Theory of light-induced current in molecular-tunneling junctions excited with intense shaped pulses

A theory for light-induced current by strong optical pulses in molecular-tunneling junctions is described. We consider a molecular bridge represented by its highest occupied and lowest unoccupied levels, HOMO and LUMO, respectively. We take into account two types of couplings between the molecule and the metal leads: electron transfer that gives rise to net current in the biased junction and energy transfer between the molecule and electron-hole excitations in the leads. Using a Markovian approximation, we derive a closed system of equations for the expectation values of the relevant variables: populations and molecular polarization that are binary, and exciton populations that are tetradic in the annihilation and creation operators for electrons in the molecular states. We have proposed an optical control method using chirped pulses for enhancing charge transfer in unbiased junctions where the bridging molecule is characterized by a strong charge-transfer transition. An approximate analytical solution of the resulting dynamical equation is supported by a full numerical solution. When energy transfer between the molecule and electron-hole excitations in the leads is absent, the optical control problem for inducing charge transfer with linearly chirped pulse can be reduced to the Landau-Zener transition to a decaying level. When chirp is fast with respect to the rate of the electron transfer, the Landau theory is recovered. The proposed control mechanism is potentially useful for developing novel opto-electronic single-electron devices with optical gating based on molecular nanojunctions.Comment: 14 pages, 7 figures; submitted to PR

Shot Noise in Mesoscopic Transport Through Localised States

We show that shot noise can be used for studies of hopping and resonant tunnelling between localised electron states. In hopping via several states, shot noise is seen to be suppressed compared with its classical Poisson value $S_I=2eI$ ($I$ is the average current) and the suppression depends on the distribution of the barriers between the localised states. In resonant tunnelling through a single impurity an enhancement of shot noise is observed. It has been established, both theoretically and experimentally, that a considerable increase of noise occurs due to Coulomb interaction between two resonant tunnelling channels.Comment: 7 pages, 5 figures; Proceedings of the 10th Conference on Hopping and Related Phenomena (Trieste 2003); requires Wiley style files (included

Statistics of Transmission Eigenvalues for a Disordered Quantum Point Contact

We study the distribution of transmission eigenvalues of a quantum point contact with nearby impurities. In the semi-classical case (the chemical potential lies at the conductance plateau) we find that the transmission properties of this system are obtained from the ensemble of Gaussian random reflection matrices. The distribution only depends on the number of open transport channels and the average reflection eigenvalue and crosses over from the Poissonian for one open channel to the form predicted by the circuit theory in the limit of large number of open channels.Comment: 8 pages, 3 figure

Enhanced shot noise in resonant tunnelling via interacting localised states

In a variety of mesoscopic systems shot noise is seen to be suppressed in comparison with its Poisson value. In this work we observe a considerable enhancement of shot noise in the case of resonant tunnelling via localised states. We present a model of correlated transport through two localised states which provides both a qualitative and quantitative description of this effect.Comment: 4 pages, 4 figure

Loss Distribution Generation in Credit Portfolio Modeling

In the current paper we analyze several methods for generation of loss distribution for credit portfolios. Loss distributions play an important role in pricing of credit derivatives and in credit portfolio optimization. A loss distribution is a function of the number of entities in the portfolio, their credit ratings, the notional amount and recovery of each entity, default probabilities, loss given defaults, and the correlation/dependence structure between entities incorporated in the portfolio. Direct generation of loss distribution may require Monte Carlo simulation which is time consuming and is not effective when applied for credit portfolio optimization. To overcome computational complexity a number of approaches were undertaken based on assumptions imposed on the input parameters, goals of loss distributions generation, and the accepted level of tolerance and computational errors

Driven coherent oscillations of a single electron spin in a quantum dot

The ability to control the quantum state of a single electron spin in a quantum dot is at the heart of recent developments towards a scalable spin-based quantum computer. In combination with the recently demonstrated exchange gate between two neighbouring spins, driven coherent single spin rotations would permit universal quantum operations. Here, we report the experimental realization of single electron spin rotations in a double quantum dot. First, we apply a continuous-wave oscillating magnetic field, generated on-chip, and observe electron spin resonance in spin-dependent transport measurements through the two dots. Next, we coherently control the quantum state of the electron spin by applying short bursts of the oscillating magnetic field and observe about eight oscillations of the spin state (so-called Rabi oscillations) during a microsecond burst. These results demonstrate the feasibility of operating single-electron spins in a quantum dot as quantum bits.Comment: Total 25 pages. 11 pages main text, 5 figures, 9 pages supplementary materia

Macroturbulence fluctuations of air impurities concentration and refractive index in the bottom layer

Spatial variability of impurity concentration and refraction index in the bottom layer for the turbulence scales interval 16 km is investigated in the work. This work based on the data of continues monitoring of urban air parameters. Structural functions of impurity concentrations and that of calculated refraction index were plotted to measuring. Approximation of the obtained structural functions by power-behaved dependence showed that in the researched range the exponent has the value (0,4-0,6) and decreases with increasing of the distance. Experimentally obtained results correspond well with theory of large-scale turbulence. The separate research has shown, that in scales range 1-3.5 kms exponent located in the range [0.6-1], and in the range 3,5-6 kms - [0.01-0.22]. Thus the impurities with the horizontal scales of 1-6 km in the bottom layer are located in the boundary of buoyancy range and of the large-scale turbulence range

First Measurement of the Transverse Spin Asymmetries of the Deuteron in Semi-Inclusive Deep Inelastic Scattering

First measurements of the Collins and Sivers asymmetries of charged hadrons produced in deep-inelastic scattering of muons on a transversely polarized 6-LiD target are presented. The data were taken in 2002 with the COMPASS spectrometer using the muon beam of the CERN SPS at 160 GeV/c. The Collins asymmetry turns out to be compatible with zero, as does the measured Sivers asymmetry within the present statistical errors.Comment: 6 pages, 2 figure

The COMPASS Experiment at CERN

The COMPASS experiment makes use of the CERN SPS high-intensitymuon and hadron beams for the investigation of the nucleon spin structure and the spectroscopy of hadrons. One or more outgoing particles are detected in coincidence with the incoming muon or hadron. A large polarized target inside a superconducting solenoid is used for the measurements with the muon beam. Outgoing particles are detected by a two-stage, large angle and large momentum range spectrometer. The setup is built using several types of tracking detectors, according to the expected incident rate, required space resolution and the solid angle to be covered. Particle identification is achieved using a RICH counter and both hadron and electromagnetic calorimeters. The setup has been successfully operated from 2002 onwards using a muon beam. Data with a hadron beam were also collected in 2004. This article describes the main features and performances of the spectrometer in 2004; a short summary of the 2006 upgrade is also given.Comment: 84 papes, 74 figure