129 research outputs found

    Detailed Measurements of Characteristic Profiles of Magnetic Diffuse Scattering in ErB2_2C2_2

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    Detailed neutron diffraction measurements on a single crystalline ErB2_2C2_2 were performed. We observed magnetic diffuse scattering which consists of three components just above the transition temperatures, which is also observed in characteristic antiferroquadrupolar ordering compounds HoB2_2C2_2 and TbB2_2C2_2. The result of this experiments indicates that the antiferroquadrupolar interaction is not dominantly important as a origin of the magnetic diffuse scattering.Comment: 5 pages, 5 figures, submitted to J. Phys. Soc. Jp

    A Coalescent Sampler Successfully Detects Biologically Meaningful Population Structure Overlooked by F‐Statistics

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    Assessing the geographic structure of populations has relied heavily on Sewell Wright\u27s F‐statistics and their numerous analogues for many decades. However, it is well appreciated that, due to their nonlinear relationship with gene flow, F statistics frequently fail to reject the null model of panmixia in species with relatively high levels of gene flow and large population sizes. Coalescent genealogy samplers instead allow a model‐selection approach to the characterization of population structure, thereby providing the opportunity for stronger inference. Here, we validate the use of coalescent samplers in a high gene flow context using simulations of a stepping‐stone model. In an example case study, we then re‐analyze genetic datasets from 41 marine species sampled from throughout the Hawaiian archipelago using coalescent model selection. Due to the archipelago\u27s linear nature, it is expected that most species will conform to some sort of stepping‐stone model (leading to an expected pattern of isolation by distance), but F‐statistics have only supported this inference in ~10% of these datasets. Our simulation analysis shows that a coalescent sampler can make a correct inference of stepping‐stone gene flow in nearly 100% of cases where gene flow is ≤100 migrants per generation (equivalent to FST = 0.002), while F‐statistics had mixed results. Our re‐analysis of empirical datasets found that nearly 70% of datasets with an unambiguous result fit a stepping‐stone model with varying population sizes and rates of gene flow, although 37% of datasets yielded ambiguous results. Together, our results demonstrate that coalescent samplers hold great promise for detecting weak but meaningful population structure, and defining appropriate management units

    Neutron scattering study of magnetic ordering and excitations in the ternary rare-earth diborocarbide Ce^{11}B_2C_2

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    Neutron scattering experiments have been performed on the ternary rare-earth diborocarbide Ce11^{11}B2_2C2_2. The powder diffraction experiment confirms formation of a long-range magnetic order at TN=7.3T_{\rm N} = 7.3 K, where a sinusoidally modulated structure is realized with the modulation vector q=[0.167(3),0.167(3),0.114(3)]{\bm q} = [0.167(3), 0.167(3), 0.114(3)]. Inelastic excitation spectra in the paramagnetic phase comprise significantly broad quasielastic and inelastic peaks centered at ω0,8\hbar \omega \approx 0, 8 and 65 meV. Crystalline-electric-field (CEF) analysis satisfactorily reproduces the observed spectra, confirming their CEF origin. The broadness of the quasielastic peak indicates strong spin fluctuations due to coupling between localized 4f4f spins and conduction electrons in the paramagnetic phase. A prominent feature is suppression of the quasielastic fluctuations, and concomitant growth of a sharp inelastic peak in a low energy region below TNT_{\rm N}. This suggests dissociation of the conduction and localized 4f4f electrons on ordering, and contrasts the presently observed incommensurate phase with spin-density-wave order frequently seen in heavy fermion compounds, such as Ce(Ru1x_{1-x}Lax_x)2_2Si2_2.Comment: accepted for publication in Phys. Rev.

    Magnetic phase diagram of antiferroquadrupole ordering in HoB2C2

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    The magnetic phase diagram for antiferro-quadrupole (AFQ) ordering in tetragonal HoB2_2C2_2 has been investigated by measurements of elastic constants C11C_{11}, C44C_{44} and C66C_{66} in fields along the basal xx-yy plane as well as the principal [001]-axis. The hybrid magnet (GAMA) in Tsukuba Magnetic Laboratory was employed for high field measurements up to 30 T. The AFQ phase is no longer observed above 26.3 T along the principal [001] axis in contrast to the relatively small critical field of 3.9 T in fields applied along the basal [110] axis. The quadrupolar intersite interaction of OxyO_{xy} and/or O22O_2^2 is consistent with the anisotropy in the magnetic phase diagram of the AFQ phase in HoB2_2C2_2.Comment: Phys. Rev. B. (2005) in press. approx 8 pages, 10 figure

    Electronic structure and magnetic properties of RMnX (R= Mg, Ca, Sr, Ba, Y; X= Si, Ge) studied by KKR method

