14 research outputs found
Tropospheric ozone over Siberia in spring 2010: remote influences and stratospheric intrusion
Pan-Eurasian Experiment (PEEX) Program : An Overview of the First 5 Years in Operation and Future Prospects
The Pan-Eurasian Experiment (PEEX) program was initiated as a bottom-up approach by the researchers coming from Finland and Russia in October 2012. The PEEX China kick off meeting was held in November 2013. During its five years in operation, the program has established a governance structure and delivered a science plan for the Northern Eurasian region. PEEX has also introduced a concept design for a modelling platform and ground-based in situ observation systems for detecting land-atmosphere and ocean-atmosphere interactions. Today, PEEX has an extensive researcher’s network representing research communities coming from the Nordic countries, Russia and China. PEEX is currently carrying out its research activities on a project basis, but is looking for more coordinated funding bases, especially in Russia and in China. The near-future challenge in implementing the PEEX research agenda is to achieve a successful integration and identification of the methodological approaches of the socio-economic research to environmental sciences. Here we give insight into these issues and provide an overview on the main tasks for the upcoming years.The Pan-Eurasian Experiment (PEEX) program was initiated as a bottom-up approach by the researchers coming from Finland and Russia in October 2012. The PEEX China kick off meeting was held in November 2013. During its five years in operation, the program has established a governance structure and delivered a science plan for the Northern Eurasian region. PEEX has also introduced a concept design for a modelling platform and ground-based in situ observation systems for detecting land-atmosphere and ocean-atmosphere interactions. Today, PEEX has an extensive researcher’s network representing research communities coming from the Nordic countries, Russia and China. PEEX is currently carrying out its research activities on a project basis, but is looking for more coordinated funding bases, especially in Russia and in China. The near-future challenge in implementing the PEEX research agenda is to achieve a successful integration and identification of the methodological approaches of the socio-economic research to environmental sciences. Here we give insight into these issues and provide an overview on the main tasks for the upcoming years.The Pan-Eurasian Experiment (PEEX) program was initiated as a bottom-up approach by the researchers coming from Finland and Russia in October 2012. The PEEX China kick off meeting was held in November 2013. During its five years in operation, the program has established a governance structure and delivered a science plan for the Northern Eurasian region. PEEX has also introduced a concept design for a modelling platform and ground-based in situ observation systems for detecting land-atmosphere and ocean-atmosphere interactions. Today, PEEX has an extensive researcher’s network representing research communities coming from the Nordic countries, Russia and China. PEEX is currently carrying out its research activities on a project basis, but is looking for more coordinated funding bases, especially in Russia and in China. The near-future challenge in implementing the PEEX research agenda is to achieve a successful integration and identification of the methodological approaches of the socio-economic research to environmental sciences. Here we give insight into these issues and provide an overview on the main tasks for the upcoming years.Peer reviewe
Overview: Recent advances in the understanding of the northern Eurasian environments and of the urban air quality in China – a Pan-Eurasian Experiment (PEEX) programme perspective
The Pan-Eurasian Experiment (PEEX) Science Plan, released in 2015, addressed a need for a holistic system understanding and outlined the most urgent research needs for the rapidly changing Arctic-boreal region. Air quality in China, together with the long-range transport of atmospheric pollutants, was also indicated as one of the most crucial topics of the research agenda. These two geographical regions, the northern Eurasian Arctic-boreal region and China, especially the megacities in China, were identified as a "PEEX region". It is also important to recognize that the PEEX geographical region is an area where science-based policy actions would have significant impacts on the global climate. This paper summarizes results obtained during the last 5 years in the northern Eurasian region, together with recent observations of the air quality in the urban environments in China, in the context of the PEEX programme. The main regions of interest are the Russian Arctic, northern Eurasian boreal forests (Siberia) and peatlands, and the megacities in China. We frame our analysis against research themes introduced in the PEEX Science Plan in 2015. We summarize recent progress towards an enhanced holistic understanding of the land-atmosphere-ocean systems feedbacks. We conclude that although the scientific knowledge in these regions has increased, the new results are in many cases insufficient, and there are still gaps in our understanding of large-scale climate-Earth surface interactions and feedbacks. This arises from limitations in research infrastructures, especially the lack of coordinated, continuous and comprehensive in situ observations of the study region as well as integrative data analyses, hindering a comprehensive system analysis. The fast-changing environment and ecosystem changes driven by climate change, socio-economic activities like the China Silk Road Initiative, and the global trends like urbanization further complicate such analyses. We recognize new topics with an increasing importance in the near future, especially "the enhancing biological sequestration capacity of greenhouse gases into forests and soils to mitigate climate change" and the "socio-economic development to tackle air quality issues".Peer reviewe
