Caloric Expenditure of Normal and Lower Body Positive Pressure Treadmill Running

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Perceived Exertion and Affective Responses During Normal and Lower Body Positive Pressure Treadmill Running

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Conditions for Adiabatic Spin Transport in Disordered Systems

We address the controversy concerning the necessary conditions for the observation of Berry phases in disordered mesoscopic conductors. For this purpose we calculate the spin-dependent conductance of disordered two-dimensional structures in the presence of inhomogeneous magnetic fields. Our numerical results show that for both, the overall conductance and quantum corrections, the relevant parameter defining adiabatic spin transport scales with the square root of the number of scattering events, in generalization of Stern's original proposal [Phys. Rev. Lett. 68, 1022 (1992)]. This could hinder a clear-cut experimental observation of Berry phase effects in diffusive metallic rings.Comment: 5 pages, 4 figures. To appear in Phys. Rev. B (Rapid Communications

Berry phase and adiabaticity of a spin diffusing in a non-uniform magnetic field

An electron spin moving adiabatically in a strong, spatially non-uniform magnetic field accumulates a geometric phase or Berry phase, which might be observable as a conductance oscillation in a mesoscopic ring. Two contradicting theories exist for how strong the magnetic field should be to ensure adiabaticity if the motion is diffusive. To resolve this controversy, we study the effect of a non-uniform magnetic field on the spin polarization and on the weak-localization effect. The diffusion equation for the Cooperon is solved exactly. Adiabaticity requires that the spin-precession time is short compared to the elastic scattering time - it is not sufficient that it is short compared to the diffusion time around the ring. This strong condition severely complicates the experimental observation.Comment: 16 pages REVTEX, including 3 figure

Berry phase and persistent current in disordered mesoscopic rings

A novel quantum interference effect in disordered quasi-one-dimensional rings in the inhomogeneous magnetic field is reported. We calculate the canonical disorder averaged persistent current using the diagrammatic perturbation theory. It is shown that within the adiabatic regime the average current oscillates as a function of the geometric flux which is related to the Berry phase and the period becomes half the value of the case of a single one-dimensional ring. We also discuss the magnetic dephasing effect on the averaged current.Comment: 6 pages, RevTeX, 2 figures. To appear in Phys. Rev. B Rapid Communications Vol.60 No.12 (1999

Conductance fluctuations in diffusive rings: Berry phase effects and criteria for adiabaticity

We study Berry phase effects on conductance properties of diffusive mesoscopic conductors, which are caused by an electron spin moving through an orientationally inhomogeneous magnetic field. Extending previous work, we start with an exact, i.e. not assuming adiabaticity, calculation of the universal conductance fluctuations in a diffusive ring within the weak localization regime, based on a differential equation which we derive for the diffuson in the presence of Zeeman coupling to a magnetic field texture. We calculate the field strength required for adiabaticity and show that this strength is reduced by the diffusive motion. We demonstrate that not only the phases but also the amplitudes of the h/2e Aharonov-Bohm oscillations are strongly affected by the Berry phase. In particular, we show that these amplitudes are completely suppressed at certain magic tilt angles of the external fields, and thereby provide a useful criterion for experimental searches. We also discuss Berry phase-like effects resulting from spin-orbit interaction in diffusive conductors and derive exact formulas for both magnetoconductance and conductance fluctuations. We discuss the power spectra of the magnetoconductance and the conductance fluctuations for inhomogeneous magnetic fields and for spin-orbit interaction.Comment: 18 pages, 13 figures; minor revisions. To appear in Phys. Rev.

Intensity distribution for waves in disordered media: deviations from Rayleigh statistics

We study the intensity distribution function, P(I), for monochromatic waves propagating in quasi one-dimensional disordered medium, assuming that a point source and a point detector are embedded in the bulk of the medium. We find deviations from the Rayleigh statistics at moderately large I and a logarithmically-normal asymptotic behavior of P(I). When the radiation source and the detector are located close to the opposite edges of the sample (on a distance much less then the sample length), an intermediate regime with a stretched-exponential behavior of P(I) emerges.Comment: 4 pages Revtex, 3 figures included as eps file

Aharonov-Bohm Physics with Spin II: Spin-Flip Effects in Two-dimensional Ballistic Systems

We study spin effects in the magneto-conductance of ballistic mesoscopic systems subject to inhomogeneous magnetic fields. We present a numerical approach to the spin-dependent Landauer conductance which generalizes recursive Green function techniques to the case with spin. Based on this method we address spin-flip effects in quantum transport of spin-polarized and -unpolarized electrons through quantum wires and various two-dimensional Aharonov-Bohm geometries. In particular, we investigate the range of validity of a spin switch mechanism recently found which allows for controlling spins indirectly via Aharonov-Bohm fluxes. Our numerical results are compared to a transfer-matrix model for one-dimensional ring structures presented in the first paper (Hentschel et al., submitted to Phys. Rev. B) of this series.Comment: 29 pages, 15 figures. Second part of a series of two article

Multi-Catalytic Route for the Synthesis of (S)-Tembamide

Enantiopure β-amino alcohols constitute one of the most significant building blocks for the synthesis of active pharmaceutical ingredients. Despite the availability of a range of chiral β-amino alcohols from a chiral pool, there is a growing demand for new enantioselective synthetic routes to vicinal amino alcohols and their derivatives. In the present study, an asymmetric 2-step catalytic route that converts 4-anisaldehyde into a β-amino alcohol derivative, (S)-tembamide, with excellent enantiopurity (98% enantiomeric excess) has been developed. The recently published initial step consists in a concurrent biocatalytic cascade for the synthesis of (S)-4-methoxymandelonitrile benzoate. The O-benzoyl cyanohydrin is then converted to (S)-tembamide in a hydrogenation reaction catalyzed by Raney Ni. To achieve hydrogenation of the nitrile moiety with highest chemoselectivity and enantioretention, various parameters such as nature of the catalyst, reaction temperature and hydrogen pressure were studied. The reported strategy might be transferrable to the synthesis of other N-acyl-β-amino alcohols

Effect of incoherent scattering on shot noise correlations in the quantum Hall regime

We investigate the effect of incoherent scattering in a Hanbury Brown and Twiss situation with electrons in edge states of a three-terminal conductor submitted to a strong perpendicular magnetic field. The modelization of incoherent scattering is performed by introducing an additional voltage probe through which the current is kept equal to zero which causes voltage fluctuations at this probe. It is shown that inelastic scattering can lead in this framework to positive correlations, whereas correlations remain always negative for quasi-elastic scattering.Comment: 5 pages latex, 5 eps figure