83 research outputs found

    Investigation of the ferromagnetic transition in the correlated 4d perovskites SrRu1−x_{1-x}Rhx_xO3_3

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    The solid-solution SrRu1−x_{1-x}Rhx_xO3_3 (0≀x≀10\le x \le1) is a variable-electron-configuration system forming in the nearly-cubic-perovskite basis, ranging from the ferromagnetic 4d4d^4 to the enhanced paramagnetic 4d5d^5. Polycrystalline single-phase samples were obtained over the whole composition range by a high-pressure-heating technique, followed by measurements of magnetic susceptibility, magnetization, specific heat, thermopower, and electrical resistivity. The ferromagnetic order in long range is gradually suppressed by the Rh substitution and vanishes at x∌0.6x \sim 0.6. The electronic term of specific-heat shows unusual behavior near the critical Rh concentration; the feature does not match even qualitatively with what was reported for the related perovskites (Sr,Ca)RuO3_3. Furthermore, another anomaly in the specific heat was observed at x∌0.9x \sim 0.9.Comment: Accepted for publication in PR

    Non-Fermi liquid behavior and scaling of low frequency suppression in optical conductivity spectra of CaRuO3_3

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    Optical conductivity spectra σ1(ω)\sigma_1(\omega) of paramagnetic CaRuO3_3 are investigated at various temperatures. At T=10 K, it shows a non-Fermi liquid behavior of σ1(ω)∌1/ω12\sigma_1(\omega)\sim 1/{\omega}^{\frac 12}, similar to the case of a ferromagnet SrRuO3_3. As the temperature (TT) is increased, on the other hand, σ1(ω)\sigma_1(\omega) in the low frequency region is progressively suppressed, deviating from the 1/{\omega}^{\frac 12%}-dependence. Interestingly, the suppression of σ1(ω)\sigma_1(\omega) is found to scale with ω/T\omega /T at all temperatures. The origin of the % \omega /T scaling behavior coupled with the non-Fermi liquid behavior is discussed.Comment: 4 pages, 3 figure

    Optical investigation on the electronic structures of Y_{2}Ru_{2}O_{7}, CaRuO_{3}, SrRuO_{3}, and Bi_{2}Ru_{2}O_{7}

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    We investigated the electronic structures of the bandwidth-controlled ruthenates, Y2_{2}Ru2_{2}O7_{7}, CaRuO3_{3}, SrRuO3_{3}, and Bi2_{2}Ru2% _{2}O7_{7}, by optical conductivity analysis in a wide energy region of 5 meV ∌\sim 12 eV. We could assign optical transitions from the systematic changes of the spectra and by comparison with the O 1ss x-ray absorption data. We estimated some physical parameters, such as the on-site Coulomb repulsion energy and the crystal-field splitting energy. These parameters show that the 4dd orbitals should be more extended than 3dd ones. These results are also discussed in terms of the Mott-Hubbard model.Comment: 12 pages (1 table), 3 figure

    Heavy Carriers and Non-Drude Optical Conductivity in MnSi

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    Optical properties of the weakly helimagnetic metal MnSi have been determined in the photon energy range from 2 meV to 4.5 eV using the combination of grazing incidence reflectance at 80 degrees (2 meV to 0.8 eV) and ellipsometry (0.8 to 4.5 eV). As the sample is cooled below 100 K the effective mass becomes strongly frequency dependent at low frequencies, while the scattering rate developes a linear frequency dependence. The complex optical conductivity can be described by the phenomenological relation \sigma(\omega,T) \propto (\Gamma(T)+i\omega)^{-1/2} used for cuprates and ruthenates.Comment: 5 pages, ReVTeX 4, 5 figures in eps forma

    Phonon anomalies and electron-phonon interaction in RuSr_2GdCu_2O_8 ferromagnetic superconductor: Evidence from infrared conductivity