Profiling of Saharan dust and biomass-burning smoke with multiwavelength polarization Raman lidar at Cape Verde
Published under the terms of the Creative Commons Attribution-Noncommercial 3.0 Unported LicenseExtensive lidar measurements of Saharan dust and biomass-burning smoke were performed with one airborne and three ground-based instruments in the framework of the second part of the SAharan Mineral dUst experiMent (SAMUM-2a) during January and February of 2008 at Cape Verde. Further lidar observations with one system only were conducted during May and June of 2008 (SAMUM-2b). The active measurements were supported by Sun photometer observations. During winter, layers of mineral dust from the Sahara and biomass-burning smoke from southern West Africa pass Cape Verde on their way to South America while pure dust layers cross the Atlantic on their way to the Caribbean during summer. The mean 500-nm aerosol optical thickness (AOT) observed during SAMUM-2a was 0.35 +/- 0.18. SAMUM-2a observations showed transport of pure dust within the lowermost 1.5 km of the atmospheric column. In the height range from 1.5 to 5.0 km, mixed dust/smoke layers with mean lidar ratios of 67 +/- 14 sr at 355 and 532 nm, respectively, prevailed. Within these layers, wavelength-independent linear particle depolarization ratios of 0.12-0.18 at 355, 532, and 710 nm indicate a large contribution (30-70%) of mineral dust to the measured optical properties. Angstrom exponents for backscatter and extinction of around 0.7 support this finding. Mean extinction coefficients in the height range between 2 and 4 km were 66 +/- 6 Mm(-1) at 355 nm and 48 +/- 5 Mm(-1) at 532 nm. Comparisons with airborne high-spectral-resolution lidar observations show good agreement within the elevated layers. 3-5 km deep dust layers where observed during SAMUM-2b. These layers showed optical properties similar to the ones of SAMUM-1 in Morocco with a mean 500-nm AOT of 0.4 +/- 0.2. Dust extinction coefficients were about 80 +/- 6 Mm(-1) at 355 and 532 nm. Dust lidar ratios were 53 +/- 10 sr at 355 and 532 nm, respectively. Dust depolarization ratios showed an increase with wavelength from 0.31 +/- 0.10 at 532 nm to 0.37 +/- 0.07 at 710 nm.Peer reviewe
Tropospheric ozone over Siberia in spring 2010: remote influences and stratospheric intrusion
International audienceWe have identified and characterised different factors influencing the tropospheric ozone over Siberia during spring 2010. This was done by analysing in-situ measurements of ozone, carbon dioxide, carbon monoxide, and methane mixing ratios measured by continuous analysers during an intensive airborne measurement campaign of the YAK-AEROSIB project, carried out between 15 and 18 April 2010. The analysis and interpretation of the observations, spanning 3000 km and stretching from 800 to 6700 m above ground level, were enhanced using the Lagrangian model FLEXPART to simulate backward air mass transport. The analysis of trace gas variability and simulated origin of air masses showed that plumes coming from east and west of the west Siberian plain and from north-eastern China related to biomass burning and anthropogenic activity had enhanced ozone mixing ratios during transport. In one case, low ozone mixing ratios were observed over a large region in the upper troposphere above 5500 m. The air mass was transported from the marine boundary layer over the Norwegian Sea where O3 background concentrations are low in the spring. The transport was coherent over thousands of kilometres, with no significant mixing with mid-upper troposphere air masses rich in O3. Finally, the stratospheric source of ozone to the troposphere was observed directly in a well-defined stratospheric intrusion. Analysis of this event suggests an input of 2.56±0.29×107 kg of ozone associated with a regional downward flux of 9.75±2.9×1010 molecules cm−2 s−1, smaller than hemispheric climatology
Assessing the near surface sensitivity of SCIAMACHY atmospheric CO2 retrieved using (FSI) WFM-DOAS
Satellite observations of atmospheric CO2 offer the potential to identify regional carbon surface sources and sinks and to investigate carbon cycle processes. The extent to which satellite measurements are useful however, depends on the near surface sensitivity of the chosen sensor. In this paper, the capability of the SCIAMACHY instrument on board ENVISAT, to observe lower tropospheric and surface CO2 variability is examined. To achieve this, atmospheric CO2 retrieved from SCIAMACHY near infrared (NIR) spectral measurements, using the Full Spectral Initiation (FSI) WFMDOAS algorithm, is compared to in-situ aircraft observations over Siberia and additionally to tower and surface CO2 data over Mongolia, Europe and North America.
