An on-line test strategy and analysis for a 1T1R crossbar memory

© 2017 IEEE. Personal use of this material is permitted. Permission from IEEE must be obtained for all other uses, in any current or future media, including reprinting/republishing this material for advertising or promotional purposes,creating new collective works, for resale or redistribution to servers or lists, or reuse of any copyrighted component of this work in other works.Memristors are emerging devices known by their nonvolability, compatibility with CMOS processes and high density in circuits density in circuits mostly owing to the crossbar nanoarchitecture. One of their most notable applications is in the memory system field. Despite their promising characteristics and the advancements in this emerging technology, variability and reliability are still principal issues for memristors. For these reasons, exploring techniques that check the integrity of circuits is of primary importance. Therefore, this paper proposes a method to perform an on-line test capable to detect a single failure inside the memory crossbar array.Peer ReviewedPostprint (author's final draft

Reliability-aware circuit design to mitigate impact of device defects and variability in emerging memristor-based applications

In the last decades, semiconductor industry has fostered a fast downscale in technology, propelling the large scale integration of CMOS-based systems. The benefits in miniaturization are numerous, highlighting faster switching frequency, lower voltage supply and higher device density. However, this aggressive scaling trend it has not been without challenges, such as leakage currents, yield reduction or the increase in the overall system power dissipation. New materials, changes in the device structures and new architectures are key to keep the miniaturization trend. It is foreseen that 2D integration will eventually come to an insurmountable physical and economic limit, in which new strategic directions are required, such as the development of new device structures, 3D architectures or heterogeneous systems that takes advantage of the best of different technologies, both the ones already consolidated as well as emergent ones that provide performance and efficiency improvements in applications. In this context, memristor arises as one of several candidates in the race to find suitable emergent devices. Memristor, a blend of the words memory and resistor, is a passive device postulated by Leon Chua in 1971. In contrast with the other fundamental passive elements, memristors have the distinctive feature of modifying their resistance according to the charge that passes through these devices, and remaining unaltered when charge no longer flows. Although when it appeared no physical device implementation was acknowledged, HP Labs claimed in 2008 the manufacture of the first real memristor. This milestone triggered an unexpectedly high research activity about memristors, both in searching new materials and structures as well as in potential applications. Nowadays, memristors are not only appreciated in memory systems by their nonvolatile storage properties, but in many other fields, such as digital computing, signal processing circuits, or non-conventional applications like neuromorphic computing or chaotic circuits. In spite of their promising features, memristors show a primarily downside: they show significant device variation and limited lifetime due degradation compared with other alternatives. This Thesis explores the challenges that memristor variation and malfunction imposes in potential applications. The main goal is to propose circuits and strategies that either avoid reliability problems or take advantage of them. Throughout a collection of scenarios in which reliability issues are present, their impact is studied by means of simulations. This thesis is contextualized and their objectives are exposed in Chapter 1. In Chapter 2 the memristor is introduced, at both conceptual and experimental levels, and different compact levels are presented to be later used in simulations. Chapter 3 deepens in the phenomena that causes the lack of reliability in memristors, and models that include these defects in simulations are provided. The rest of the Thesis covers different applications. Therefore, Chapter 4 exhibits nonvolatile memory systems, and specifically an online test method for faulty cells. Digital computing is presented in Chapter 5, where a solution for the yield reduction in logic operations due to memristors variability is proposed. Lastly, Chapter 6 reviews applications in the analog domain, and it focuses in the exploitation of results observed in faulty memristor-based interconnect mediums for chaotic systems synchronization purposes. Finally, the Thesis concludes in Chapter 7 along with perspectives about future work.Este trabajo desarrolla un novedoso dispositivo condensador basado en el uso de la nanotecnología. El dispositivo parte del concepto existente de metal-aislador-metal (MIM), pero en lugar de una capa aislante continua, se utilizan nanopartículas dieléctricas. Las nanopartículas son principalmente de óxido de silicio (sílice) y poliestireno (PS) y los valores de diámetro son 255nm y 295nm respectivamente. Las nanopartículas contribuyen a una alta relación superficie/volumen y están fácilmente disponibles a bajo costo. La tecnología de depósito desarrollada en este trabajo se basa en la técnica de electrospray, que es una tecnología de fabricación ascendente (bottom-up) que permite el procesamiento por lotes y logra un buen compromiso entre una gran superficie y un bajo tiempo de depósito. Con el objetivo de aumentar la superficie de depósito, la configuración de electrospray ha sido ajustada para permitir áreas de depósito de 1cm2 a 25cm2. El dispositivo fabricado, los llamados condensadores de metal aislante de nanopartículas (NP-MIM) ofrecen valores de capacidad más altos que un condensador convencional similar con una capa aislante continua. En el caso de los NP-MIM de sílice, se alcanza un factor de hasta 1000 de mejora de la capacidad, mientras que los NP-MIM de poliestireno exhibe una ganancia de capacidad en el rango de 11. Además, los NP-MIM de sílice muestran comportamientos capacitivos en específicos rangos de frecuencias que depende de la humedad y el grosor de la capa de nanopartículas, mientras que los NP-MIM de poliestireno siempre mantienen su comportamiento capacitivo. Los dispositivos fabricados se han caracterizado mediante medidas de microscopía electrónica de barrido (SEM) complementadas con perforaciones de haz de iones focalizados (FIB) para caracterizar la topografía de los NP-MIMs. Los dispositivos también se han caracterizado por medidas de espectroscopia de impedancia, a diferentes temperaturas y humedades. El origen de la capacitancia aumentada está asociado en parte a la humedad en las interfaces de las nanopartículas. Se ha desarrollado un modelo de un circuito basado en elementos distribuidos para ajustar y predecir el comportamiento eléctrico de los NP-MIMs. En resumen, esta tesis muestra el diseño, fabricación, caracterización y modelización de un nuevo y prometedor condensador nanopartículas metal-aislante-metal que puede abrir el camino al desarrollo de una nueva tecnología de supercondensadores MIM.Postprint (published version

