389 research outputs found
Auxiliary fermion approach to the resonant inelastic x-ray scattering response in an underdoped cuprate
We describe a method for calculating the resonant inelastic x-ray scattering (RIXS) response—including the dynamics of the transient core hole—of many-body systems with nontrivial gap structure encoded in their single particle Green's function. Our approach introduces auxiliary fermions in order to obtain a form amenable to the determinant method of Benjamin et al., [Phys. Rev. Lett. 112, 247002 (2014)], and is applicable to systems where interactions are most strongly felt through a renormalization of the single particle propagator. As a test case we consider the Yang-Rice-Zhang ansatz for cuprate phenomena in the underdoped “pseudogap” regime, which remains a popular tool for interpreting the results of experimental probes. We show that taking the core hole dynamics into account for a system described by this ansatz pushes the RIXS peaks towards higher energy transfer, improving agreement with experiments
Electronic structure, local magnetism, and spin-orbit effects of Ir(IV)-, Ir(V)-, and Ir(VI)-based compounds
Element- and orbital-selective x-ray absorption and magnetic circular dichroism measurements are carried out to probe the electronic structure and magnetism of Ir 5d electronic states in double perovskite Sr2MIrO6 (M=Mg, Ca, Sc, Ti, Ni, Fe, Zn, In) and La2NiIrO6 compounds. All the studied systems present a significant influence of spin-orbit interactions in the electronic ground state. In addition, we find that the Ir 5d local magnetic moment shows different character depending on the oxidation state despite the net magnetization being similar for all the compounds. Ir carries an orbital contribution comparable to the spin contribution for Ir4+ (5d5) and Ir5+ (5d4) oxides, whereas the orbital contribution is quenched for Ir6+ (5d3) samples. Incorporation of a magnetic 3d atom allows getting insight into the magnetic coupling between 5d and 3d transition metals. Together with previous susceptibility and neutron diffraction measurements, the results indicate that Ir carries a significant local magnetic moment even in samples without a 3d metal. The size of the (small) net magnetization of these compounds is a result of predominant antiferromagnetic interactions between local moments coupled with structural details of each perovskite structure.This work was partially supported by the Spanish MINECO Projects No. MAT2014-54425-R and No. MAT2013-41099-R and by the Comunidad de Madrid Project No. S2009/PPQ-1551. M. A. Laguna-Marco acknowledges CSIC and European
Social Fund for a JAE-Doc contract. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE)
Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357.Peer Reviewe
Resonant Inelastic X-Ray Scattering at the K Edge of Ge
We study the resonant inelastic x-ray scattering (RIXS) at the edge of
Ge. We measure RIXS spectra with systematically varying momenta in the final
state. The spectra are a measure of exciting an electron-hole pair. We find a
single peak structure (except the elastic peak) as a function of photon energy,
which is nearly independent of final-state momenta. We analyze the experimental
data by means of the band structure calculation. The calculation reproduces
well the experimental shape, clarifying the implication of the spectral shape.Comment: 17 pages,9 figures, Please also see our related paper:
cond-mat/040500
Transfer of Spectral Weight in Spectroscopies of Correlated Electron Systems
We study the transfer of spectral weight in the photoemission and optical
spectra of strongly correlated electron systems. Within the LISA, that becomes
exact in the limit of large lattice coordination, we consider and compare two
models of correlated electrons, the Hubbard model and the periodic Anderson
model. The results are discussed in regard of recent experiments. In the
Hubbard model, we predict an anomalous enhancement optical spectral weight as a
function of temperature in the correlated metallic state which is in
qualitative agreement with optical measurements in . We argue that
anomalies observed in the spectroscopy of the metal are connected to the
proximity to a crossover region in the phase diagram of the model. In the
insulating phase, we obtain an excellent agreement with the experimental data
and present a detailed discussion on the role of magnetic frustration by
studying the resolved single particle spectra. The results for the periodic
Anderson model are discussed in connection to recent experimental data of the
Kondo insulators and . The model can successfully explain
the different energy scales that are associated to the thermal filling of the
optical gap, which we also relate to corresponding changes in the density of
states. The temperature dependence of the optical sum rule is obtained and its
relevance for the interpretation of the experimental data discussed. Finally,
we argue that the large scattering rate measured in Kondo insulators cannot be
described by the periodic Anderson model.Comment: 19 pages + 29 figures. Submitted to PR
Comment on ``Spin Polarization and Magnetic Circular Dichroism in Photoemission from the 2p Core Level of Ferromagnetic Ni''
Although the Ni_4 cluster includes more information regarding the Ni band
structure with respect to the Anderson impurity model, it also favors very
peculiar ground states which are incompatible with a coherent picture of all
