44 research outputs found

    Aerosol climatology: on the discrimination of aerosol types over four AERONET sites

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    International audienceAerosols have a significant regional and global effect on climate, which is about equal in magnitude but opposite in sign to that of greenhouse gases. Nevertheless, the aerosol climatic effect changes strongly with space and time because of the large variability of aerosol physical and optical properties, which is due to the variety of their sources, which are natural, and anthropogenic, and their dependence on the prevailing meteorological and atmospheric conditions. Characterization of aerosol properties is of major importance for the assessment of their role for climate. In the present study, 3-year AErosol RObotic NETwork (AERONET) data from ground-based sunphotometer measurements are used to establish climatologies of aerosol optical depth (AOD) and Ångström exponent ? in several key locations of the world, characteristic of different atmospheric environments. Using daily mean values of AOD at 500 nm (AOD500) and Ångström exponent at the pair of wavelengths 440 and 870 nm (? 440?870), a discrimination of the different aerosol types occurring in each location is achieved. For this discrimination, appropriate thresholds for AOD500 and ? 440?870 are applied. The discrimination of aerosol types in each location is made on an annual and seasonal basis. It is shown that a single aerosol type in a given location can exist only under specific conditions (e.g. intense forest fires or dust outbreaks), while the presence of well-mixed aerosols is the accustomed situation. Background clean aerosol conditions (AOD500<0.06) are mostly found over remote oceanic surfaces occurring on average in ~56.7% of total cases, while this situation is quite rare over land (occurrence of 3.8?13.7%). Our analysis indicates that these percentages change significantly from season to season. The spectral dependence of AOD exhibits large differences between the examined locations, while it exhibits a strong annual cycle

    Variability and Trends of Aerosol Properties over Kanpur, Northern India using AERONET Data (2001-10)

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    Natural and anthropogenic aerosols over northern India play an important role in influencing the regional radiation budget, causing climate implications to the overall hydrological cycle of South Asia. In the context of regional climate change and air quality, we discuss aerosol loading variability and trends at Kanpur AERONET station located in the central part of the Indo-Gangetic plains (IGP), during the last decade (2001-10). Ground-based radiometric measurements show an overall increase in column-integrated aerosol optical depth (AOD) on a yearly basis. This upward trend is mainly due to a sustained increase in the seasonal/monthly averaged AOD during the winter (Dec-Feb) and post-monsoon (Oct-Nov) seasons (dominated by anthropogenic emissions). In contrast, a neutral to weak declining trend is observed during late pre-monsoon (Mar-May) and monsoon (Jun-Sep) months, mainly influenced by inter-annual variations of dust outbreaks. A general decrease in coarse-mode aerosols associated with variable dust activity is observed, whereas the statistically significant increasing post-monsoon/winter AOD is reflected in a shift of the columnar size distribution towards relatively larger particles in the accumulation mode. Overall, the present study provides an insight into the pronounced seasonal behavior in aerosol loading trends and, in general, is in agreement with that associating the findings with those recently reported by satellite observations (MODIS and MISR) over northern India. Our results further suggest that anthropogenic emissions (due mainly to fossil-fuel and biomass combustion) over the IGP have continued to increase in the last decade

    Heterogeneity in pre-monsoon aerosol types over the Arabian Sea deduced from ship-borne measurements of spectral AODs

