413 research outputs found

    Critical Phenomena at the Antiferromagnetic Phase Transition of Azurite

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    We report on high-resolution acoustic, specific-heat and thermal expansion measurements in the vicinity of the antiferromagnetic phase transition at T_N = 1.88 K on a high-quality single crystal of the natural mineral azurite. A detailed investigation of the critical contribution to the various quantities at T_N is presented. The set of critical exponents and amplitude ratios of the singular contributions above and below the transition indicate that the system can be reasonably well described by a three-dimensional Heisenberg antiferromagnet.Comment: 9 pages, 3 figures, proceedings of ICM 2012, JKP

    Geometrical quadrupolar frustration in DyB4_4

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    Physical properties of DyB4_4 have been studied by magnetization, specific heat, and ultrasonic measurements. The magnetic entropy change and the ultrasonic properties in the intermediate phase II indicate that the degeneracy of internal degrees of freedom is not fully lifted in spite of the formation of magnetic order. The ultrasonic attenuation and the huge softening of C44C_{44} in phase II suggests existence of electric-quadrupolar (orbital) fluctuations of the 4ff-electron. These unusual properties originate from the geometrical quadrupolar frustration.Comment: 4 pages, 4 figures, accepted for publication in Journal of the Physical Society of Japa

    Submillimeter and X-ray observations of an X Class flare

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    The GOES X1.5 class flare that occurred on August 30,2002 at 1327:30 UT is one of the few events detected so far at submillimeter wavelengths. We present a detailed analysis of this flare combining radio observations from 1.5 to 212 GHz (an upper limit of the flux is also provided at 405 GHz) and X-ray. Although the observations of radio emission up to 212 GHz indicates that relativistic electrons with energies of a few MeV were accelerated, no significant hard X-ray emission was detected by RHESSI above ~ 250 keV. Images at 12--20 and 50--100 keV reveal a very compact, but resolved, source of about ~ 10" x 10". EUV TRACE images show a multi-kernel structure suggesting a complex (multipolar) magnetic topology. During the peak time the radio spectrum shows an extended flatness from ~ 7 to 35 GHz. Modeling the optically thin part of the radio spectrum as gyrosynchrotron emission we obtained the electron spectrum (spectral index delta, instantaneous number of emitting electrons). It is shown that in order to keep the expected X-ray emission from the same emitting electrons below the RHESSI background at 250 keV, a magnetic field above 500 G is necessary. On the other hand, the electron spectrum deduced from radio observations >= 50 GHz is harder than that deduced from ~ 70 - 250 keV X-ray data, meaning that there must exist a breaking energy around a few hundred keV. During the decay of the impulsive phase, a hardening of the X-ray spectrum is observed which is interpreted as a hardening of the electron distribution spectrum produced by the diffusion due to Coulomb collisions of the trapped electrons in a medium with an electron density of n_e ~ 3E10 - 5E10 cm-3.Comment: Accpeted in Astronomy & Astrophysics. 9 Pages, 6 Figures ADDED REFERENCE

    Gap opening and orbital modification of superconducting FeSe above the structural distortion

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    We utilize steady-state and transient optical spectroscopies to examine the responses of nonthermal quasiparticles with respect to orbital modifications in normal-state iron-chalcogenide superconductors. The dynamics shows the emergence of gap-like quasiparticles (associated to a ~36 meV energy gap) with a coincident transfer of the optical spectral weight in the visible range, at temperatures above the structural distortion. Our observations suggest that opening of the high-temperature gap and the lattice symmetry breaking are possibly driven by short-range orbital and/or charge orders, implicating a close correlation between electronic nematicity and precursor order in iron-based superconductors

