Observables of interest for the characterisation of Spent Nuclear Fuel

The characterisation of Spent Nuclear Fuel (SNF) in view of intermediate storage and final disposal is discussed. The main observables of interest that need to be determined are the decay heat, neutron and -ray emission spectra. In addition, the inventory of specific nuclides that are important for criticality safety analysis and to verify the fuel history has to be determined. Some of the observables such as the decay heat and neutron and -ray emission rate can be determined by Non-Destructive Analysis (NDA) methods. Unfortunately, this is not always possible especially during routine operation. Hence, a characterisation of SNF will rely on theoretical calculations combined with results of NDA methods. In this work the observables of interest, also referred to as source terms, are discussed based on theoretical calculations starting from fresh UO2 and MOX fuel. The irradiation conditions are representative for PWR. The Serpent code is used to define the nuclides which have an important contribution to the observables. The emphasis is on cooling times between 1 a and 1000 a.JRC.G.2-Standards for Nuclear Safety, Security and Safeguard

An absolute measurement of the neutron production rate of a spent nuclear fuel sample used for depletion code validation

A method to determine the neutron production rate of a spent nuclear fuel segment sample by means of non-destructive assay conducted under standard controlled-area conditions is described and demonstrated. A neutron well counter designed for routine nuclear safeguards applications is applied. The method relies on a transfer procedure that is adapted to the hot cell facilities at the Laboratory for High and Medium level Activity of SCK CEN in Belgium. Experiments with 252Cf(sf) sources, certified for their neutron emission rate, were carried out at the Joint Research Centre to determine the characteristics of the detection device. Measurements of a segment of a spent nuclear fuel rod were carried out at SCK CEN resulting in an absolute and non-destructive measurement of the neutron production rate avoiding any reference to a representative spent nuclear fuel sample to calibrate the device. Results of these measurements were used to study the performance of depletion codes, i.e., ALEPH2, SCALE, and Serpent2. The study includes a code-to-code and code-to-experiment comparison using different nuclear data libraries

The joint evaluated fission and fusion nuclear data library, JEFF-3.3

The joint evaluated fission and fusion nuclear data library 3.3 is described. New evaluations for neutron-induced interactions with the major actinides $^{235}$U, $^{238}$U and $^{239}$Pu, on $^{241}$Am and $^{23}$Na, $^{59}$Ni, Cr, Cu, Zr, Cd, Hf, W, Au, Pb and Bi are presented. It includes new fission yields, prompt fission neutron spectra and average number of neutrons per fission. In addition, new data for radioactive decay, thermal neutron scattering, gamma-ray emission, neutron activation, delayed neutrons and displacement damage are presented. JEFF-3.3 was complemented by files from the TENDL project. The libraries for photon, proton, deuteron, triton, helion and alpha-particle induced reactions are from TENDL-2017. The demands for uncertainty quantification in modeling led to many new covariance data for the evaluations. A comparison between results from model calculations using the JEFF-3.3 library and those from benchmark experiments for criticality, delayed neutron yields, shielding and decay heat, reveals that JEFF-3.3 performes very well for a wide range of nuclear technology applications, in particular nuclear energy

Benchmarking and validation activities within JEFF project

The challenge for any nuclear data evaluation project is to periodically release a revised, fully consistent and complete library, with all needed data and covariances, and ensure that it is robust and reliable for a variety of applications. Within an evaluation effort, benchmarking activities play an important role in validating proposed libraries. The Joint Evaluated Fission and Fusion (JEFF) Project aims to provide such a nuclear data library, and thus, requires a coherent and efficient benchmarking process. The aim of this paper is to present the activities carried out by the new JEFF Benchmarking and Validation Working Group, and to describe the role of the NEA Data Bank in this context. The paper will also review the status of preliminary benchmarking for the next JEFF-3.3 candidate cross-section files

Advanced Method for Calculations of Core Burn-Up, Activation of Structural Materials, and Spallation Products Accumulation in Accelerator-Driven Systems

The ALEPH2 Monte Carlo depletion code has two principal features that make it a flexible and powerful tool for reactor analysis. First of all, it uses a nuclear data library covering neutron- and proton-induced reactions, neutron and proton fission product yields, spontaneous fission product yields, radioactive decay data, and total recoverable energies per fission. Secondly, it uses a state-of-the-art numerical solver for the first-order ordinary differential equations describing the isotope balances, namely, a Radau IIA implicit Runge-Kutta method. The versatility of the code allows using it for time behavior simulation of various systems ranging from single pin model to full-scale reactor model, including such specific facilities as accelerator-driven systems. The core burn-up, activation of the structural materials, irradiation of samples, and, in addition, accumulation of spallation products in accelerator-driven systems can be calculated in a single ALEPH2 run. The code is extensively used for the neutronics design of the MYRRHA research facility which will operate in both critical and subcritical modes