Full characterization of vibrational coherence in a porphyrin chromophore by two-dimensional electronic spectroscopy

In this work we present experimental and calculated two-dimensional electronic spectra for a 5,15-bisalkynyl porphyrin chromophore. The lowest energy electronic Qy transition couples mainly to a single 380 cm–1 vibrational mode. The two-dimensional electronic spectra reveal diagonal and cross peaks which oscillate as a function of population time. We analyze both the amplitude and phase distribution of this main vibronic transition as a function of excitation and detection frequencies. Even though Feynman diagrams provide a good indication of where the amplitude of the oscillating components are located in the excitation-detection plane, other factors also affect this distribution. Specifically, the oscillation corresponding to each Feynman diagram is expected to have a phase that is a function of excitation and detection frequencies. Therefore, the overall phase of the experimentally observed oscillation will reflect this phase dependence. Another consequence is that the overall oscillation amplitude can show interference patterns resulting from overlapping contributions from neighboring Feynman diagrams. These observations are consistently reproduced through simulations based on third order perturbation theory coupled to a spectral density described by a Brownian oscillator model

Field Effect Transistors for Terahertz Detection: Physics and First Imaging Applications

Resonant frequencies of the two-dimensional plasma in FETs increase with the reduction of the channel dimensions and can reach the THz range for sub-micron gate lengths. Nonlinear properties of the electron plasma in the transistor channel can be used for the detection and mixing of THz frequencies. At cryogenic temperatures resonant and gate voltage tunable detection related to plasma waves resonances, is observed. At room temperature, when plasma oscillations are overdamped, the FET can operate as an efficient broadband THz detector. We present the main theoretical and experimental results on THz detection by FETs in the context of their possible application for THz imaging.Comment: 22 pages, 12 figures, review pape

On the development of QPOs in Bondi-Hoyle accretion flows

The numerical investigation of Bondi-Hoyle accretion onto a moving black hole has a long history, both in Newtonian and in general-relativistic physics. By performing new two-dimensional and general-relativistic simulations onto a rotating black hole, we point out a novel feature, namely, that quasi-periodic oscillations (QPOs) are naturally produced in the shock cone that develops in the downstream part of the flow. Because the shock cone in the downstream part of the flow acts as a cavity trapping pressure perturbations, modes with frequencies in the integer ratios 2:1 and 3:1 are easily produced. The frequencies of these modes depend on the black-hole spin and on the properties of the flow, and scale linearly with the inverse of the black-hole mass. Our results may be relevant for explaining the detection of QPOs in Sagittarius A*, once such detection is confirmed by further observations. Finally, we report on the development of the flip-flop instability, which can affect the shock cone under suitable conditions; such an instability has been discussed before in Newtonian simulations but was never found in a relativistic regime.Comment: 11 pages, 7 figure

Plasma mechanisms of resonant terahertz detection in two-dimensional electron channel with split gates

We analyze the operation of a resonant detector of terahertz (THz) radiation based on a two-dimensional electron gas (2DEG) channel with split gates. The side gates are used for the excitation of plasma oscillations by incoming THz radiation and control of the resonant plasma frequencies. The central gate provides the potential barrier separating the source and drain portions of the 2DEG channel. Two possible mechanisms of the detection are considered: (1) modulation of the ac potential drop across the barrier and (2) heating of the 2DEG due to the resonant plasma-assisted absorption of THz radiation followed by an increase in thermionic dc current through the barrier. Using the device model we calculate the frequency and temperature dependences of the detector responsivity associated with both dynamic and heating (bolometric) mechanisms. It is shown that the dynamic mechanisms dominates at elevated temperatures, whereas the heating mechanism provides larger contribution at low temperatures, T=35-40 K.Comment: 7 pages, 4 figure

The propagating speed of relic gravitational waves and their refractive index during inflation

If the refractive index of the tensor modes increases during a conventional inflationary stage of expansion the relic graviton spectrum is tilted towards high frequencies. Two apparently diverse parametrizations of this effect are shown to be related by a rescaling of the four-dimensional metric through a conformal factor that involves the refractive index itself. Non-monotonic spectra with a maximum in the MHz region correspond to a limited variation of the refractive index terminating well before the end of inflation. After exploring a general approach encompassing the ones proposed so far, we estimate the required sensitivity for the direct detection of the predicted gravitational radiation and demonstrate that the allowed regions of the parameter space are within reach for some of the planned detectors operating either in the audio band (like Ligo/Virgo and Kagra) or in the mHz band (like Lisa, Bbo and Decigo).Comment: 32 pages, 12 figures; corrected typos and comments adde

Cavity-enhanced optical Hall effect in two-dimensional free charge carrier gases detected at terahertz frequencies

The effect of a tunable, externally coupled Fabry-P\'{e}rot cavity to resonantly enhance the optical Hall effect signatures at terahertz frequencies produced by a traditional Drude-like two-dimensional electron gas is shown and discussed in this communication. As a result, the detection of optical Hall effect signatures at conveniently obtainable magnetic fields, for example by neodymium permanent magnets, is demonstrated. An AlInN/GaN-based high electron mobility transistor structure grown on a sapphire substrate is used for the experiment. The optical Hall effect signatures and their dispersions, which are governed by the frequency and the reflectance minima and maxima of the externally coupled Fabry-P\'{e}rot cavity, are presented and discussed. Tuning the externally coupled Fabry-P\'{e}rot cavity strongly modifies the optical Hall effect signatures, which provides a new degree of freedom for optical Hall effect experiments in addition to frequency, angle of incidence and magnetic field direction and strength

Simultaneous projection and detection system of four different frequencies for microwave imaging reflectometry in Large Helical Device

A simultaneous projection/detection system of four different frequencies for microwave imaging reflectometry (MIR) was developed for three-dimensional observation of electron density fluctuations in the Large Helical Device (LHD). The microwave with four frequency components at 60.410, 61.808, 63.008, and 64.610 GHz is projected in a continuous-wave mode to illuminate the target LHD plasma. A two-dimensional horn-antenna mixer array (2D HMA) receives the reflected wave from the plasma as well as the wave from the local oscillator operating at 55.800 GHz. The first intermediate frequency (IF) signals at 4.610, 6.008, 7.208, and 8.810 GHz were confirmed to be obtained by downconversion of these microwaves using the 2D HMA. Each of these first IF components is filtered from each other and downconverted again for the superheterodyne detection. It was confirmed that both the amplitudes and the phases of the detected signals reflect the fluctuations in LHD plasmas