Reliability-aware circuit design to mitigate impact of device defects and variability in emerging memristor-based applications

In the last decades, semiconductor industry has fostered a fast downscale in technology, propelling the large scale integration of CMOS-based systems. The benefits in miniaturization are numerous, highlighting faster switching frequency, lower voltage supply and higher device density. However, this aggressive scaling trend it has not been without challenges, such as leakage currents, yield reduction or the increase in the overall system power dissipation. New materials, changes in the device structures and new architectures are key to keep the miniaturization trend. It is foreseen that 2D integration will eventually come to an insurmountable physical and economic limit, in which new strategic directions are required, such as the development of new device structures, 3D architectures or heterogeneous systems that takes advantage of the best of different technologies, both the ones already consolidated as well as emergent ones that provide performance and efficiency improvements in applications. In this context, memristor arises as one of several candidates in the race to find suitable emergent devices. Memristor, a blend of the words memory and resistor, is a passive device postulated by Leon Chua in 1971. In contrast with the other fundamental passive elements, memristors have the distinctive feature of modifying their resistance according to the charge that passes through these devices, and remaining unaltered when charge no longer flows. Although when it appeared no physical device implementation was acknowledged, HP Labs claimed in 2008 the manufacture of the first real memristor. This milestone triggered an unexpectedly high research activity about memristors, both in searching new materials and structures as well as in potential applications. Nowadays, memristors are not only appreciated in memory systems by their nonvolatile storage properties, but in many other fields, such as digital computing, signal processing circuits, or non-conventional applications like neuromorphic computing or chaotic circuits. In spite of their promising features, memristors show a primarily downside: they show significant device variation and limited lifetime due degradation compared with other alternatives. This Thesis explores the challenges that memristor variation and malfunction imposes in potential applications. The main goal is to propose circuits and strategies that either avoid reliability problems or take advantage of them. Throughout a collection of scenarios in which reliability issues are present, their impact is studied by means of simulations. This thesis is contextualized and their objectives are exposed in Chapter 1. In Chapter 2 the memristor is introduced, at both conceptual and experimental levels, and different compact levels are presented to be later used in simulations. Chapter 3 deepens in the phenomena that causes the lack of reliability in memristors, and models that include these defects in simulations are provided. The rest of the Thesis covers different applications. Therefore, Chapter 4 exhibits nonvolatile memory systems, and specifically an online test method for faulty cells. Digital computing is presented in Chapter 5, where a solution for the yield reduction in logic operations due to memristors variability is proposed. Lastly, Chapter 6 reviews applications in the analog domain, and it focuses in the exploitation of results observed in faulty memristor-based interconnect mediums for chaotic systems synchronization purposes. Finally, the Thesis concludes in Chapter 7 along with perspectives about future work.Este trabajo desarrolla un novedoso dispositivo condensador basado en el uso de la nanotecnología. El dispositivo parte del concepto existente de metal-aislador-metal (MIM), pero en lugar de una capa aislante continua, se utilizan nanopartículas dieléctricas. Las nanopartículas son principalmente de óxido de silicio (sílice) y poliestireno (PS) y los valores de diámetro son 255nm y 295nm respectivamente. Las nanopartículas contribuyen a una alta relación superficie/volumen y están fácilmente disponibles a bajo costo. La tecnología de depósito desarrollada en este trabajo se basa en la técnica de electrospray, que es una tecnología de fabricación ascendente (bottom-up) que permite el procesamiento por lotes y logra un buen compromiso entre una gran superficie y un bajo tiempo de depósito. Con el objetivo de aumentar la superficie de depósito, la configuración de electrospray ha sido ajustada para permitir áreas de depósito de 1cm2 a 25cm2. El dispositivo fabricado, los llamados condensadores de metal aislante de nanopartículas (NP-MIM) ofrecen valores de capacidad más altos que un condensador convencional similar con una capa aislante continua. En el caso de los NP-MIM de sílice, se alcanza un factor de hasta 1000 de mejora de la capacidad, mientras que los NP-MIM de poliestireno exhibe una ganancia de capacidad en el rango de 11. Además, los NP-MIM de sílice muestran comportamientos capacitivos en específicos rangos de frecuencias que depende de la humedad y el grosor de la capa de nanopartículas, mientras que los NP-MIM de poliestireno siempre mantienen su comportamiento capacitivo. Los dispositivos fabricados se han caracterizado mediante medidas de microscopía electrónica de barrido (SEM) complementadas con perforaciones de haz de iones focalizados (FIB) para caracterizar la topografía de los NP-MIMs. Los dispositivos también se han caracterizado por medidas de espectroscopia de impedancia, a diferentes temperaturas y humedades. El origen de la capacitancia aumentada está asociado en parte a la humedad en las interfaces de las nanopartículas. Se ha desarrollado un modelo de un circuito basado en elementos distribuidos para ajustar y predecir el comportamiento eléctrico de los NP-MIMs. En resumen, esta tesis muestra el diseño, fabricación, caracterización y modelización de un nuevo y prometedor condensador nanopartículas metal-aislante-metal que puede abrir el camino al desarrollo de una nueva tecnología de supercondensadores MIM

Reliability-aware circuit design to mitigate impact of device defects and variability in emerging memristor-based applications