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    Electronic structure calculations, using the charge and spin self-consistent Korringa- Kohn-Rostoker (KKR) method, have been performed for several RRMnXX compounds (RR = Mg, Ca, Sr, Ba, Y; XX = Si, Ge) of the CeFeSi-type structure. The origin of their magnetic properties has been investigated emphasizing the role of the Mn sublattice. The significant influence of the Mn-Mn and Mn-XX interatomic distances on the Mn magnetic moment value is delineated from our computations, supporting many neutron diffraction data. We show that the marked change of μMn\mu_{Mn} with the Mn-Mn and Mn-XX distances resulted from a redistribution between spin-up and spin-down dd-Mn DOS rather than from different fillings of the Mn 3dd-shell. Bearing in mind that the neutron diffraction data reported for the RRMnXX compounds are rather scattered, the KKR computations of μMn\mu_{Mn} are in fair agreement with the experimental values. Comparing density of states near EFE_{F} obtained in different magnetic orderings, one can notice that the entitled RRMnXX systems seem to 'adapt' their magnetic structures to minimize the DOS in the vicinity of the Fermi level. Noteworthy, the SrMnGe antiferromagnet exhibits a pseudo-gap behaviour at EFE_{F}, suggesting anomalous electron transport properties. In addition, the F-AF transition occurring in the disordered La1x_{1-x}Yx_{x}MnSi alloy for the 0.8<x<10.8<x<1 range is well supported by the DOS features of La0.2_{0.2}Y0.8_{0.8}MnSi. In contrast to the investigated RRMnXX compounds, YFeSi was found to be non-magnetic, which is in excellent agreement with the experimental data.Comment: 10 pages + 14 figures, to appear in Eur. Phys. Jour.

    Inclusion of soy oil levels on the acceptability and digestibility of diets for equines

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    The effects of different quantities and types of dietary fats on the digestibility of feeds for equines are complicated and not fully understood. The present work was undertaken to evaluate the acceptability and digestibility of dry matter (DM), organic matter (OM), crude protein (CP), ether extract (EE), and neutral and acid detergent fibers (NDF, ADF), upon increasing inclusion levels of soybean oil (SBO) (5, 10, 15 and 20%) in the concentrate portion of diets composed of equal parts of grass hay and concentrate. The total collection of feces method was used with four yearling colts. The experimental design was 4 x 4 Latin square and the data were analyzed by simple polynomic regression. The SBO showed good acceptability as all of the concentrates offered were consumed. Level of SBO inclusion in the concentrate affected (P &lt; 0.05) OM digestibility, there being and initial increase up to a maximum of 66.7% at the 10.74% inclusion level and decreasing digestibility thereafter; in analogous fashion the digestibilities of NDF and ADF increased to maxima of 51.8% and 45.5% at SBO inclusion levels of 9.5% and 10.56%, respectively. The lower digestibilities at higher inclusion levels were presumably due to inhibitory effects of added lipid on the cecal cellulolytic microflora. Level of SBO inclusion did not significantly affect the digestibilities of DM, CP and EE, although DM digestion followed a quadratic tendency (P = 0.08) very similar to that observed for OM

    A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water

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    We present the laboratory results of immersion freezing efficiencies of cellulose particles at supercooled temperature (T) conditions. Three types of chemically homogeneous cellulose samples are used as surrogates that represent supermicron and submicron ice-nucleating plant structural polymers. These samples include microcrystalline cellulose (MCC), fibrous cellulose (FC) and nanocrystalline cellulose (NCC). Our immersion freezing dataset includes data from various ice nucleation measurement techniques available at 17 different institutions, including nine dry dispersion and 11 aqueous suspension techniques. With a total of 20 methods, we performed systematic accuracy and precision analysis of measurements from all 20 measurement techniques by evaluating T-binned (1 ∘C) data over a wide T range (−36 ∘C <T<−4 ∘C). Specifically, we intercompared the geometric surface area-based ice nucleation active surface site (INAS) density data derived from our measurements as a function of T, ns,geo(T). Additionally, we also compared the ns,geo(T) values and the freezing spectral slope parameter (Δlog(ns,geo)/ΔT) from our measurements to previous literature results. Results show all three cellulose materials are reasonably ice active. The freezing efficiencies of NCC samples agree reasonably well, whereas the diversity for the other two samples spans ≈ 10 ∘C. Despite given uncertainties within each instrument technique, the overall trend of the ns,geo(T) spectrum traced by the T-binned average of measurements suggests that predominantly supermicron-sized cellulose particles (MCC and FC) generally act as more efficient ice-nucleating particles (INPs) than NCC with about 1 order of magnitude higher ns,geo(T)
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