Selective excitation of plasmons superlocalized at sharp perturbations of metal nanoparticles

Sharp metal corners and tips support plasmons localized on the scale of the curvature radius -- superlocalized plasmons. We analyze plasmonic properties of nanoparticles with small and sharp corner- and tip-shaped surface perturbations in terms of hybridization of the superlocalized plasmons, which frequencies are determined by the perturbations shape, and the ordinary plasmons localized on the whole particle. When the frequency of a superlocalized plasmon gets close to that of the ordinary plasmon, their strong hybridization occurs and facilitates excitation of an optical hot-spot near the corresponding perturbation apex. The particle is then employed as a nano-antenna that selectively couples the free-space light to the nanoscale vicinity of the apex providing precise local light enhancement by several orders of magnitude

Asymmetry in shape causing absolute negative mobility

We propose a simple classical concept of nanodevices working in an absolute negative mobility (ANM) regime: The minimal spatial asymmetry required for ANM to occur is embedded in the geometry of the transported particle, rather than in the channel design. This allows for a tremendous simplification of device engineering, thus paving the way towards practical implementations of ANM. Operating conditions and performance of our model device are investigated, both numerically and analytically.Comment: 6 pages; accepted for publication in PR

Probing Pauli Blocking Factors in Quantum Pumps with Broken Time-Reversal Symmetry

A recently demonstrated quantum electron pump is discussed within the framework of photon-assisted tunneling. Due to lack of time-reversal symmetry, different results are obtained for the pump current depending on whether or not final-state Pauli blocking factors are used when describing the tunneling process. Whilst in both cases the current depends quadratically on the driving amplitude for moderate pumping, a marked difference is predicted for the temperature dependence. With blocking factors the pump current decreases roughly linearly with temperature until k_B T ~ \hbar\omega is reached, whereas without them it is unaffected by temperature, indicating that the entire Fermi sea participates in the electronic transport.Comment: 4 pages in RevTex4 (beta4), 6 figures; status: to appear in PR

Highly tunable low-threshold optical parametric oscillation in radially poled whispering gallery resonators

Whispering gallery resonators (WGR's), based on total internal reflection, possess high quality factors in a broad spectral range. Thus, nonlinear optical processes in such cavities are ideally suited for the generation of broadband or tunable electromagnetic radiation. Experimentally and theoretically, we investigate the tunability of optical parametric oscillation in a radially structured WGR made of lithium niobate. With a 1.04 /mum pump wave, the signal and idler waves are tuned from 1.78 to 2.5 \mum - including the point of degeneracy - by varying the temperature between 20 and 62 {\deg}C. A weak off-centering of the radial domain structure extends considerably the tuning capabilities. The oscillation threshold lies in the mW-power range.Comment: 4 pages, 5 figure

Direct current driven by ac electric field in quantum wells

It is shown that the excitation of charge carriers by ac electric field with zero average driving leads to a direct electric current in quantum well structures. The current emerges for both linear and circular polarization of the ac electric field and depends on the field polarization and frequency. We present a micoscopic model and an analytical theory of such a nonlinear electron transport in quantum wells with structure inversion asymmetry. In such systems, dc current is induced by ac electric field which has both the in-plane and out-of-plane components. The ac field polarized in the interface plane gives rise to a direct current if the quantum well is subjected to an in-plane static magnetic field.Comment: 6 pages, 3 figure

First principles calculations of the Shift Current Bulk Photovoltaic Effect in Ferroelectrics

We calculate the bulk photovoltaic response of the ferroelectrics BaTiO$_3$ and PbTiO$_3$ from first principles by applying "shift current" theory to the electronic structure from density functional theory. The first principles results for BaTiO$_3$ reproduce eperimental photocurrent direction and magnitude as a function of light frequency, as well as the dependence of current on light polarization, demonstrating that shift current is the dominant mechanism of the bulk photovoltaic effect in BaTiO$_3$. Additionally, we analyze the relationship between response and material properties in detail. The photocurrent does not depend simply or strongly on the magnitude of material polarization, as has been previously assumed; instead, electronic states with delocalized, covalent bonding that is highly asymmetric along the current direction are required for strong shift current enhancements. The complexity of the response dependence on both external and material parameters suggests applications not only in solar energy conversion, but to photocatalysis and sensor and switch type devices as well.Comment: First submitted April 2011, submitted PRL July 201

Maxwell-Drude-Bloch dissipative few-cycle optical solitons

We study the propagation of few-cycle pulses in two-component medium consisting of nonlinear amplifying and absorbing two-level centers embedded into a linear and conductive host material. First we present a linear theory of propagation of short pulses in a purely conductive material, and demonstrate the diffusive behavior for the evolution of the low-frequency components of the magnetic field in the case of relatively strong conductivity. Then, numerical simulations carried out in the frame of the full nonlinear theory involving the Maxwell-Drude-Bloch model reveal the stable creation and propagation of few-cycle dissipative solitons under excitation by incident femtosecond optical pulses of relatively high energies. The broadband losses that are introduced by the medium conductivity represent the main stabilization mechanism for the dissipative few-cycle solitons.Comment: 38 pages, 10 figures. submitted to Physical Review

Signature of the electron-electron interaction in the magnetic field dependence of nonlinear I-V characteristics in mesoscopic systems

We show that the nonlinear I-V characteristics of mesoscopic samples with metallic conductivity should contain parts which are linear in the magnetic field and quadratic in the electric field. These contributions to the current are entirely due to the electron-electron interaction and consequently they are proportional to the electron-electron interaction constant. We also note that both the amplitude and the sign of the current exhibit random oscillations as a function of temperature

Investigation of photorefractive subharmonics in the absence of wavemixing

Using a new optical configuration free from the influence of photorefractive optical nonlinearity, we investigate the main characteristics of the spatial subharmonic K/2 excited in a Bi12SiO20 crystal by a light-intensity pattern with wave vector K and frequency O. It is shown that in a large region of intensity and applied electric field the optimum value O of the frequency corresponds to the conditions of parametric excitation of the weakly damped eigenmodes of the medium: the space-charge waves. The threshold and above-threshold characteristics of the subharmonic regime are in good agreement with the theory

Asymmetry of Nonlinear Transport and Electron Interactions in Quantum Dots

The symmetry properties of transport beyond the linear regime in chaotic quantum dots are investigated experimentally. A component of differential conductance that is antisymmetric in both applied source-drain bias V and magnetic field B, absent in linear transport, is found to exhibit mesoscopic fluctuations around a zero average. Typical values of this component allow a measurement of the electron interaction strength.Comment: related papers at http://marcuslab.harvard.ed