Pushing indium phosphide quantum dot emission deeper into the near infrared

Cadmium-free near infrared (NIR) emitting quantum dots (QDs) have significant potential for multiplexed tissue-depth imaging applications in the first optical tissue window (i.e., 650 – 900 nm). Indium phosphide (InP) chemistry provides one of the more promising cadmium-free options for biomedical imaging, but the full tunability of this material has not yet been achieved. Specifically, InP QD emission has been tuned from 480 – 730 nm in previous literature reports, but examples of samples emitting from 730 nm to the InP bulk bandgap limit of 925 nm are lacking. We hypothesize that by generating inverted structures comprising ZnSe/InP/ZnS in a core/shell/shell heterostructure, optical emission from the InP shell can be tuned by changing the InP shell thickness, including pushing deeper into the NIR than current InP QDs. Colloidal synthesis methods including hot injection precipitation of the ZnSe core and a modified successive ion layer adsorption and reaction (SILAR) method for stepwise shell deposition were used to promote growth of core/shell/shell materials with varying thicknesses of the InP shell. By controlling the number of injections of indium and phosphorous precursor material, the emission peak was tuned from 515 nm to 845 nm (2.41 – 1.47 eV) with consistent full width half maximum (FWHM) values of the emission peak ~0.32 eV. To confer water solubility, the nanoparticles were encapsulated in PEGylated phospholipid micelles, and multiplexing of NIR-emitting InP QDs was demonstrated using an IVIS imaging system. These materials show potential for multiplexed imaging of targeted QD contrast agents in the first optical tissue window

Letter from A.M. Alexander to James B. Finley

A.M. Alexander informs Finley of the death of Brother Isaac C. Hunter, elder from the Marietta District. Hunter died on June 28th after a lingering illness which began as a cold and developed into pleurisy and consumption. The letter contains a description of Rev. Hunter\u27s illness and death, which is to be incorporated into the memoir to be read at Conference. Brother Hunter was beloved in this region by all who knew him. Abstract Number - 205https://digitalcommons.owu.edu/finley-letters/1204/thumbnail.jp

Complete Models of Axisymmetric Sunspots: Magnetoconvection with Coronal Heating

We present detailed results of numerical experiments into the nature of complete sunspots. The models remain highly idealized but include fully nonlinear compressible magnetoconvection in an axisymmetric layer that drives energy into an overlying, low-B plasma. We survey a range of parameters in which the resulting magnetoconvection displays the formation of pore- and sunspot-like behavior and assess the coronal signatures resulting from the energy generated by the magnetoconvection. The coronal heating is assumed to be a result of the dissipation by an unspecified means of a fraction of the Poynting flux entering the corona. The expected signatures in the EUV and soft X-ray bandpasses of the Transition Region and Coronal Explorer and Yohkoh/SXT, respectively, are examined. This ad hoc coupling of the corona to the subphotospheric region results in a dynamical behavior that is consistent with recent observational results. This agreement demonstrates that even simple coupled modeling can lead to diagnostics for investigations of both subphotospheric sunspot structures and coronal heating mechanisms

Neutrino spin evolution in presence of general external fields

The derivation of the quasiclassical Lorentz invariant neutrino spin evolution equation taking into account general types of neutrino non-derivative interactions with external fields is presented. We discuss the constraints on the characteristics of matter and neutrino under which this quasiclassical approach is valid. The application of the obtained equation for the case of the Standard Model neutrino interactions with moving and polarized background matter is considered.Comment: The form of the article has been sufficiently improve

Exotic composites: the decay of deficit angles in global-local monopoles

We study static, spherically symmetric, composite global-local monopoles with a direct interaction term between the two sectors in the regime where the interaction potential is large. At some critical coupling the global defect disappears and with it the deficit angle of the space-time. We find new solutions which represent local monopoles in an Anti-de-Sitter spacetime. In another parameter range the magnetic monopole, or even both, disappear. The decay of the magnetic monopole is accompanied by a dynamical transition from the higgsed phase to the gauge-symmetric phase. We comment on the applications to cosmology, topological inflation and braneworlds.Comment: 17 pages, 11 figures; Minor corrections, matches published versio

New Travelling Wave Solutions of Two Nonlinear Physical Models by Using a Modified Tanh-Coth Method

In this work, a modified tanh – coth method is used to derive travelling wave solutions for (2 + 1)-dimensional Zakharov-Kuznetsov (ZK) equation and (3 + 1)-dimensional Burgers equation. A new variable is used to solve these equations and established new travelling wave solutions. </jats:p

Directed and Elliptic Flow in Pb+Pb collisions at 40 and 158 AGeV

Directed and elliptic flow are reported for charged pions and protons as a function of transverse momentum, rapidity, and centrality in 40 and 158 AGeV Pb + Pb collisions. The standard method of correlating particles with an event plane is used. The directed flow of protons is small and shows little variation near to midrapidity, but rises fast towards projectile rapidity in the 40 AGeV data. For most peripheral collisions the flat region becomes negative resulting in $v_1$ changing sign three times. Elliptic flow doesn't seem to change very much from 40 AGeV to 158 AGeV. The difference is smaller than anticipated from the overall energy dependence from AGS to RHIC.Comment: Presented at 16th International Conference on Ultrarelativistic Nucleus-Nucelus Collisions, Quark Matter 2002 (QM 2002), Nantes, France, 18-24 Jul 2002, 4 pages, 3 figure

More on core instabilities of magnetic monopoles

In this paper we present new results on the core instability of the 't Hooft Polyakov monopoles we reported on before. This instability, where the spherical core decays in a toroidal one, typically occurs in models in which charge conjugation is gauged. In this paper we also discuss a third conceivable configuration denoted as ``split core'', which brings us to some details of the numerical methods we employed. We argue that a core instability of 't Hooft Polyakov type monopoles is quite a generic feature of models with charged Higgs particles.Comment: Latex, 15 pages, 6 figures; published versio

Cycling chaos: its creation, persistence and loss of stability in a model of nonlinear magnetoconvection

We examine a model system where attractors may consist of a heteroclinic cycle between chaotic sets; this ‘cycling chaos’ manifests itself as trajectories that spend increasingly long periods lingering near chaotic invariant sets interspersed with short transitions between neighbourhoods of these sets. Such behaviour is robust to perturbations that preserve the symmetry of the system; we examine bifurcations of this state. We discuss a scenario where an attracting cycling chaotic state is created at a blowout bifurcation of a chaotic attractor in an invariant subspace. This differs from the standard scenario for the blowout bifurcation in that in our case, the blowout is neither subcritical nor supercritical. The robust cycling chaotic state can be followed to a point where it loses stability at a resonance bifurcation and creates a series of large period attractors. The model we consider is a ninth-order truncated ordinary differential equation (ODE) model of three-dimensional incompressible convection in a plane layer of conducting fluid subjected to a vertical magnetic field and a vertical temperature gradient. Symmetries of the model lead to the existence of invariant subspaces for the dynamics; in particular there are invariant subspaces that correspond to regimes of two-dimensional flows, with variation in the vertical but only one of the two horizontal directions. Stable two-dimensional chaotic flow can go unstable to three-dimensional flow via the cross-roll instability. We show how the bifurcations mentioned above can be located by examination of various transverse Liapunov exponents. We also consider a reduction of the ODE to a map and demonstrate that the same behaviour can be found in the corresponding map. This allows us to describe and predict a number of observed transitions in these models. The dynamics we describe is new but nonetheless robust, and so should occur in other applications