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    Critical behavior of the infrared reflectivity of RuSr_2GdCu_2O_8 ceramics is observed near the superconducting T_{SC} = 45 K and magnetic T_M = 133 K transition temperatures. The optical conductivity reveals the typical features of the c-axis optical conductivity of strongly underdoped multilayer superconducting cuprates. The transformation of the Cu-O bending mode at 288 cm^{-1} to a broad absorption peak at the temperatures between T^* = 90 K and T_{SC} is clearly observed, and is accompanied by the suppression of spectral weight at low frequencies. The correlated shifts to lower frequencies of the Ru-related phonon mode at 190 cm^{-1} and the mid-IR band at 4800 cm^{-1} on decreasing temperature below T_M are observed. It provides experimental evidence in favor of strong electron-phonon coupling of the charge carriers in the Ru-O layers which critically depends on the Ru core spin alignment. The underdoped character of the superconductor is explained by strong hole depletion of the CuO_2 planes caused by the charge carrier self-trapping at the Ru moments.Comment: 11 pages incl. 5 figures, submitted to PR

    Efficacy of Maternal Choline Supplementation During Pregnancy in Mitigating Adverse Effects of Prenatal Alcohol Exposure on Growth and Cognitive Function: A Randomized, Double-Blind, Placebo-Controlled Clinical Trial

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    Background: We recently demonstrated the acceptability and feasibility of a randomized, double-blind choline supplementation intervention for heavy drinking women during pregnancy. In this study, we report our results relating to the efficacy of this intervention in mitigating adverse effects of prenatal alcohol exposure (PAE) on infant growth and cognitive function. Methods: Sixty-nine Cape Coloured (mixed ancestry) heavy drinkers in Cape Town, South Africa, recruited in mid-pregnancy, were randomly assigned to receive a daily oral dose of either 2 g of choline or placebo from time of enrollment until delivery. Each dose consisted of an individually wrapped packet of powder that, when mixed with water, produced a sweet tasting grape-flavored drink. The primary outcome, eyeblink conditioning (EBC), was assessed at 6.5 months. Somatic growth was measured at birth, 6.5, and 12 months, recognition memory and processing speed on the Fagan Test of Infant Intelligence, at 6.5 and 12 months. Results: Infants born to choline-treated mothers were more likely to meet criterion for conditioning on EBC than the placebo group. Moreover, within the choline arm, degree of maternal adherence to the supplementation protocol strongly predicted EBC performance. Both groups were small at birth, but choline-treated infants showed considerable catch-up growth in weight and head circumference at 6.5 and 12 months. At 12 months, the infants in the choline treatment arm had higher novelty preference scores, indicating better visual recognition memory. Conclusions: This exploratory study is the first to provide evidence that a high dose of choline administered early in pregnancy can mitigate adverse effects of heavy PAE on EBC, postnatal growth, and cognition in human infants. These findings are consistent with studies of alcohol-exposed animals that have demonstrated beneficial effects of choline supplementation on classical conditioning, learning, and memory

    Virtual Compton Scattering and Neutral Pion Electroproduction in the Resonance Region up to the Deep Inelastic Region at Backward Angles

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    We have made the first measurements of the virtual Compton scattering (VCS) process via the H(e,eâ€Čp)Îł(e,e'p)\gamma exclusive reaction in the nucleon resonance region, at backward angles. Results are presented for the WW-dependence at fixed Q2=1Q^2=1 GeV2^2, and for the Q2Q^2-dependence at fixed WW near 1.5 GeV. The VCS data show resonant structures in the first and second resonance regions. The observed Q2Q^2-dependence is smooth. The measured ratio of H(e,eâ€Čp)Îł(e,e'p)\gamma to H(e,eâ€Čp)π0(e,e'p)\pi^0 cross sections emphasizes the different sensitivity of these two reactions to the various nucleon resonances. Finally, when compared to Real Compton Scattering (RCS) at high energy and large angles, our VCS data at the highest WW (1.8-1.9 GeV) show a striking Q2Q^2- independence, which may suggest a transition to a perturbative scattering mechanism at the quark level.Comment: 20 pages, 8 figures. To appear in Phys.Rev.

    Consensus on the use and interpretation of cystic fibrosis mutation analysis in clinical practice

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    It is often challenging for the clinician interested in cystic fibrosis (CF) to interpret molecular genetic results, and to integrate them in the diagnostic process. The limitations of genotyping technology, the choice of mutations to be tested, and the clinical context in which the test is administered can all influence how genetic information is interpreted. This paper describes the conclusions of a consensus conference to address the use and interpretation of CF mutation analysis in clinical settings
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