307 research outputs found

    Tailoring correlations of the local density of states in disordered photonic materials

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    We present experimental evidence for the different mechanisms driving the fluctuations of the local density of states (LDOS) in disordered photonic systems. We establish a clear link between the microscopic structure of the material and the frequency correlation function of LDOS accessed by a near-field hyperspectral imaging technique. We show, in particular, that short- and long-range frequency correlations of LDOS are controlled by different physical processes (multiple or single scattering processes, respectively) that can be---to some extent---manipulated independently. We also demonstrate that the single scattering contribution to LDOS fluctuations is sensitive to subwavelength features of the material and, in particular, to the correlation length of its dielectric function. Our work paves a way towards a complete control of statistical properties of disordered photonic systems, allowing for designing materials with predefined correlations of LDOS.Comment: 5+9 pages, 5+6 figures. Fixed confusion of references between the main text and the supplemental material in version

    Large K-exciton dynamics in GaN epilayers: the non-thermal and thermal regime

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    We present a detailed investigation concerning the exciton dynamics in GaN epilayers grown on c-plane sapphire substrates, focussing on the exciton formation and the transition from the nonthermal to the thermal regime. The time-resolved kinetics of LO-phonon replicas is used to address the energy relaxation in the excitonic band. From ps time-resolved spectra we bring evidence for a long lasting non-thermal excitonic distribution which accounts for the rst 50 ps. Such a behavior is con rmed in di erent experimental conditions, both when non-resonant and resonant excitation are used. At low excitation power density the exciton formation and their subsequent thermalization is dominated by impurity scattering rather than by acoustic phonon scattering. The estimate of the average energy of the excitons as a function of delay after the excitation pulse provides information on the relaxation time, which describes the evolution of the exciton population to the thermal regime.Comment: 9 pages,8 figure

    Excitonic Effects in Quantum Wires

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    We review the effects of Coulomb correlation on the linear and non-linear optical properties of semiconductor quantum wires, with emphasis on recent results for the bound excitonic states. Our theoretical approach is based on generalized semiconductor Bloch equations, and allows full three-dimensional multisubband description of electron-hole correlation for arbitrary confinement profiles. In particular, we consider V- and T-shaped structures for which significant experimental advances were obtained recently. Above band gap, a very general result obtained by this approach is that electron-hole Coulomb correlation removes the inverse-square-root single-particle singularity in the optical spectra at band edge, in agreement with previous reports from purely one-dimensional models. Strong correlation effects on transitions in the continuum are found to persist also at high densities of photoexcited carriers. Below bandgap, we find that the same potential- (Coulomb) to kinetic-energy ratio holds for quite different wire cross sections and compositions. As a consequence, we identify a shape- and barrier-independent parameter that governs a universal scaling law for exciton binding energy with size. Previous indications that the shape of the wire cross-section may have important effects on exciton binding are discussed in the light of the present results.Comment: Proc. OECS-5 Conference, G\"ottingen, 1997 (To appear in Phys. Stat. Sol. (b)

    Multimode photonic molecules for advanced force sensing

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    We propose a force sensor, with optical detection, based on a reconfigurable multicavity photonic molecule distributed over two parallel photonic crystal membranes. The system spectral behaviour is described with an analytical model based on coupled mode theory and validated by finite difference time domain simulations. The deformation of the upper photonic crystal membrane, due to a localized vertical force, is monitored by the relative spectral positions of the photonic molecule resonances. The proposed system can act both as force sensor, with pico-newton sensitivity, able to identify the position where the force is applied, and as torque sensor able to measure the torsion of the membrane along two perpendicular directions

    Post-fabrication control of evanescent tunnelling in photonic crystal molecules

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    The post-fabrication control of evanescent tunnelling in photonic crystal molecules is demonstrated through the combination of selective infiltration and oxidation. By laser non thermal oxidation, we reduce the photonic coupling by more than 30% while by means of water micro-infiltration, we increase it by 28%. Fine-tuning of the photonic coupling is achieved by low-power laser oxidation and forced evaporation, opening the route to post-fabrication control of array of coupled cavities

    Superlinear emission in bare perovskite: amplified spontaneous emission in disordered film versus single crystal lasing

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    Abstract We present an experimental study concerning the superlinear emission in organic-inorganic halide perovskites. Microphotoluminescence experiments under CW and picosecond excitation condition at low temperature and near field optical photoluminescence spectra at room temperature provide clear evidence of the very different origin of the superlinear regime in disordered films and microplates/microwires. Insights on the origin of modal structures of the emission spectra in the high excitation regime will be given by polarization-resolved photoluminescence experiments

    Near-field imaging of single walled carbon nanotubes emitting in the telecom wavelength range

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    International audienceHybrid systems based on carbon nanotubes emitting in the telecom wavelength range and Si-photonic platforms are promising candidates for developing integrated photonic circuits. Here, we consider semiconducting single walled carbon nanotubes (s-SWNTs) emitting around 1300 nm or 1550 nm wavelength. The nanotubes are deposited on quartz substrate for mapping their photoluminescence in hyperspectral near-field microscopy. This method allows for a sub-wavelength resolution in detecting the spatial distribution of the emission of single s-SWNTs at room temperature. Optical signature delocalized over several micrometers is observed, thus denoting the high quality of the produced carbon nanotubes on a wide range of tube diameters. Noteworthy, the presence of both nanotube bundles and distinct s-SWNT chiralities is uncovered

    Nonlinear optical tuning of photonic crystal microcavities by near-field probe

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    We report on a nonlinear way to control and tune the dielectric environment of photonic crystalmicrocavities exploiting the local heating induced by near-field laser excitation at differentexcitation powers. The temperature gradient due to the optical absorption results in an index ofrefraction gradient which modifies the dielectric surroundings of the cavity and shifts the opticalmodes. Reversible tuning can be obtained either by changing the excitation power density or byexciting in different points of the photonic crystal microcavity
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