Preliminary validation of daily averaged SCIAMACHY/FSI CO2 against ground based Fourier Transform Spectrometer (FTS) column measurements made at Park Falls, reveal a negative bias of about −2.0% for collocated
measurements within +/-1.0 of the site. However, at this spatial threshold SCIAMACHY can only capture the variability of the FTS observations at monthly timescales. To observe day to day variability of the FTS observations, the collocation limits must be increased. Furthermore, comparisons to in-situ CO2 observations demonstrate that
SCIAMACHY is capable of observing a seasonal signal that is representative of lower tropospheric variability on (at least) monthly timescales. Out of seventeen time series comparisons, eleven have correlation coefficients of 0.7 or more, and have similar seasonal cycle amplitudes. Additional
evidence of the near surface sensitivity of SCIAMACHY, is provided through the significant correlation of FSI derived
CO2 with MODIS vegetation indices at over twenty selected locations in the United States. The SCIAMACHY/MODIS comparison reveals that at many of the sites, the amount of CO2 variability is coincident with the amount of vegetation activity. The presented analysis suggests that SCIAMACHY
has the potential to detect CO2 variability within the lowermost troposphere arising from the activity of the terrestrial biosphere
Tropospheric ozone over Siberia in spring 2010: remote influences and stratospheric intrusion
EARLINET climatology (2000-2010)
A European Aerosol Research Lidar Network to Establish an Aerosol ClimatologyAerosols affect life on earth in several ways. They play an important role in the climate system; the effect of aerosols on the global climate system is one of the major uncertainties of present climate predictions. They play a major role in atmospheric chemistry and hence affect the concentrations of other potentially harmful atmospheric constituents, e.g. ozone. They are an important controlling factor for the radiation budget, in particular in the UV-B part of the spectrum. At ground level, they can be harmful, even toxic, to man, animals, and plants. Because of these adverse effects that aerosols can have on human life, it is necessary to achieve an advanced understanding of the processes that generate, redistribute, and remove aerosols in the atmosphere.A quantitative dataset describing the aerosol vertical, horizontal, and temporal distribution, including its variability on a continental scale, is necessary. The dataset is used to validate and improve models that predict the future state of the atmosphere and its dependence on different scenarios describing economic development, including those actions taken to preserve the quality of the environment. The EARLINET data set is the most comprehensive compilation of data available for this purpose.This project description is taken from: http://www.earlinet.org/index.php?id=earlinet_homepageSummary: EARLINET climatological lidar observations are performed on a regularschedule of one daytime measurement per week around noon (on Monday), when theboundary layer is usually well developed, and two night-time measurements per week(on Monday and Thursday), with low background light, in order to perform Ramanextinction measurements. This regular schedule for observations minimizes the biasin the dataset possibly related to specific measurement conditions. The resultingdataset is used to obtain unbiased data for climatological studies.This dataset contains profiles of aerosol extinction, backscatter and lidar ratio.Several aerosol extinction/backscatter datasets can be present for the sameclimatological measurement in order to provide profiles either with a better temporalresolution or with an extended height range by using a larger temporal average.This is by far the largest dataset on the aerosol vertical distribution, and it isthe only one which is collected systematically and is covering a whol
EARLINET observations related to volcanic eruptions (2000-2010)
A European Aerosol Research Lidar Network to Establish an Aerosol ClimatologyAerosols affect life on earth in several ways. They play an important role in the climate system; the effect of aerosols on the global climate system is one of the major uncertainties of present climate predictions. They play a major role in atmospheric chemistry and hence affect the concentrations of other potentially harmful atmospheric constituents, e.g. ozone. They are an important controlling factor for the radiation budget, in particular in the UV-B part of the spectrum. At ground level, they can be harmful, even toxic, to man, animals, and plants. Because of these adverse effects that aerosols can have on human life, it is necessary to achieve an advanced understanding of the processes that generate, redistribute, and remove aerosols in the atmosphere.A quantitative dataset describing the aerosol vertical, horizontal, and temporal distribution, including its variability on a continental scale, is necessary. The dataset is used to validate and improve models that predict the future state of the atmosphere and its dependence on different scenarios describing economic development, including those actions taken to preserve the quality of the environment. The EARLINET data set is the most comprehensive compilation of data available for this purpose.This project description is taken from: http://www.earlinet.org/index.php?id=earlinet_homepageSummary: Aerosols originating from volcanic emissions have an impact on the climate: sulfate and ash particles from volcanic emissions reflect solar radiation, act as cloud condensation and ice nuclei, and modify the radiative properties and lifetime of clouds, and therefore influence the precipitation cycle. These volcanic particles can also have an impact on environmental conditions and could be very dangerous for aircraft in flight. In addition to the routine measurements, further EARLINET observations are devoted to monitor volcano eruptions. The EARLINET volcanic dataset includes extended observations related to two different volcanoes in Europe Mt. Etna (2001 and 2002 eruptions), and the Eyjafjallajokull volcano in Iceland (April - May 2010 eruption). This dataset includes also recent events of volcanic eruptions in the North Pacific region (2008-2010) that emitted sulfuric acid droplets into the upper troposphere - lower stratosphere (UTLS) height region of the northern hemisphere. The EARLINET volcanic observations in the UTLS are complemented by the long-term stratospheric aerosol observations collected in the Stratosphere category