    A burst with double radio spectrum observed up to 212 GHz

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    We study a solar flare that occurred on September 10, 2002, in active region NOAA 10105 starting around 14:52 UT and lasting approximately 5 minutes in the radio range. The event was classified as M2.9 in X-rays and 1N in H\alpha. Solar Submillimeter Telescope observations, in addition to microwave data give us a good spectral coverage between 1.415 and 212 GHz. We combine these data with ultraviolet images, hard and soft X-rays observations and full-disk magnetograms. Images obtained from Ramaty High Energy Solar Spectroscopic Imaging data are used to identify the locations of X-ray sources at different energies and to determine the X-ray spectrum, while ultra violet images allow us to characterize the coronal flaring region. The magnetic field evolution of the active region is analyzed using Michelson Doppler Imager magnetograms. The burst is detected at all available radio-frequencies. X-ray images (between 12 keV and 300 keV) reveal two compact sources and 212 GHz data, used to estimate the radio source position, show a single compact source displaced by 25" from one of the hard X-ray footpoints. We model the radio spectra using two homogeneous sources, and combine this analysis with that of hard X-rays to understand the dynamics of the particles. Relativistic particles, observed at radio wavelengths above 50 GHz, have an electron index evolving with the typical soft-hard-soft behaviour.Comment: Submitted to Solar Physics, 20 pages, 8 fugure

    Magneto-structural transitions in a frustrated magnet at high fields

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    Ultrasound and magnetization studies of bond-frustrated ZnCr2S4 spinel are performed in static magnetic fields up to 18 T and in pulsed fields up to 62 T. At temperatures below the antiferromagnetic transition at T_N1 14 K the sound velocity as function of magnetic field reveals a sequence of steps followed by plateaus indicating a succession of crystallographic structures with constant stiffness. At the same time, the magnetization evolves continuously with field up to full magnetic polarization without any plateaus in contrast to geometrically frustrated chromium oxide spinels. The observed high-field magneto-structural states are discussed within a H-T phase diagram taking into account the field and temperature evolution of three coexisting spin structures and subsequent lattice transformations induced by magnetic field.Comment: 4 pages, 3 figure

    Magnetic phase transitions in Gd64Sc36 studied using non-contact ultrasonics

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    The speed and attenuation of ultrasound propagation can be used to determine material properties and identify phase transitions. Standard ultrasonic contact techniques are not always convenient due to the necessity of using couplant; however, recently reliable non-contact ultrasonic techniques involving electromagnetic generation and detection of ultrasound with electromagnetic acoustic transducers (EMATs) have been developed for use on electrically conducting and/or magnetic materials. We present a detailed study of magnetic phase transitions in a single crystal sample of Gd64Sc36 magnetic alloy using contact and non-contact ultrasonic techniques for two orientations of external magnetic field. Phase diagrams are constructed based on measurements of elastic constant C33, the attenuation and the efficiency of generation when using an EMAT. The EMATs are shown to provide additional information related to the magnetic phase transitions in the studied sample, and results identify a conical helix phase in Gd64Sc36 in the magnetic field orientation

    Anomalous elastic softening of SmRu_{4}P_{12} under high pressure

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    The filled skutterudite compound SmRu_4P_{12} undergoes a complex evolution from a paramagnetic metal (phase I) to a probable multipolar ordering insulator (phase II) at T_{MI} = 16.5 K, then to a magnetically ordered phase (phase III) at T_{N} = 14 K. Elastic properties under hydrostatic pressures were investigated to study the nature of the ordering phases. We found that distinct elastic softening above T_{MI} is induced by pressure, giving evidence of quadrupole degeneracy of the ground state in the crystalline electric field. It also suggests that quadrupole moment may be one of the order parameters below T_{MI} under pressure. Strangely, the largest degree of softening is found in the transverse elastic constant C_{T} at around 0.5-0.6 GPa, presumably having relevancy to the competing and very different Gruneisen parameters \Omega of T_{MI} and T_{N}. Interplay between the two phase transitions is also verified by the rapid increase of T_{MI} under pressure with a considerably large \Omega of 9. Our results can be understood on the basis of the proposed octupole scenario for SmRu_4P_{12}.Comment: 7 pages, 7 figure

    Solving variational inequalities defined on a domain with infinitely many linear constraints

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    We study a variational inequality problem whose domain is defined by infinitely many linear inequalities. A discretization method and an analytic center based inexact cutting plane method are proposed. Under proper assumptions, the convergence results for both methods are given. We also provide numerical examples to illustrate the proposed method
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