386 research outputs found

    Coherent control of a surface structural phase transition

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    Active optical control over matter is desirable in many scientific disciplines, with prominent examples in all-optical magnetic switching1,2, light-induced metastable or exotic phases of solids3,4,5,6,7,8 and the coherent control of chemical reactions9,10. Typically, these approaches dynamically steer a system towards states or reaction products far from equilibrium. In solids, metal-to-insulator transitions are an important target for optical manipulation, offering ultrafast changes of the electronic4 and lattice11,12,13,14,15,16 properties. The impact of coherences on the efficiencies and thresholds of such transitions, however, remains a largely open subject. Here, we demonstrate coherent control over a metal–insulator structural phase transition in a quasi-one-dimensional solid-state surface system. A femtosecond double-pulse excitation scheme17,18,19,20 is used to switch the system from the insulating to a metastable metallic state, and the corresponding structural changes are monitored by ultrafast low-energy electron diffraction21,22. To govern the transition, we harness vibrational coherence in key structural modes connecting both phases, and observe delay-dependent oscillations in the double-pulse switching efficiency. Mode-selective coherent control of solids and surfaces could open new routes to switching chemical and physical functionalities, enabled by metastable and non-equilibrium states

    Levodopa‐induced dyskinesia are mediated by cortical gamma oscillations in experimental Parkinsonism

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    Background Levodopa is the most efficacious drug in the symptomatic therapy of motor symptoms in Parkinson's disease (PD); however, long‐term treatment is often complicated by troublesome levodopa‐induced dyskinesia (LID). Recent evidence suggests that LID might be related to increased cortical gamma oscillations. Objective The objective of this study was to test the hypothesis that cortical high‐gamma network activity relates to LID in the 6‐hydroxydopamine model and to identify new biomarkers for adaptive deep brain stimulation (DBS) therapy in PD. Methods We recorded and analyzed primary motor cortex (M1) electrocorticogram data and motor behavior in freely moving 6‐OHDA lesioned rats before and during a daily treatment with levodopa for 3 weeks. The results were correlated with the abnormal involuntary movement score (AIMS) and used for generalized linear modeling (GLM). Results Levodopa reverted motor impairment, suppressed beta activity, and, with repeated administration, led to a progressive enhancement of LID. Concurrently, we observed a highly significant stepwise amplitude increase in finely tuned gamma (FTG) activity and gamma centroid frequency. Whereas AIMS and FTG reached their maximum after the 4th injection and remained on a stable plateau thereafter, the centroid frequency of the FTG power continued to increase thereafter. Among the analyzed gamma activity parameters, the fraction of longest gamma bursts showed the strongest correlation with AIMS. Using a GLM, it was possible to accurately predict AIMS from cortical recordings. Conclusions FTG activity is tightly linked to LID and should be studied as a biomarker for adaptive DBS

    Microphysical properties and radiative impact of an intense biomass burning aerosol event measured over Ny-Ålesund, Spitsbergen in July 2015

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    In this work, an evaluation of an intense biomass burning event observed over Ny-Ålesund (Spitsbergen, European Arctic) in July 2015 is presented. Data from the multi-wavelengths Raman-lidar KARL, a sun photometer and radiosonde measurements are used to derive some microphysical properties of the biomass burning aerosol as size distribution, refractive index and single scattering albedo at different relative humidities. Predominantly particles in the accumulation mode have been found with a bi-modal distribution and dominance of the smaller mode. Above 80% relative humidity, hygroscopic growth in terms of an increase of particle diameter and a slight decrease of the index of refraction (real and imaginary part) has been found. Values of the single scattering albedo around 0.9 both at 355 nm and 532 nm indicate some absorption by the aerosol. Values of the lidar ratio are around 26 sr for 355 nm and around 50 sr for 532 nm, almost independent of the relative humidity. Further, data from the photometer and surface radiation values from the local baseline surface radiation network (BSRN) have been applied to derive the radiative impact of the biomass burning event purely from observational data by comparison with a clear background day. We found a strong cooling for the visible radiation and a slight warming in the infra-red. The net aerosol forcing, derived by comparison with a clear background day purely from observational data, obtained a value of –95 W/m2 per unit AOD500

