A new type of temperature driven reorientation transition in magnetic thin films

We present a new type of temperature driven spin reorientation transition (SRT) in thin films. It can occur when the lattice and the shape anisotropy favor different easy directions of the magnetization. Due to different temperature dependencies of the two contributions the effective anisotropy may change its sign and thus the direction of the magnetization as a function of temperature may change. Contrary to the well-known reorientation transition caused by competing surface and bulk anisotropy contributions the reorientation that we discuss is also found in film systems with a uniform lattice anisotropy. The results of our theoretical model study may have experimental relevance for film systems with positive lattice anisotropy, as e.g. thin iron films grown on copper.Comment: 7 pages, 4 figures, accepted for publication in EPJ

Non-collapsing renormalized QRPA with proton-neutron pairing for neutrinoless double beta decay

Using the renormalized quasiparticle random phase approximation (RQRPA), we calculate the light neutrino mass mediated mode of neutrinoless double beta decay of Ge76, Mo100, Te128 and Te130. Our results indicate that the simple quasiboson approximation is not good enough to study the neutrinoless double beta decay, because its solutions collapse for physical values of g_pp. We find that extension of the Hilbert space and inclusion of the Pauli Principle in the QRPA with proton-neutron pairing, allows us to extend our calculations beyond the point of collapse, for physical values of the nuclear force strength. As a consequence one might be able to extract more accurate values on the effective neutrino mass by using the best available experimental limits on the half-life of neutrinoless double beta decay.Comment: 15 pages, RevTex, 2 Postscript figures, to appear in Phys. Lett.

Self Consistent and Renormalized particle-particle RPA in a Schematic Model

The dynamical effects of ground state correlations for excitation energies and transition strengths near the superfluid phase transition are studied in the soluble two level pairing model, in the context of the particle-particle self consistent Random Phase Approximation (SCRPA). Exact results are well reproduced across the transition region, beyond the collapse of the standard particle-particle Random Phase Approximation. The effects of two-body correlation in the SCRPA are displayed explicitly.Comment: 11 pages, revtex, 3ps figures, to appear in Phys. Rev.

A large Hilbert space QRPA and RQRPA calculation of neutrinoless double beta decay

A large Hilbert space is used for the calculation of the nuclear matrix elements governing the light neutrino mass mediated mode of neutrinoless double beta decay of Ge76, Mo100, Cd116, Te128 and Xe136 within the proton-neutron quasiparticle random phase approximation (pn-QRPA) and the renormalized QRPA with proton-neutron pairing (full-RQRPA) methods. We have found that the nuclear matrix elements obtained with the standard pn-QRPA for several nuclear transitions are extremely sensitive to the renormalization of the particle-particle component of the residual interaction of the nuclear hamiltonian. Therefore the standard pn-QRPA does not guarantee the necessary accuracy to allow us to extract a reliable limit on the effective neutrino mass. This behaviour, already known from the calculation of the two-neutrino double beta decay matrix elements, manifests itself in the neutrinoless double-beta decay but only if a large model space is used. The full-RQRPA, which takes into account proton-neutron pairing and considers the Pauli principle in an approximate way, offers a stable solution in the physically acceptable region of the particle-particle strength. In this way more accurate values on the effective neutrino mass have been deduced from the experimental lower limits of the half-lifes of neutrinoless double beta decay.Comment: 19 pages, RevTex, 1 Postscript figur

Zn(O, S) layers for chalcoyprite solar cells sputtered from a single target

A simplified Cu(In, Ga)(S, Se)2/Zn(O, S)/ZnO:Al stack for chalcopyrite thin- film solar cells is proposed. In this stack the Zn(O, S) layer combines the roles of the traditional CdS buffer and undoped ZnO layers. It will be shown that Zn(O, S) films can be sputtered in argon atmosphere from a single mixed target without substrate heating. The photovoltaic performance of the simplified stack matches that of the conventional approach. Replacing the ZnO target with a ZnO/ZnS target may therefore be sufficient to omit the CdS buffer layer and avoid the associated complexity, safety and recycling issues, and to lower production cost

