In-source resonant ionization laser spectroscopy of the even-A polonium
isotopes 192−210,216,218Po has been performed using the 6p37s5S2
to 6p37p5P2 (λ=843.38 nm) transition in the polonium atom
(Po-I) at the CERN ISOLDE facility. The comparison of the measured isotope
shifts in 200−210Po with a previous data set allows to test for the first
time recent large-scale atomic calculations that are essential to extract the
changes in the mean-square charge radius of the atomic nucleus. When going to
lighter masses, a surprisingly large and early departure from sphericity is
observed, which is only partly reproduced by Beyond Mean Field calculations.Comment: As submitted to PR