An improved method for estimating the neutron background in measurements of neutron capture reactions

The relation between the neutron background in neutron capture measurements and the neutron sensitivity related to the experimental setup is examined. It is pointed out that a proper estimate of the neutron background may only be obtained by means of dedicated simulations taking into account the full framework of the neutron-induced reactions and their complete temporal evolution. No other presently available method seems to provide reliable results, in particular under the capture resonances. An improved neutron background estimation technique is proposed, the main improvement regarding the treatment of the neutron sensitivity, taking into account the temporal evolution of the neutron-induced reactions. The technique is complemented by an advanced data analysis procedure based on relativistic kinematics of neutron scattering. The analysis procedure allows for the calculation of the neutron background in capture measurements, without requiring the time-consuming simulations to be adapted to each particular sample. A suggestion is made on how to improve the neutron background estimates if neutron background simulations are not available.Comment: 11 pages, 9 figure

High-accuracy determination of the neutron flux in the new experimental area n_TOF-EAR2 at CERN

A new high flux experimental area has recently become operational at the n_TOF facility at CERN. This new measuring station, n_TOF-EAR2, is placed at the end of a vertical beam line at a distance of approximately 20m from the spallation target. The characterization of the neutron beam, in terms of flux, spatial profile and resolution function, is of crucial importance for the feasibility study and data analysis of all measurements to be performed in the new area. In this paper, the measurement of the neutron flux, performed with different solid-state and gaseous detection systems, and using three neutron-converting reactions considered standard in different energy regions is reported. The results of the various measurements have been combined, yielding an evaluated neutron energy distribution in a wide energy range, from 2meV to 100MeV, with an accuracy ranging from 2%, at low energy, to 6% in the high-energy region. In addition, an absolute normalization of the n_TOF-EAR2 neutron flux has been obtained by means of an activation measurement performed with 197Au foils in the beam.Comisión Europea FP7/2007-2011 No.605203Centro Nacional de Ciencias de Polonia UMO- 2012/04/M/ST2/00700Centro Nacional de Ciencias de Polonia UMO-2016/22/M/ST2/00183Fundación de Ciencia Croata No. 168

The neutron time-of-flight facility n-TOF at CERN: Phase II

Neutron-induced reactions are studied at the neutron time-of-flight facility n-TOF at CERN. The facility uses 6∼ns wide pulses of 20 GeV/c protons impinging on a lead spallation target. The large neutron energy range and the high instantaneous neutron flux combined with high resolution are among the key characteristics of the facility. After a first phase of data taking during the period 2001-2004, the facility has been refurbished with an upgraded spallation target and cooling system for a second phase of data taking which started in 2009. Since 2010, the experimental area at 185 m where the neutron beam arrives, has been modified into a worksector of type A, allowing the extension of the physics program to include neutron-induced reactions on radioactive isotopes

Pulse processing routines for neutron time-of-flight data

A pulse shape analysis framework is described, which was developed for n_TOF-Phase3, the third phase in the operation of the n_TOF facility at CERN. The most notable feature of this new framework is the adoption of generic pulse shape analysis routines, characterized by a minimal number of explicit assumptions about the nature of pulses. The aim of these routines is to be applicable to a wide variety of detectors, thus facilitating the introduction of the new detectors or types of detectors into the analysis framework. The operational details of the routines are suited to the specific requirements of particular detectors by adjusting the set of external input parameters. Pulse recognition, baseline calculation and the pulse shape fitting procedure are described. Special emphasis is put on their computational efficiency, since the most basic implementations of these conceptually simple methods are often computationally inefficient.Comment: 13 pages, 10 figures, 5 table

Observation of large scissors resonance strength in actinides

The orbital M1-scissors resonance (SR) has been measured for the first time in the quasi-continuum of actinides. Particle-gamma coincidences are recorded with deuteron and 3He induced reactions on 232Th. The residual nuclei 231,232,233Th and 232,233Pa show an unexpectedly strong integrated strength of $B_{M1} = 11-15 \mu_{n}^{2}$ in the Egamma=1.0 - 3.5 MeV region. The increased gamma-decay probability in actinides due to the SR is important for cross-section calculations for future fuel cycles of fast nuclear reactors and may also have impact on stellar nucleosynthesis.Comment: 5 pages and 4 figure