In the last decades, semiconductor industry has fostered a fast downscale in technology, propelling the large scale integration of CMOS-based systems. The benefits in miniaturization are numerous, highlighting faster switching frequency, lower voltage supply and higher device density. However, this aggressive scaling trend it has not been without challenges, such as leakage currents, yield reduction or the increase in the overall system power dissipation. New materials, changes in the device structures and new architectures are key to keep the miniaturization trend. It is foreseen that 2D integration will eventually come to an insurmountable physical and economic limit, in which new strategic directions are required, such as the development of new device structures, 3D architectures or heterogeneous systems that takes advantage of the best of different technologies, both the ones already consolidated as well as emergent ones that provide performance and efficiency improvements in applications. In this context, memristor arises as one of several candidates in the race to find suitable emergent devices. Memristor, a blend of the words memory and resistor, is a passive device postulated by Leon Chua in 1971. In contrast with the other fundamental passive elements, memristors have the distinctive feature of modifying their resistance according to the charge that passes through these devices, and remaining unaltered when charge no longer flows. Although when it appeared no physical device implementation was acknowledged, HP Labs claimed in 2008 the manufacture of the first real memristor. This milestone triggered an unexpectedly high research activity about memristors, both in searching new materials and structures as well as in potential applications. Nowadays, memristors are not only appreciated in memory systems by their nonvolatile storage properties, but in many other fields, such as digital computing, signal processing circuits, or non-conventional applications like neuromorphic computing or chaotic circuits. In spite of their promising features, memristors show a primarily downside: they show significant device variation and limited lifetime due degradation compared with other alternatives. This Thesis explores the challenges that memristor variation and malfunction imposes in potential applications. The main goal is to propose circuits and strategies that either avoid reliability problems or take advantage of them. Throughout a collection of scenarios in which reliability issues are present, their impact is studied by means of simulations. This thesis is contextualized and their objectives are exposed in Chapter 1. In Chapter 2 the memristor is introduced, at both conceptual and experimental levels, and different compact levels are presented to be later used in simulations. Chapter 3 deepens in the phenomena that causes the lack of reliability in memristors, and models that include these defects in simulations are provided. The rest of the Thesis covers different applications. Therefore, Chapter 4 exhibits nonvolatile memory systems, and specifically an online test method for faulty cells. Digital computing is presented in Chapter 5, where a solution for the yield reduction in logic operations due to memristors variability is proposed. Lastly, Chapter 6 reviews applications in the analog domain, and it focuses in the exploitation of results observed in faulty memristor-based interconnect mediums for chaotic systems synchronization purposes. Finally, the Thesis concludes in Chapter 7 along with perspectives about future work.Este trabajo desarrolla un novedoso dispositivo condensador basado en el uso de la nanotecnología. El dispositivo parte del concepto existente de metal-aislador-metal (MIM), pero en lugar de una capa aislante continua, se utilizan nanopartículas dieléctricas. Las