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    Ship-borne sunphotometer measurements obtained in the Arabian Sea (AS) in the pre-monsoon season (18 April–10 May 2006) during a cruise campaign (ICARB) have been used to retrieve the Aerosol Optical Depth (AOD; &amp;tau;) and the Ångström wavelength exponent (α). The continents surrounding the AS produce natural and anthropogenic aerosols that have distinctive influences on α and its spectral distribution. The α values were estimated by means of the least-squares method over the spectral bands 340–1020 nm and 340–870 nm. The spectral distribution of AOD in logarithmic co-ordinates could be fit using a 2nd order polynomial with higher accuracy in the wavelength band 340–1020 nm than in the 340–870 nm band. A polynomial fit analytically parameterizes the observed wavelength dependencies of AOD with least errors in spectral variation of α and yields accurate estimates of the coefficients (&lt;i&gt;a&lt;/i&gt;&lt;sub&gt;1&lt;/sub&gt; and &lt;i&gt;a&lt;/i&gt;&lt;sub&gt;2&lt;/sub&gt;). The coarse-mode (positive curvature in the ln&amp;tau;&lt;sub&gt;&amp;lambda;&lt;/sub&gt; vs. ln&amp;lambda;) aerosols are mainly depicted in the Northern part of the AS closely associated with the nearby arid areas while fine-mode aerosols are mainly observed over the far and coastal AS regions. In the study period the mean AOD at 500 nm is 0.25&amp;plusmn;0.11 and the α&lt;sub&gt;340-1020&lt;/sub&gt; is 0.90&amp;plusmn;0.19. The α&lt;sub&gt;340-870&lt;/sub&gt; exhibits similar values (0.92&amp;plusmn;0.18), while significant differences revealed for the constant terms of the polynomial fit (&lt;i&gt;a&lt;/i&gt;&lt;sub&gt;1&lt;/sub&gt; and &lt;i&gt;a&lt;/i&gt;&lt;sub&gt;2&lt;/sub&gt;) proportionally to the wavelength band used for their determination. Observed day-to-day variability in the aerosol load and optical properties are direct consequence of the local winds and air-mass trajectories along with the position of the ship

    Identification of the Aerosol Types over Athens, Greece: The Influence of Air-Mass Transport

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    Aerosol optical depth at 550 nm (AOD550) and fine-mode (FM) fraction data from Terra-MODIS were obtained over the Greater Athens Area covering the period February 2000–December 2005. Based on both AOD550 and FM values three main aerosol types have been discriminated corresponding to urban/industrial aerosols, clean maritime conditions, and coarse-mode, probably desert dust, particles. Five main sectors were identified for the classification of the air-mass trajectories, which were further used in the analysis of the (AOD550 and FM data for the three aerosol types). The HYSPLIT model was used to compute back trajectories at three altitudes to investigate the relation between AOD550-FM and wind sector depending on the altitude. The accumulation of local pollution is favored in spring and corresponds to air masses at lower altitudes originating from Eastern Europe and the Balkan. Clean maritime conditions are rare over Athens, limited in the winter season and associated with air masses from the Western or Northwestern sector. The coarse-mode particles origin seems to be more complicated proportionally to the season. Thus, in summer the Northern sector dominates, while in the other seasons, and especially in spring, the air masses belong to the Southern sector enriched with Saharan dust aerosols

    Results from the Fourth WMO Filter Radiometer Comparison for aerosol optical depth measurements

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    This study presents the results of the Fourth Filter Radiometer Comparison that was held in Davos, Switzerland, between 28 September and 16 October 2015. Thirty filter radiometers and spectroradiometers from 12 countries participated including reference instruments from global aerosol networks. The absolute differences of all instruments compared to the reference have been based on the World Meteorological Organization (WMO) criterion defined as follows: 95% of the measured data has to be within 0.005±0.001∕m (where m is the air mass). At least 24 out of 29 instruments achieved this goal at both 500 and 865nm, while 12 out of 17 and 13 out of 21 achieved this at 368 and 412nm, respectively. While searching for sources of differences among different instruments, it was found that all individual differences linked to Rayleigh, NO2, ozone, water vapor calculations and related optical depths and air mass calculations were smaller than 0.01 in aerosol optical depth (AOD) at 500 and 865nm. Different cloud-detecting algorithms used have been compared. Ångström exponent calculations showed relatively large differences among different instruments, partly because of the high calculation uncertainty of this parameter in low AOD conditions. The overall low deviations of these AOD results and the high accuracy of reference aerosol network instruments demonstrated a promising framework to achieve homogeneity, compatibility and harmonization among the different spectral AOD networks in the near future

    Outdoor particulate matter and childhood asthma admissions in Athens, Greece: a time-series study

