741 research outputs found
Letter-speech sound learning in children with dyslexia:From behavioral research to clinical practice
Letter-speech sound learning in children with dyslexia:From behavioral research to clinical practice
Charge transport through a single molecule of trans-1-bis-diazofluorene [60]fullerene
Fullerenes have attracted interest for their possible applications in various
electronic, biological, and optoelectronic devices. However, for efficient use
in such devices, a suitable anchoring group has to be employed that forms
well-defined and stable contacts with the electrodes. In this work, we propose
a novel fullerene tetramalonate derivate functionalized with trans-1
4,5-diazafluorene anchoring groups. The conductance of single-molecule
junctions, investigated in two different setups with the mechanically
controlled break junction technique, reveals the formation of molecular
junctions at three conductance levels. We attribute the conductance peaks to
three binding modes of the anchoring groups to the gold electrodes. Density
functional theory calculations confirm the existence of multiple binding
configurations and calculated transmission functions are consistent with
experimentally determined conductance values.Comment: 22 pages, 6 figure
ALLSMOG: an APEX Low-redshift Legacy Survey for MOlecular Gas. I - molecular gas scaling relations, and the effect of the CO/H2 conversion factor
We present ALLSMOG, the APEX Low-redshift Legacy Survey for MOlecular Gas.
ALLSMOG is a survey designed to observe the CO(2-1) emission line with the APEX
telescope, in a sample of local galaxies (0.01 < z < 0.03), with stellar masses
in the range 8.5 < log(M*/Msun) < 10. This paper is a data release and initial
analysis of the first two semesters of observations, consisting of 42 galaxies
observed in CO(2-1). By combining these new CO(2-1) emission line data with
archival HI data and SDSS optical spectroscopy, we compile a sample of low-mass
galaxies with well defined molecular gas masses, atomic gas masses, and
gas-phase metallicities. We explore scaling relations of gas fraction and gas
consumption timescale, and test the extent to which our findings are dependent
on a varying CO/H2 conversion factor. We find an increase in the H2/HI mass
ratio with stellar mass which closely matches semi-analytic predictions. We
find a mean molecular gas fraction for ALLSMOG galaxies of MH2/M* = (0.09 -
0.13), which decreases with stellar mass. We measure a mean molecular gas
consumption timescale for ALLSMOG galaxies of 0.4 - 0.7 Gyr. We also confirm
the non-universality of the molecular gas consumption timescale, which varies
(with stellar mass) from ~100 Myr to ~2 Gyr. Importantly, we find that the
trends in the H2/HI mass ratio, gas fraction, and the non-universal molecular
gas consumption timescale are all robust to a range of recent
metallicity-dependent CO/H2 conversion factors.Comment: 25 pages, 15 figures. Accepted for publication in MNRA
A Survey of Atomic Carbon [C I] in High-redshift Main-Sequence Galaxies
We present the first results of an ALMA survey of the lower fine structure
line of atomic carbon [C I](^3P_1\,-\,^{3}P_0) in far infrared-selected
galaxies on the main sequence at in the COSMOS field. We compare our
sample with a comprehensive compilation of data available in the literature for
local and high-redshift starbursting systems and quasars. We show that the [C
I]() luminosity correlates on global scales with the
infrared luminosity similarly to low- CO transitions. We report
a systematic variation of L'_{\rm [C\,I]^3P_1\,-\, ^3P_0}/ as a
function of the galaxy type, with the ratio being larger for main-sequence
galaxies than for starbursts and sub-millimeter galaxies at fixed .
The L'_{\rm [C\,I]^3P_1\,-\, ^3P_0}/ and / mass ratios are similar for main-sequence galaxies and for
local and high-redshift starbursts within a 0.2 dex intrinsic scatter,
suggesting that [C I] is a good tracer of molecular gas mass as CO and dust. We
derive a fraction of %
of the total carbon mass in the atomic neutral phase. Moreover, we estimate the
neutral atomic carbon abundance, the fundamental ingredient to calibrate [C I]
as a gas tracer, by comparing L'_{\rm [C\,I]^3P_1\,-\, ^3P_0} and available
gas masses from CO lines and dust emission. We find lower [C I] abundances in
main-sequence galaxies than in starbursting systems and sub-millimeter
galaxies, as a consequence of the canonical and gas-to-dust
conversion factors. This argues against the application to different galaxy
populations of a universal standard [C I] abundance derived from highly biased
samples.Comment: 14 pages + Appendix. Accepted for publication in ApJ. All the data
tables in Appendix will be also released in electronic forma
ALMA observations of atomic carbon in z~4 dusty star-forming galaxies
We present ALMA [CI]() (rest frequency 492 GHz) observations for a
sample of 13 strongly-lensed dusty star-forming galaxies originally discovered
at 1.4mm in a blank-field survey by the South Pole Telescope. We compare these
new data with available [CI] observations from the literature, allowing a study
of the ISM properties of extreme dusty star-forming galaxies spanning
a redshift range . Using the [CI] line as a tracer of the molecular
ISM, we find a mean molecular gas mass for SPT-DSFGs of
M. This is in tension with gas masses derived via low- CO
and dust masses; bringing the estimates into accordance requires either (a) an
elevated CO-to-H conversion factor for our sample of and a gas-to-dust ratio , or (b) an high carbon abundance . Using observations of a range of additional atomic
and molecular lines (including [CI], [CII], and multiple transitions of CO), we
use a modern Photodissociation Region code (3D-PDR) to assess the physical
conditions (including the density, UV radiation field strength, and gas
temperature) within the ISM of the DSFGs in our sample. We find that the ISM
within our DSFGs is characterised by dense gas permeated by strong UV fields.