nanopartículas son principalmente de óxido de silicio (sílice) y poliestireno (PS) y los valores de diámetro son 255nm y 295nm respectivamente. Las nanopartículas contribuyen a una alta relación superficie/volumen y están fácilmente disponibles a bajo costo. La tecnología de depósito desarrollada en este trabajo se basa en la técnica de electrospray, que es una tecnología de fabricación ascendente (bottom-up) que permite el procesamiento por lotes y logra un buen compromiso entre una gran superficie y un bajo tiempo de depósito. Con el objetivo de aumentar la superficie de depósito, la configuración de electrospray ha sido ajustada para permitir áreas de depósito de 1cm2 a 25cm2. El dispositivo fabricado, los llamados condensadores de metal aislante de nanopartículas (NP-MIM) ofrecen valores de capacidad más altos que un condensador convencional similar con una capa aislante continua. En el caso de los NP-MIM de sílice, se alcanza un factor de hasta 1000 de mejora de la capacidad, mientras que los NP-MIM de poliestireno exhibe una ganancia de capacidad en el rango de 11. Además, los NP-MIM de sílice muestran comportamientos capacitivos en específicos rangos de frecuencias que depende de la humedad y el grosor de la capa de nanopartículas, mientras que los NP-MIM de poliestireno siempre mantienen su comportamiento capacitivo. Los dispositivos fabricados se han caracterizado mediante medidas de microscopía electrónica de barrido (SEM) complementadas con perforaciones de haz de iones focalizados (FIB) para caracterizar la topografía de los NP-MIMs. Los dispositivos también se han caracterizado por medidas de espectroscopia de impedancia, a diferentes temperaturas y humedades. El origen de la capacitancia aumentada está asociado en parte a la humedad en las interfaces de las nanopartículas. Se ha desarrollado un modelo de un circuito basado en elementos distribuidos para ajustar y predecir el comportamiento eléctrico de los NP-MIMs. En resumen, esta tesis muestra el diseño, fabricación, caracterización y modelización de un nuevo y prometedor condensador nanopartículas metal-aislante-metal que puede abrir el camino al desarrollo de una nueva tecnología de supercondensadores MIM

Crossbar-based memristive logic-in-memory architecture

The use of memristors and resistive random access memory (ReRAM) technology to perform logic computations, has drawn considerable attention from researchers in recent years. However, the topological aspects of the underlying ReRAM architecture and its organization have received less attention, as the focus has mainly been on device-specific properties for functionally complete logic gates through conditional switching in ReRAM circuits. A careful investigation and optimization of the target geometry is thus highly desirable for the implementation of logic-in-memory architectures. In this paper, we propose a crossbar-based in-memory parallel processing system in which, through the heterogeneity of the resistive cross-point devices, we achieve local information processing in a state-of-the-art ReRAM crossbar architecture with vertical group-accessed transistors as cross-point selector devices. We primarily focus on the array organization, information storage, and processing flow, while proposing a novel geometry for the cross-point selection lines to mitigate current sneak-paths during an arbitrary number of possible parallel logic computations. We prove the proper functioning and potential capabilities of the proposed architecture through SPICE-level circuit simulations of half-adder and sum-of-products logic functions. We compare certain features of the proposed logic-in-memory approach with another work of the literature, and present an analysis of circuit resources, integration density, and logic computation parallelism.Peer ReviewedPostprint (author's final draft