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    <p>Abstract</p> <p>Background</p> <p>Particulate matter with diameter less than 10 micrometers (PM<sub>10</sub>) that originates from anthropogenic activities and natural sources may settle in the bronchi and cause adverse effects possibly via oxidative stress in susceptible individuals, such as asthmatic children. This study aimed to investigate the effect of outdoor PM<sub>10 </sub>concentrations on childhood asthma admissions (CAA) in Athens, Greece.</p> <p>Methods</p> <p>Daily counts of CAA from the three Children's Hospitals within the greater Athens' area were obtained from the hospital records during a four-year period (2001-2004, n = 3602 children). Mean daily PM<sub>10 </sub>concentrations recorded by the air pollution-monitoring network of the greater Athens area were also collected. The relationship between CAA and PM<sub>10 </sub>concentrations was investigated using the Generalized Linear Models with Poisson distribution and logistic analysis.</p> <p>Results</p> <p>There was a statistically significant (95% CL) relationship between CAA and mean daily PM<sub>10 </sub>concentrations on the day of exposure (+3.8% for 10 μg/m<sup>3 </sup>increase in PM<sub>10 </sub>concentrations), while a 1-day lag (+3.4% for 10 μg/m<sup>3 </sup>increase in PM<sub>10 </sub>concentrations) and a 4-day lag (+4.3% for 10 μg/m<sup>3 </sup>increase in PM<sub>10 </sub>concentrations) were observed for older asthmatic children (5-14 year-old). High mean daily PM<sub>10 </sub>concentration (the highest 10%; >65.69 μg/m<sup>3</sup>) doubled the risk of asthma exacerbations even in younger asthmatic children (0-4 year-old).</p> <p>Conclusions</p> <p>Our results provide evidence of the adverse effect of PM<sub>10 </sub>on the rates of paediatric asthma exacerbations and hospital admissions. A four-day lag effect between PM<sub>10 </sub>peak exposure and asthma admissions was also observed in the older age group.</p

    Aerosol climatology: dependence of the Angstrom exponent on wavelength over four AERONET sites

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    International audienceThe Ångström exponent, ?, is often used as a qualitative indicator of aerosol particle size. In this study, aerosol optical depth (AOD) and Ångström exponent (?) data were analyzed to obtain information about the adequacy of the simple use of the Ångström exponent for characterizing aerosols, and for exploring possibilities for a more efficient characterization of aerosols. This was made possible by taking advantage of the spectral variation of ?, the so-called curvature. The data were taken from four selected AERONET stations, which are representative of four aerosol types, i.e. biomass burning, pollution, desert dust and maritime. Using the least-squares method, the Ångström-? was calculated in the spectral interval 340?870 nm, along with the coefficients ?1 and ?2 of the second order polynomial fit to the plotted logarithm of AOD versus the logarithm of wavelength, and the second derivative of ?. The results show that the spectral curvature can provide important additional information about the different aerosol types, and can be effectively used to discriminate between them, since the fine-mode particles exhibit negative curvature, while the coarse-mode aerosols positive. In addition, the curvature has always to be taken into account in the computations of Ångström exponent values in the spectral intervals 380?440 nm and 675?870 nm, since fine-mode aerosols exhibit larger ?675?870 than ?380?440 values, and vice-versa for coarse-mode particles. A second-order polynomial fit simulates the spectral dependence of the AODs very well, while the associated constant term varies proportionally to the aerosol type. The correlation between the coefficients ?1 and ?2 of the second-order polynomial fit and the Ångström exponent ?, and the atmospheric turbidity, is further investigated. The obtained results reveal important features, which can be used for better discriminating between different aerosol types

    Identification of the Aerosol Types over Athens, Greece: The Influence of Air-Mass Transport

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    Aerosol optical depth at 550nm (AOD(550)) and fine-mode (FM) fraction data from Terra-MODIS were obtained over the Greater Athens Area covering the period February 2000-December 2005. Based on both AOD(550) and FM values three main aerosol types have been discriminated corresponding to urban/industrial aerosols, clean maritime conditions, and coarse-mode, probably desert dust, particles. Five main sectors were identified for the classification of the air-mass trajectories, which were further used in the analysis of the (AOD(550) and FM data for the three aerosol types). The HYSPLIT model was used to compute back trajectories at three altitudes to investigate the relation between AOD(550)-FM and wind sector depending on the altitude. The accumulation of local pollution is favored in spring and corresponds to air masses at lower altitudes originating from Eastern Europe and the Balkan. Clean maritime conditions are rare over Athens, limited in the winter season and associated with air masses from the Western or Northwestern sector. The coarse-mode particles origin seems to be more complicated proportionally to the season. Thus, in summer the Northern sector dominates, while in the other seasons, and especially in spring, the air masses belong to the Southern sector enriched with Saharan dust aerosols
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