We note that previous efforts to characterise PDR regions in DSFGs may have
significantly underestimated the density of the ISM. Combined, our analysis
suggests that the ISM of extreme dusty starbursts at high redshift consists of
dense, carbon-rich gas not directly comparable to the ISM of starbursts in the
local Universe.Comment: 21 pages, 12 figures. Accepted for publication in MNRA
Quest for COSMOS Submillimeter Galaxy Counterparts using CARMA and VLA: Identifying Three High-redshift Starburst Galaxies
We report on interferometric observations at 1.3 mm at 2"-3" resolution using the Combined Array for Research in Millimeter-wave Astronomy. We identify multi-wavelength counterparts of three submillimeter galaxies (SMGs; F_(1mm) > 5.5 mJy) in the COSMOS field, initially detected with MAMBO and AzTEC bolometers at low, ~10"-30", resolution. All three sourcesâAzTEC/C1, Cosbo-3, and Cosbo-8âare identified to coincide with positions of 20 cm radio sources. Cosbo-3, however, is not associated with the most likely radio counterpart, closest to the MAMBO source position, but with that farther away from it. This illustrates the need for intermediate-resolution (~2") mm-observations to identify the correct counterparts of single-dish-detected SMGs. All of our three sources become prominent only at NIR wavelengths, and their mm-to-radio flux based redshifts suggest that they lie at redshifts z âł 2. As a proof of concept, we show that photometric redshifts can be well determined for SMGs, and we find photometric redshifts of 5.6 Âą 1.2, 1.9^(+0.9)_(â0.5), and ~4 for AzTEC/C1, Cosbo-3, and Cosbo-8, respectively. Using these we infer that these galaxies have radio-based star formation rates of âł 1000 M_â yr^(â1) and IR luminosities of ~10^(13) L_â consistent with properties of high-redshift SMGs. In summary, our sources reflect a variety of SMG properties in terms of redshift and clustering, consistent with the framework that SMGs are progenitors of z ~ 2 and today's passive galaxies
Unraveling biogeochemical phosphorus dynamics in hyperarid Marsâanalogue soils using stable oxygen isotopes in phosphate
With annual precipitation less than 20 mm and extreme UV intensity, the Atacama Desert in northern Chile has long been utilized as an analogue for recent Mars. In these hyperarid environments, water and biomass are extremely limited, and thus, it becomes difficult to generate a full picture of biogeochemical phosphateâwater dynamics. To address this problem, we sampled soils from five Atacama study sites and conducted three main analysesâstable oxygen isotopes in phosphate, enzyme pathway predictions, and cell culture experiments. We found that high sedimentation rates decrease the relative size of the organic phosphorus pool, which appears to hinder extremophiles. Phosphoenzyme and pathway prediction analyses imply that inorganic pyrophosphatase is the most likely catalytic agent to cycle P in these environments, and this process will rapidly overtake other P utilization strategies. In these soils, the biogenic δ18O signatures of the soil phosphate (δ18OPO4) can slowly overprint lithogenic δ18OPO4 values over a timescale of tens to hundreds of millions of years when annual precipitation is more than 10 mm. The δ18OPO4 of calciumâbound phosphate minerals seems to preserve the δ18O signature of the water used for biogeochemical P cycling, pointing toward sporadic rainfall and gypsum hydration water as key moisture sources. Where precipitation is less than 2 mm, biological cycling is restricted and bedrock δ18OPO4 values are preserved. This study demonstrates the utility of δ18OPO4 values as indicative of biogeochemical cycling and hydrodynamics in an extremely dry Marsâanalogue environment
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