Correlation and surface effects in Vanadium Oxides

Recent photoemission experiments have shown strong surface modifications in the spectra from vanadium oxides as (V,Cr)_2O_3 or (Sr,Ca)VO_3. The effective mass is enhanced at the surface and the coherent part of the surface spectrum is narrowed as compared to the bulk. The quasiparticle weight is more sensitive at the surface than in the bulk against bandwidth variations. We investigate these effects theoretically considering the single-band Hubbard model for a film geometry. A simplified dynamical mean-field scheme is used to calculate the main features of the interacting layer-dependent spectral function. It turns out that the experimentally confirmed effects are inherent properties of a system of strongly correlated electrons. The reduction of the weight and the variance of the coherent part of the surface spectrum can be traced back to the reduced surface coordination number. Surface correlation effects can be strongly amplified by changes of the hopping integrals at the surface.Comment: to appear in PRB; 8 pages, 6 figure

Neutrinoless double beta decay within Self-consistent Renormalized Quasiparticle Random Phase Approximation and inclusion of induced nucleon currents

The first, to our knowledge, calculation of neutrinoless double beta decay ($0\nu\beta\beta$-decay) matrix elements within the self-consistent renormalised Quasiparticle Random Phase Approximation (SRQRPA) is presented. The contribution from the momentum-dependent induced nucleon currents to $0\nu\beta\beta$-decay amplitude is taken into account. A detailed nuclear structure study includes the discussion of the sensitivity of the obtained SRQRPA results for $0\nu\beta\beta$-decay of $^{76}$Ge to the parameters of nuclear Hamiltonian, two-nucleon short-range correlations and the truncation of the model space. A comparision with the standard and renormalized QRPA is presented. We have found a considerable reduction of the SRQRPA nuclear matrix elements, resulting in less stringent limits for the effective neutrino mass.Comment: 13 pages, 3 figures, 1 tabl

The Pauli principle, QRPA and the two-neutrino double beta decay

We examine the violation of the Pauli exclusion principle in the Quasiparticle Random Phase Approximation (QRPA) calculation of the two-neutrino double beta decay matrix elements, which has its origin in the quasi-boson approximation. For that purpose we propose a new renormalized QRPA with proton-neutron pairing method (full-RQRPA) for nuclear structure studies, which includes ground state correlation beyond the QRPA. This is achieved by using of renormalized quasi-boson approximation, in which the Pauli exclusion principle is taken into account more carefully. The full-RQRPA has been applied to two-neutrino double beta decay of $^{76}Ge$, $^{82}Se$, $^{128}Te$ and $^{130}Te$. The nuclear matrix elements have been found significantly less sensitive to the increasing strength of particle-particle interaction in the physically interesting region in comparison with QRPA results. The strong differences between the results of both methods indicate that the Pauli exclusion principle plays an important role in the evaluation of the double beta decay. The inclusion of the Pauli principle removes the difficulties with the strong dependence on the particle-particle strength $g_{pp}$ in the QRPA on the two-neutrino double beta decay.Comment: Accepted for publication in Nucl. Phys. A, 22 pages, including 5 figures, LaTeX (using REVTeX and epsfig-style

MFI Type Zeolite Aggregates with Nanosized Particles via a Combination of Spray Drying and Steam-Assisted Crystallization (SAC) Techniques

This article belongs to the Special Issue Catalysis on Zeolites and Zeolite-Like Materials II

Fully-Renormalized QRPA fulfills Ikeda sum rule exactly

The renormalized quasiparticle-RPA is reformulated for even-even nuclei using restrictions imposed by the commutativity of the phonon creation operator with the total particle number operator. This new version, Fully-Renormalized QRPA (FR-QRPA), is free from the spurious low-energy solutions. Analytical proof is given that the Ikeda sum rule is fullfiled within the FR-QRPA.Comment: 9 page