    Novel Weak Decays in Doubly Strange Systems

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    The strangeness-changing (ΔS=1\Delta S = 1) weak baryon-baryon interaction is studied through the nonmesonic weak decay of double-Λ\Lambda hypernuclei. Besides the usual nucleon-induced decay ΛN→NN\Lambda N \to N N we discuss novel hyperon-induced decay modes ΛΛ→ΛN\Lambda \Lambda \to \Lambda N and ΛΛ→ΣN\Lambda \Lambda \to \Sigma N. These reactions provide unique access to the exotic ΛΛ\Lambda \LambdaK and ΛΣ\Lambda \SigmaK vertices which place new constraints on Chiral Pertubation Theory (χ\chiPT) in the weak SU(3) sector. Within a meson-exchange framework, we use the pseudoscalar π,η,K\pi,\eta,K octet for the long-range part while parametrizing the short-range part through the vector mesons ρ,ω,K∗\rho, \omega, K^*. Realistic baryon-baryon forces for the S=0,−1S=0,-1 and -2 sectors account for the strong interaction in the initial and final states. For ΛΛ6^6_{\Lambda \Lambda}He the new hyperon-induced decay modes account for up to 4% of the total nonmesonic decay rate. Predictions are made for all possible nonmesonic decay modes.Comment: 19 pages, 2 ps figures, 9 table

    Meson-Meson Scattering in the Quark Model: Spin Dependence and Exotic Channels

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    We apply a quark interchange model to spin-dependent and exotic meson-meson scattering. The model includes the complete set of standard quark model forces, including OGE spin-orbit and tensor and scalar confinement spin-orbit. Scattering amplitudes derived assuming SHO and Coulomb plus linear plus hyperfine meson wavefunctions are compared. In I=2 pi pi we find approximate agreement with the S-wave phase shift from threshold to 1.5 GeV, where we predict an extremum that is supported by the data. Near threshold we find rapid energy dependence that may reconcile theoretical estimates of small scattering lengths with experimental indications of larger ones based on extrapolation of measurements at moderate kpi^2. In PsV scattering we find that the quark-quark L*S and T forces map into L*S and T meson-meson interactions, and the P-wave L*S force is large. Finally we consider scattering in J^PC-exotic channels, and note that some of the Deck effect mechanisms suggested as possible nonresonant origins of the pi_1(1400) signal are not viable in this model.Comment: 51 pages, 10 figures, uses epsf.sty epsfig.st

    What is the structure of the Roper resonance?

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    We investigate the structure of the nucleon resonance N^*(1440) (Roper) within a coupled-channel meson exchange model for pion-nucleon scattering. The coupling to pipiN states is realized effectively by the coupling to the sigmaN, piDelta and rhoN channels. The interaction within and between these channels is derived from an effective Lagrangian based on a chirally symmetric Lagrangian, which is supplemented by well known terms for the coupling of the Delta isobar, the omega meson and the 'sigma', which is the name given here to the strong correlation of two pions in the scalar-isoscalar channel. In this model the Roper resonance can be described by meson-baryon dynamics alone; no genuine N^*(1440) (3 quark) resonance is needed in order to fit piN phase shifts and inelasticities.Comment: 55 pages, 14 figure

    Retrieval of optical and microphysical properties of transported Saharan dust over Athens and Granada based on multi-wavelength Raman lidar measurements: Study of the mixing processes

