Empirical description of beta-delayed fission partial half-lives

Background: The process of beta-delayed fission (bDF) provides a versatile tool to study low-energy fission in nuclei far away from the beta-stability line, especially for nuclei which do not fission spontaneously. Purpose: The aim of this paper is to investigate systematic trends in bDF partial half-lives. Method: A semi-phenomenological framework was developed to systematically account for the behavior of bDF partial half-lives. Results: The bDF partial half-life appears to exponentially depend on the difference between the Q value for beta decay of the parent nucleus and the fission-barrier energy of the daughter (after beta decay) product. Such dependence was found to arise naturally from some simple theoretical considerations. Conclusions: This systematic trend was confirmed for experimental bDF partial half-lives spanning over 7 orders of magnitudes when using fission barriers calculated from either the Thomas-Fermi or the liquid-drop fission model. The same dependence was also observed, although less pronounced, when comparing to fission barriers from the finite-range liquid-drop model or the Thomas-Fermi plus Strutinsky Integral method.Comment: accepted for publication in Phys. Rev.

In-source laser spectroscopy with the laser ion source and trap: first direct study of the ground-state properties of Po-217,Po-219

D. A. Fink et al.; 15 págs.; 17 figs.; 3 tabs.; Open Access funded by Creative Commons Atribution Licence 3.0A Laser Ion Source and Trap (LIST) for a thick-target, isotope-separation on-line facility has been implemented at CERN ISOLDE for the production of pure, laser-ionized, radioactive ion beams. It offers two modes of operation, either as an ion guide, which performs similarly to the standard ISOLDE resonance ionization laser ion source (RILIS), or as a more selective ion source, where surface-ionized ions from the hot ion-source cavity are repelled by an electrode, while laser ionization is done within a radiofrequency quadrupole ion guide. The first physics application of the LIST enables the suppression of francium contamination in ion beams of neutron-rich polonium isotopes at ISOLDE by more than 1000 with a reduction in laser-ionization efficiency of only 20. Resonance ionization spectroscopy is performed directly inside the LIST device, allowing the study of the hyperfine structure and isotope shift of 217Po for the first time. Nuclear decay spectroscopy of 219Po is performed for the first time, revealing its half-life, α- to-β-decay branching ratio, and α-particle energy. This experiment demonstrates the applicability of the LIST at radioactive ion-beam facilities for the production and study of pure beams of exotic isotopes. Published by the American Physical SocietyThis work was supported by the Bundesministerium für Bildung und Forschung (BMBF, Germany) within the Wolfgang- Gentner programme as well as through the consecutive project fundings of 06Mz9181I, 06Mz7177D, and 05P12UMCIA, by FWO-Vlaanderen (Belgium), by GOA/2010/010 (BOF-KULeuven), by the IUAP-Belgian State Belgian Science Policy (BRIX network P7/12), by the U.K. Science and Technology Facilities Council (STFC), by the European Union within FP7 (ENSAR No. 262010), by the Slovak Research and Development Agency (Contract No. APVV-0105-10), by the Slovak grant agency VEGA, and the Reimei Foundation of JAEA (Contract No. 1/0576/13). T. E. C. was supported by STFC Ernest Rutherford Grant No. ST/J004189/1.Peer Reviewe

Early onset of ground-state deformation in the neutron-deficient polonium isotopes

In-source resonant ionization laser spectroscopy of the even-$A$ polonium isotopes $^{192-210,216,218}$Po has been performed using the $6p^37s$ $^5S_2$ to $6p^37p$ $^5P_2$ ($\lambda=843.38$ nm) transition in the polonium atom (Po-I) at the CERN ISOLDE facility. The comparison of the measured isotope shifts in $^{200-210}$Po with a previous data set allows to test for the first time recent large-scale atomic calculations that are essential to extract the changes in the mean-square charge radius of the atomic nucleus. When going to lighter masses, a surprisingly large and early departure from sphericity is observed, which is only partly reproduced by Beyond Mean Field calculations.Comment: As submitted to PR

Alpha decay of 176Au

International audienceThe isotope Au176 has been studied in the complete fusion reaction Ca40+Pr141 → 176Au+5n at the velocity filter SHIP (GSI, Darmstadt). The complex fine-structure α decay of two isomeric states in Au176 feeding several previously unknown excited states in the daughter nucleus Ir172 is presented. An α-decay branching ratio of bα=9.5(11)% was deduced for the high-spin isomer in Ir172

Short-lived isomers in Po-192 and Po-194

Isomeric states in Po194 and Po192 were studied at the velocity filter SHIP. The isotopes were produced in the fusion-evaporation reactions Pr141(Fe56, p2n)Po194 and Sm144(V51, p2n)Po192. Several new γ-ray transitions were attributed to the isomers and γ−γ coincidences for both isomers were studied for the first time. The 459-keV transition earlier, tentatively proposed as de-exciting the isomeric level in Po194, was replaced by a new 248-keV transition, and the spin of this isomer was reassigned from (11−) to (10−). The de-excitation of the (11−) isomeric level in Po192 by the 154-keV transition was confirmed and a parallel de-excitation by a 733-keV (E3) transition to (8+) level of the ground-state band was suggested. Moreover, side feeding to the (4+) level of the ground-state band was proposed. The paper also discusses strengths of transitions de-exciting 11− isomers in neighboring Po and Pb isotopes