Abstract

In-source resonant ionization laser spectroscopy of the even-AA polonium isotopes 192210,216,218^{192-210,216,218}Po has been performed using the 6p37s6p^37s 5S2^5S_2 to 6p37p6p^37p 5P2^5P_2 (λ=843.38\lambda=843.38 nm) transition in the polonium atom (Po-I) at the CERN ISOLDE facility. The comparison of the measured isotope shifts in 200210^{200-210}Po with a previous data set allows to test for the first time recent large-scale atomic calculations that are essential to extract the changes in the mean-square charge radius of the atomic nucleus. When going to lighter masses, a surprisingly large and early departure from sphericity is observed, which is only partly reproduced by Beyond Mean Field calculations.Comment: As submitted to PR

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