Preparation of magnetic ferrofluids in alternative carrier liquids

Ferrofluids are made by grinding magnetic particles together with a polar surfactant and a nonpolar solvent. The surfactant is adsorbed on the particle surfaces and acts as a coupling agent between the particles and the solvent

Nonlinear Dynamics of a Single Ferrofluid-Peak in an Oscillating Magnetic Field

If a magnetic field normal to the surface of a magnetic fluid is increased beyond a critical value a spontaneous deformation of the surface arises (normal field instability). The instability is subcritical and leads to peaks of a characteristic shape. We investigate the neighborhood of this instability experimentally under the influence of a temporal modulation of the magnetic field. We use a small vessel, where only one peak arises. The modulation can either be stabilizing or destabilizing, depending on the frequency and amplitude. We observe a cascade of odd-numbered response-periods up to period 11, and also a domain of even-numbered periods. We propose a minimal model involving a cutoff-condition which captures the essence of the experimental observations. PACS: 47.20.-k, 47.20.Ky, 75.50.Mm Keywords: magnetic fluid; nonlinear oscillator; subharmonic response; surface instability;Comment: 13 pages, 12 Postscript figures, LaTeX, uses elsart.sty, to be published in Physica

Hysteresis in a magnetic bead and its applications

We study hysteresis in a micron-sized bead: a non-magnetic matrix embedded with super- paramagnetic nanoparticles. These hold tremendous promise in therapeutic applications as heat generating machines. The theoretical formulation uses a mean-field theory to account for dipolar interactions between the supermoments. The study enables manipulation of heat dissipation by a compatible selection of commercially available beads and the frequency f and amplitude ho of the applied oscillating field in the labortory. We also introduce the possibility of utilizing return point memory for gradual heating of a local region.Comment: 8 pages, 4 figure

Solitary waves on a ferrofluid jet

The propagation of axisymmetric solitary waves on the surface of an otherwise cylindrical ferrofluid jet subjected to a magnetic field is investigated. An azimuthal magnetic field is generated by an electric current flowing along a stationary metal rod which is mounted along the axis of the moving jet. A numerical method is used to compute fully-nonlinear travelling solitary waves and predictions of elevation waves and depression waves by Rannacher & Engel (2006) using a weakly-nonlinear theory are confirmed in the appropriate ranges of the magnetic Bond number. New nonlinear branches of solitary wave solutions are identified. As the Bond number is varied, the solitary wave profiles may approach a limiting configuration with a trapped toroidal-shaped bubble, or they may approach a static wave (i.e. one with zero phase speed). For a sufficiently large axial rod, the limiting profile may exhibit a cusp

Fluid pumped by magnetic stress

A magnetic field rotating on the free surface of a ferrofluid layer is shown to induce considerable fluid motion toward the direction the field is rolling. The measured flow velocity i) increases with the square of the magnetic field amplitude, ii) is proportional to the thickness of the fluid layer, and iii) has a maximum at a driving frequency of about 3 kHz. The pumping speed can be estimated with a two-dimensional flow model.Comment: 3 pages, 4 figure

A Mesoscopic Approach to the ``Negative'' Viscosity Effect in Ferrofluids

We present a mesoscopic approach to analyze the dynamics of a single magnetic dipole under the influence of an oscillating magnetic field, based on the formulation of a Fokker-Planck equation. The dissipated power and the viscosity of a suspension of such magnetic dipoles are calculated from non-equilibrium thermodynamics of magnetized systems. By means of this method we have found a non-monotonous behaviour of the viscosity as a function of the frequency of the field which has been referred to as the ``negative'' viscosity effect. Moreover, we have shown that the viscosity depends on the vorticity field thus exhibiting non-Newtonian behaviour. Our analysis is complemented with numerical simulations which reproduce the behaviour of the viscosity we have found and extend the scope of our analytical approach to higher values of the magnetic field.Comment: 9 pages, 2 eps figures, simulations have been adde

New nonlinear dielectric materials: Linear electrorheological fluids under the influence of electrostriction

The usual approach to the development of new nonlinear dielectric materials focuses on the search for materials in which the components possess an inherently large nonlinear dielectric response. In contrast, based on thermodynamics, we have presented a first-principles approach to obtain the electrostriction-induced effective third-order nonlinear susceptibility for the electrorheological (ER) fluids in which the components have inherent linear, rather than nonlinear, responses. In detail, this kind of nonlinear susceptibility is in general of about the same order of magnitude as the compressibility of the linear ER fluid at constant pressure. Moreover, our approach has been demonstrated in excellent agreement with a different statistical method. Thus, such linear ER fluids can serve as a new nonlinear dielectric material.Comment: 11 page

The Surface Topography of a Magnetic Fluid -- a Quantitative Comparison between Experiment and Numerical Simulation

The normal field instability in magnetic liquids is investigated experimentally by means of a radioscopic technique which allows a precise measurement of the surface topography. The dependence of the topography on the magnetic field is compared to results obtained by numerical simulations via the finite element method. Quantitative agreement has been found for the critical field of the instability, the scaling of the pattern amplitude and the detailed shape of the magnetic spikes. The fundamental Fourier mode approximates the shape to within 10% accuracy for a range of up to 40% of the bifurcation parameter of this subcritical bifurcation. The measured control parameter dependence of the wavenumber differs qualitatively from analytical predictions obtained by minimization of the free energy.Comment: 21 pages, 16 figures; corrected typos, added reference to Kuznetsov and Spector(1976), S.J. Fortune(1995) and Harkins&Jordan (1930). Figures revise

Role of interactions in ferrofluid thermal ratchets

Orientational fluctuations of colloidal particles with magnetic moments may be rectified with the help of external magnetic fields with suitably chosen time dependence. As a result a noise-driven rotation of particles occurs giving rise to a macroscopic torque per volume of the carrier liquid. We investigate the influence of mutual interactions between the particles on this ratchet effect by studying a model system with mean-field interactions. The stochastic dynamics may be described by a nonlinear Fokker-Planck equation for the collective orientation of the particles which we solve approximately by using the effective field method. We determine an interval for the ratio between coupling strength and noise intensity for which a self-sustained rectification of fluctuations becomes possible. The ratchet effect then operates under conditions for which it were impossible in the absence of interactions.Comment: 18 pages, 10 figure

Magnetic traveling-stripe-forcing: enhanced transport in the advent of the Rosensweig instability

A new kind of contactless pumping mechanism is realized in a layer of ferrofluid via a spatio-temporally modulated magnetic field. The resulting pressure gradient leads to a liquid ramp, which is measured by means of X-rays. The transport mechanism works best if a resonance of the surface waves with the driving is achieved. The behavior can be understood semi-quantitatively by considering the magnetically influenced dispersion relation of the fluid.Comment: 6 Pages, 8 Figure