is not a mere precursor to extended stability; since the protons carry the nuclear charge, their spatial arrangement also drives the nuclear electromagnetism. We report high-precision measurements of the electromagnetic moments and isomeric differences in charge radii between the lowest 1/2(+), 3/2(+), and 11/2(-) states in Sn117-131, obtained by collinear laser spectroscopy. Supported by state-of-the-art atomic-structure calculations, the data accurately show a considerable attenuation of the quadrupole moments in the closed-shell tin isotopes relative to those of cadmium, with two protons less. Linear and quadratic mass-dependent trends are observed. While microscopic density functional theory explains the global behaviour of the measured quantities, interpretation of the local patterns demands higher-fidelity modelling. Measurements of the hyperfine structure of chemical elements isotopes provide unique insight into the atomic nucleus in a nuclear model-independent way. The authors present collinear laser spectroscopy data obtained at the CERN ISOLDE and measure hyperfine splitting along a long chain of odd-mass tin isotopes.Peer reviewe
Quadrupole moments of odd-A â”Âłâ»â¶ÂłMn: Onset of collectivity towards N = 40
The spectroscopic quadrupole moments of the oddâeven Mn isotopes between N=28 and N=38 have been measured using bunched-beam collinear laser spectroscopy at ISOLDE, CERN. In order to increase sensitivity to the quadrupole interaction, the measurements have been done using a transition in the ion rather than in the atom, with the additional advantage of better spectroscopic efficiency. Since the chosen transition is from a metastable state, optical pumping in ISOLDEâs cooler and buncher (ISCOOL) was used to populate this state. The extracted quadrupole moments are compared to large-scale shell model predictions using three effective interactions, GXPF1A, LNPS and modified A3DA. The inclusion of both the 1Îœg9/2and 2Îœd5/2orbitals in the model space is shown to be necessary to reproduce the observed increase in the quadrupole deformation from N=36 onwards. Specifically, the inclusion of the 2Îœd5/2orbital induces an increase in neutron and proton excitations across the reduced gaps at N=40and Z=28, leading to an increase in deformation above N=36
Nuclear charge radii of â¶ÂČâ»âžâ°Zn and their dependence on cross-shell proton excitations
Nuclear charge radii of â¶ÂČâ»âžâ°Zn have been determined using collinear laser spectroscopy of bunched ion beams at CERN-ISOLDE. The subtle variations of observed charge radii, both within one isotope and along the full range of neutron numbers, are found to be well described in terms of the proton
excitations across the Z = 28 shell gap, as predicted by large-scale shell model calculations. It comprehensively explains the changes in isomer-to-ground state mean square charge radii of â¶âčâ»â·âčZn, the inversion of the
odd-even staggering around N = 40 and the odd-even staggering systematics of the Zn charge radii. With two protons above Z = 28, the observed charge radii of the Zn isotopic chain show a cumulative effect of different aspects of nuclear structure including single particle structure, shell closure, correlations and deformations near the proposed doubly magic nuclei, â¶âžNi and â·âžNi
Changes in nuclear structure along the Mn isotopic chain studied via charge radii.
The hyperfine spectra of Mn-51,Mn-53-64 were measured in two experimental runs using collinear laser spectroscopy at ISOLDE, CERN. Laser spectroscopy was performed on the atomic 3d(5) 4s(2) S-6(5/2) -> 3d(5) 4s4p P-6(3/2) and ionic 3d(5) 4s S-5(2) -> 3d(5) 4p P-5(3) transitions, yielding two sets of isotope shifts. The mass and field shift factors for both transitions have been calculated in the multiconfiguration Dirac-Fock framework and were combined with a King plot analysis in order to obtain a consistent set of mean-square charge radii which, together with earlier work on neutron-deficient Mn, allow the study of nuclear structure changes from N = 25 across N = 28 up to N = 39. A clear development of deformation is observed towards N = 40, confirming the conclusions of the nuclear moments studies. From a Monte Carlo shell-model study of the shape in the Mn isotopic chain, it is suggested that the observed development of deformation is not only due to an increase in static prolate deformation but also due to shape fluctuations and triaxiality. The changes in mean-square charge radii are well reproduced using the Duflo-Zuker formula except in the case of large deformation
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