Exotic magnetism on the quasi-FCC lattices of the d3d^3 double perovskites La2_2NaB′'O6_6 (B′' == Ru, Os)

We find evidence for long-range and short-range ($\zeta$ $=$ 70 \AA~at 4 K) incommensurate magnetic order on the quasi-face-centered-cubic (FCC) lattices of the monoclinic double perovskites La$_2$NaRuO$_6$ and La$_2$NaOsO$_6$ respectively. Incommensurate magnetic order on the FCC lattice has not been predicted by mean field theory, but may arise via a delicate balance of inequivalent nearest neighbour and next nearest neighbour exchange interactions. In the Ru system with long-range order, inelastic neutron scattering also reveals a spin gap $\Delta$ $\sim$ 2.75 meV. Magnetic anisotropy is generally minimized in the more familiar octahedrally-coordinated $3d^3$ systems, so the large gap observed for La$_2$NaRuO$_6$ may result from the significantly enhanced value of spin-orbit coupling in this $4d^3$ material.Comment: 5 pages, 4 figure

Effect of Mn substitution by Ga on the optical properties of a metallic manganite

In a metallic manganite like La(2/3)Sr(1/3)MnO(3), the substitution of Mn(+3) by Ga(+3) dilutes the ferromagnetic order and locally cancels the Jahn-Teller distortion, without heavily affecting the crystal structure. One can thus follow the changes in the charge dynamics induced by Ga, until the ferro-metallic manganite is turned into an insulator. Here this phenomenon is studied in detail through the infrared reflectivity of five samples of La(2/3)Sr(1/3)Mn(1-x)Ga(x)O(3), with x increasing from 0 to 0.30 and for 50 < T < 320 K. A simple model which links the measured optical parameters to the magnetization M(x, T) well describes the behavior of the plasma frequency, the scattering rate, and the mid-infrared absorption along the metal-to-insulator transition.Comment: 8 pages including 7 figure

Spectrum of a magnetized strong-leg quantum spin ladder

Inelastic neutron scattering is used to measure the spin excitation spectrum of the Heisenberg $S=1/2$ ladder material (C$_7$H$_10$N)$_2$CuBr$_4$ in its entirety, both in the gapped spin-liquid and the magnetic field induced Tomonaga-Luttinger spin liquid regimes. A fundamental change of the spin dynamics is observed between these two regimes. DMRG calculations quantitatively reproduce and help understand the observed commensurate and incommensurate excitations. The results validate long-standing quantum field theoretical predictions, but also test the limits of that approach

Spin dynamics of heterometallic Cr7M wheels (M = Mn, Zn, Ni) probed by inelastic neutron scattering

Inelastic neutron scattering has been applied to the study of the spin dynamics of Cr-based antiferromagnetic octanuclear rings where a finite total spin of the ground state is obtained by substituting one Cr(III) ion (s = 3/2) with Zn (s = 0), Mn (s = 5/2) or Ni (s = 1) di-cations. Energy and intensity measurements for several intra-multiplet and inter-multiplet magnetic excitations allow us to determine the spin wavefunctions of the investigated clusters. Effects due to the mixing of different spin multiplets have been considered. Such effects proved to be important to correctly reproduce the energy and intensity of magnetic excitations in the neutron spectra. On the contrary to what is observed for the parent homonuclear Cr8 ring, the symmetry of the first excited spin states is such that anticrossing conditions with the ground state can be realized in the presence of an external magnetic field. Heterometallic Cr7M wheels are therefore good candidates for macroscopic observations of quantum effects.Comment: 9 pages, 11 figures, submitted to Phys. Rev. B, corrected typos and added references, one sentence change

Bound states and field-polarized Haldane modes in a quantum spin ladder

The challenge of one-dimensional systems is to understand their physics beyond the level of known elementary excitations. By high-resolution neutron spectroscopy in a quantum spin ladder material, we probe the leading multiparticle excitation by characterizing the two-magnon bound state at zero field. By applying high magnetic fields, we create and select the singlet (longitudinal) and triplet (transverse) excitations of the fully spin-polarized ladder, which have not been observed previously and are close analogs of the modes anticipated in a polarized Haldane chain. Theoretical modelling of the dynamical response demonstrates our complete quantitative understanding of these states.Comment: 6 pages, 3 figures plus supplementary material 7 pages 5 figure

Stroboscopic Laser Diagnostics for Detection of Ordering in One-Dimensional Ion beam

A novel diagnostic method for detecting ordering in one-dimensional ion beams is presented. The ions are excited by a pulsed laser at two different positions along the beam and fluorescence is observed by a group of four photomultipliers. Correlation in fluorescence signals is firm indication that the ion beam has an ordered structure.Comment: 7 pages, REVTEX, fig3 uuencoded, figs 1-2 available upon request from [email protected], to appear in Phys. Rev.

Infrared characterization of silicon carbide nanowires

Silicon carbide nanowires have been obtained via combustion synthesis route. X-ray diffraction analysis confirmed that the synthesized material is the 3C polytype of silicon carbide with zincblende unit cell. Detailed investigations of such SiC 1D nanostructures were carried out exploiting Fourier transform infrared spectroscopy. IR measurements we performed using BRUKER HYPERION FT-IR microscope. For the purpose of comparison, a series of powder samples were examined, including raw synthesis product, purified SiC nanowires and several commercially available microand nanopowders (from Alpha Aesar and PlasmaChem). Comprehensive comparative analysis of the MIR spectra has been performed. When you are citing the document, use the following link http://essuir.sumdu.edu.ua/handle/123456789/2063