Neutron transmission and capture of 241Am

A set of neutron transmission and capture experiments based on the Time Of Flight (TOF) technique, were performed in order to determine the 241Am capture cross section in the energy range from 0.01 eV to 1 keV. The GELINA facility of the Institute for Reference Materials and Measurements (IRMM) served as the neutron source. A pair of C6D6 liquid scintillators was used to register the prompt gamma rays emerging from the americium sample, while a Li-glass detector was used in the transmission setup. Results from the capture and transmission data acquired are consistent with each other, but appear to be inconsistent with the evaluated data files. Resonance parameters have been derived for the data up to the energy of 100 eV.JRC.D.4-Standards for Nuclear Safety, Security and Safeguard

Scissors resonance in the quasi-continuum of Th, Pa and U isotopes

The gamma-ray strength function in the quasi-continuum has been measured for 231-233Th, 232,233Pa and 237-239U using the Oslo method. All eight nuclei show a pronounced increase in gamma strength at omega_SR approx 2.4 MeV, which is interpreted as the low-energy M1 scissors resonance (SR). The total strength is found to be B_SR = 9-11 mu_N^2 when integrated over the 1 - 4 MeV gamma-energy region. The SR displays a double-hump structure that is theoretically not understood. Our results are compared with data from (gamma, gamma') experiments and theoretical sum-rule estimates for a nuclear rigid-body moment of inertia.Comment: 11 pages, 9 figure

Measurement of the 70Ge(n,γ) cross section up to 300 keV at the CERN n_TOF facility

Neutron capture data on intermediate mass nuclei are of key importance to nucleosynthesis in the weak component of the slow neutron capture processes, which occurs in massive stars. The (n,γ) cross section on 70Ge, which is mainly produced in the s process, was measured at the neutron time-of-flight facility n_TOF at CERN. Resonance capture kernels were determined up to 40 keV neutron energy and average cross sections up to 300 keV. Stellar cross sections were calculated from kT =5 keV tokT =100 keV and are in very good agreement with a previous measurement by Walter and Beer (1985) and recent evaluations. Average cross sectionsareinagreementwithWalterandBeer(1985)overmostoftheneutronenergyrangecovered,whilethey aresystematicallysmallerforneutronenergiesabove150keV.Wehavecalculatedisotopicabundancesproduced in s-process environments in a 25 solar mass star for two initial metallicities (below solar and close to solar). While the low metallicity model reproduces best the solar system germanium isotopic abundances, the close to solar model shows a good global match to solar system abundances in the range of mass numbers A=60–80.Austrian Science Fund J3503Adolf Messer Foundation ST/M006085/1European Research Council ERC2015-StGCroatian Science Foundation IP-2018-01-857

Design study for a new spallation target of the n_TOF facility at CERN

The n_TOF facility is a time of flight spectrometer dedicated to measuring neutron capture and fission cross sections. The neutron source consists on a lead target bombarded by a high energetic proton beam. After finishing a successful period of data taking by the end of 2004, it has been decided to upgrade the neutron spallation source with a cladded target. In this study, Monte Carlo simulations are reported for the assessment and comparison of the neutron and gamma fluxes from different target configurations. In addition, the plans for a second vertical measuring station with a flight path of 20 m above the spallation target have been considered in the simulations as well. Results for the energy deposition and the target heating are also presented

Measurement of the 242Pu(n,f) cross section at n_TOF

Knowledge of neutron cross sections of various plutonium isotopes and other minor actinides is crucial for the design of advanced nuclear systems. The 242Pu(n,f) cross sections were measured at the CERN n-TOF facility, taking advantage of the wide energy range (from thermal to GeV) and the high instantaneous flux of the neutron beam. In this work, preliminary results are presented along with a theoretical cross section calculation performed with the EMPIRE code. © Owned by the authors, published by EDP Sciences, 2014