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    In this paper we extract the aerosol microphysical properties for a collection of mineral dust cases measured by multi-wavelength depolarization Raman lidar systems located at the National Technical University of Athens (NTUA, Athens, Greece) and the Andalusian Institute for Earth System Research (IISTA-CEAMA, Granada, Spain). The lidar-based retrievals were carried out with the Spheroidal Inversion eXperiments software tool (SphInX) developed at the University of Potsdam (Germany). The software uses regularized inversion of a two-dimensional enhancement of the Mie model based on the spheroid-particle approximation with the aspect ratio determining the particle shape. The selection of the cases was based on the transport time from the source regions to the measuring sites. The aerosol optical depth as measured by AERONET ranged from 0.27 to 0.54 (at 500 nm) depending on the intensity of each event. Our analysis showed the hourly mean particle linear depolarization ratio and particle lidar ratio values at 532 nm ranging from 11 to 34% and from 42 to 79 sr respectively, depending on the mixing status, the corresponding air mass pathways and their transport time. Cases with shorter transport time showed good agreement in terms of the optical and SphInX-retrieved microphysical properties between Athens and Granada providing a complex refractive index value equal to 1.4 + 0.004i. On the other hand, the results for cases with higher transport time deviated from the aforementioned ones as well as from each other, providing, in particular, an imaginary part of the refractive index ranging from 0.002 to 0.005. Reconstructions of two-dimensional shape-size distributions for each selected layer showed that the dominant effective particle shape was prolate with diverse spherical contributions. The retrieved volume concentrations reflect overall the intensity of the episodes.Spanish Ministry of Sciences, Innovation and Universities through project CGL2016-81092,Spanish Ministry of Education, Culture and Sports through grant FPU14/0368

    Solid-state NMR evidence for inequivalent GvpA subunits in gas vesicles

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    Gas vesicles are organelles that provide buoyancy to the aquatic microorganisms that harbor them. The gas vesicle shell consists almost exclusively of the hydrophobic 70-residue gas vesicle protein A, arranged in an ordered array. Solid-state NMR spectra of intact collapsed gas vesicles from the cyanobacterium Anabaena flos-aquae show duplication of certain gas vesicle protein A resonances, indicating that specific sites experience at least two different local environments. Interpretation of these results in terms of an asymmetric dimer repeat unit can reconcile otherwise conflicting features of the primary, secondary, tertiary, and quaternary structures of the gas vesicle protein. In particular, the asymmetric dimer can explain how the hydrogen bonds in the ÎČ-sheet portion of the molecule can be oriented optimally for strength while promoting stabilizing aromatic and electrostatic side-chain interactions among highly conserved residues and creating a large hydrophobic surface suitable for preventing water condensation inside the vesicle.National Institutes of Health (U.S.) (Grant EB002175)National Institutes of Health (U.S.) (Grant EB003151)National Institutes of Health (U.S.) (Grant EB002026

    Central radio galaxies in galaxy clusters: Joint surveys by eROSITA and ASKAP

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    The extended ROentgen Survey with an Imaging Telescope Array (eROSITA) telescope onboard the Spectrum-Roentgen-Gamma (SRG) mission has finished the first eROSITA All-Sky Survey (eRASS:1), and detected 104^4 galaxy clusters in the western Galactic hemisphere. In the radio band, the Australian Square Kilometre Array Pathfinder (ASKAP) telescope finished its pilot 1 phase of the project 'Evolutionary Map of the Universe' (EMU) with 220.000 sources in a 270 deg2^2 field overlapping with eRASS:1. These two surveys are used to study radio-mode Active Galactic Nuclei (AGN) in clusters. In order to understand the efficiency of radio-mode feedback at the centers of galaxy clusters, we relate the radio properties of brightest cluster galaxies (BCG) to the X-ray properties of the host clusters. We identify the central radio sources in eRASS:1 clusters or calculate corresponding upper limits on the radio luminosity. Then, we derive relations between the X-ray properties of the clusters and the radio properties of the corresponding central radio source. We also apply a mid-infrared color criterion using WISE colors to identify AGN. In total we investigate a sample of 75 clusters. We find a statistically significant correlation between the X-ray luminosity of the cluster and the 944 MHz radio luminosity of the corresponding central radio galaxy. There is also a positive trend between the radio power and the largest linear size (LLS) of the radio source. The density and the LLS do not show any correlation. We find that in high luminosity clusters with L_X > 104310^{43} erg s−1^{-1} the kinetic luminosity of the radio jets is not longer correlated with the X-ray luminosity and discuss various reasons. We find an anti-correlation between the central cooling time t_cool and the radio luminosity L_R indicating a need for more powerful AGN in clusters with short central cooling times.Comment: 16 pages, 12 figures, accepted for publication in A&
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