dichroism experiments.Comment: 1 page, RevTeX, 1 epsf figur
Resonant Inelastic X-ray Scattering Studies of Elementary Excitations
In the past decade, Resonant Inelastic X-ray Scattering (RIXS) has made
remarkable progress as a spectroscopic technique. This is a direct result of
the availability of high-brilliance synchrotron X-ray radiation sources and of
advanced photon detection instrumentation. The technique's unique capability to
probe elementary excitations in complex materials by measuring their energy-,
momentum-, and polarization-dependence has brought RIXS to the forefront of
experimental photon science. We review both the experimental and theoretical
RIXS investigations of the past decade, focusing on those determining the
low-energy charge, spin, orbital and lattice excitations of solids. We present
the fundamentals of RIXS as an experimental method and then review the
theoretical state of affairs, its recent developments and discuss the different
(approximate) methods to compute the dynamical RIXS response. The last decade's
body of experimental RIXS data and its interpretation is surveyed, with an
emphasis on RIXS studies of correlated electron systems, especially transition
metal compounds. Finally, we discuss the promise that RIXS holds for the near
future, particularly in view of the advent of x-ray laser photon sources.Comment: Review, 67 pages, 44 figure
The Herschel Comprehensive (U)LIRG Emission Survey (HerCULES): CO Ladders, fine structure lines, and neutral gas cooling
(Ultra) Luminous Infrared Galaxies ((U)LIRGs) are objects characterized by
their extreme infrared (8-1000 m) luminosities (L and L). The Herschel Comprehensive ULIRG
Emission Survey (HerCULES; PI van der Werf) presents a representative
flux-limited sample of 29 (U)LIRGs that spans the full luminosity range of
these objects (10). With the \emph{Herschel
Space Observatory}, we observe [CII] 157 m, [OI] 63 m, and [OI] 145
m line emission with PACS, CO J=4-3 through J=13-12, [CI] 370 m, and
[CI] 609 m with SPIRE, and low-J CO transitions with ground-based
telescopes. The CO ladders of the sample are separated into three classes based
on their excitation level. In 13 of the galaxies, the [OI] 63 m emission
line is self absorbed. Comparing the CO excitation to the IRAS 60/100 m
ratio and to far infrared luminosity, we find that the CO excitation is more
correlated to the far infrared colors. We present cooling budgets for the
galaxies and find fine-structure line flux deficits in the [CII], [SiII], [OI],
and [CI] lines in the objects with the highest far IR fluxes, but do not
observe this for CO . In order to study the heating of the
molecular gas, we present a combination of three diagnostic quantities to help
determine the dominant heating source. Using the CO excitation, the CO J=1-0
linewidth, and the AGN contribution, we conclude that galaxies with large CO
linewidths always have high-excitation CO ladders, and often low AGN
contributions, suggesting that mechanical heating is important
Recommended from our members
Stability of the ferromagnetic ground state of La₂ MnNiO₆ against large compressive stress
The effect of quasi-hydrostatic pressure upon the ferromagnetic ground state of magnetodielectric, double-
perovskite La₂ MnNiO₆ is investigated using x-ray absorption spectroscopy and diffraction measurements in a
diamond anvil cell. The Mn-O-Ni superexchange interaction that gives rise to ferromagnetism in this cation-
ordered structure is stable to at least 38 GPa (380 000 atm). Such unusual stability of a ferromagnetic state to
applied pressure can be rationalized in terms of the electronic and crystal structure and should help preserve
the outstanding electronic and magnetic properties of this material when grown epitaxially under moderate
compressive and tensile strain conditions
The potential and limitations of intrahepatic cholangiocyte organoids to study inborn errors of metabolism
Inborn errors of metabolism (IEMs) comprise a diverse group of individually rare monogenic disorders that affect metabolic pathways. Mutations lead to enzymatic deficiency or dysfunction, which results in intermediate metabolite accumulation or deficit leading to disease phenotypes. Currently, treatment options for many IEMs are insufficient. Rarity of individual IEMs hampers therapy development and phenotypic and genetic heterogeneity suggest beneficial effects of personalized approaches. Recently, cultures of patient-own liver-derived intrahepatic cholangiocyte organoids (ICOs) have been established. Since most metabolic genes are expressed in the liver, patient-derived ICOs represent exciting possibilities for in vitro modeling and personalized drug testing for IEMs. However, the exact application range of ICOs remains unclear. To address this, we examined which metabolic pathways can be studied with ICOs and what the potential and limitations of patient-derived ICOs are to model metabolic functions. We present functional assays in patient ICOs with defects in branched-chain amino acid metabolism (methylmalonic acidemia), copper metabolism (Wilson disease), and transporter defects (cystic fibrosis). We discuss the broad range of functional assays that can be applied to ICOs, but also address the limitations of these patient-specific cell models. In doing so, we aim to guide the selection of the appropriate cell model for studies of a specific disease or metabolic process
- …