Reconfigurable writing architecture for reliable RRAM operation in wide temperature ranges

Resistive switching memories [resistive RAM (RRAM)] are an attractive alternative to nonvolatile storage and nonconventional computing systems, but their behavior strongly depends on the cell features, driver circuit, and working conditions. In particular, the circuit temperature and writing voltage schemes become critical issues, determining resistive switching memories performance. These dependencies usually force a design time tradeoff among reliability, device endurance, and power consumption, thereby imposing nonflexible functioning schemes and limiting the system performance. In this paper, we present a writing architecture that ensures the correct operation no matter the working temperature and allows the dynamic load of application-oriented writing profiles. Thus, taking advantage of more efficient configurations, the system can be dynamically adapted to overcome RRAM intrinsic challenges. Several profiles are analyzed regarding power consumption, temperature-variations protection, and operation speed, showing speedups near 700x compared with other published drivers

Design of Resistive Synaptic Devices and Array Architectures for Neuromorphic Computing

abstract: Over the past few decades, the silicon complementary-metal-oxide-semiconductor (CMOS) technology has been greatly scaled down to achieve higher performance, density and lower power consumption. As the device dimension is approaching its fundamental physical limit, there is an increasing demand for exploration of emerging devices with distinct operating principles from conventional CMOS. In recent years, many efforts have been devoted in the research of next-generation emerging non-volatile memory (eNVM) technologies, such as resistive random access memory (RRAM) and phase change memory (PCM), to replace conventional digital memories (e.g. SRAM) for implementation of synapses in large-scale neuromorphic computing systems. Essentially being compact and “analog”, these eNVM devices in a crossbar array can compute vector-matrix multiplication in parallel, significantly speeding up the machine/deep learning algorithms. However, non-ideal eNVM device and array properties may hamper the learning accuracy. To quantify their impact, the sparse coding algorithm was used as a starting point, where the strategies to remedy the accuracy loss were proposed, and the circuit-level design trade-offs were also analyzed. At architecture level, the parallel “pseudo-crossbar” array to prevent the write disturbance issue was presented. The peripheral circuits to support various parallel array architectures were also designed. One key component is the read circuit that employs the principle of integrate-and-fire neuron model to convert the analog column current to digital output. However, the read circuit is not area-efficient, which was proposed to be replaced with a compact two-terminal oscillation neuron device that exhibits metal-insulator-transition phenomenon. To facilitate the design exploration, a circuit-level macro simulator “NeuroSim” was developed in C++ to estimate the area, latency, energy and leakage power of various neuromorphic architectures. NeuroSim provides a wide variety of design options at the circuit/device level. NeuroSim can be used alone or as a supporting module to provide circuit-level performance estimation in neural network algorithms. A 2-layer multilayer perceptron (MLP) simulator with integration of NeuroSim was demonstrated to evaluate both the learning accuracy and circuit-level performance metrics for the online learning and offline classification, as well as to study the impact of eNVM reliability issues such as data retention and write endurance on the learning performance.Dissertation/ThesisDoctoral Dissertation Electrical Engineering 201

Réseaux neuronaux robustes face à la variabilité de l’apprentissage machine sur crossbar passif de mémoires résistives à base de TiO2

La présence des réseaux neuronaux dans notre quotidien connaît une augmentation exponentielle. Les réseaux sociaux, les moteurs de recherche et le commerce électronique ne sont que quelques exemples de domaines les sollicitant en permanence. La taille de ces réseaux, à l'image de leur présence, a également connu un constant essor. Or, plus un réseau neuronal comporte de paramètres, plus il consomme d'énergie puisqu'il nécessite toujours plus d'accès successifs en mémoire afin de chercher et/ou d'altérer ceux-ci. C'est ce goulot d'étranglement entre le processeur et les données qui limite dramatiquement l'efficience énergétique des réseaux neuronaux implémentés sur l'architecture de von Neumann. Une approche prometteuse pour détourner ce problème est l'utilisation d'une composante électronique permettant une version analogue des opérations de multiplication matrice-vecteur essentielles à l'apprentissage machine directement sur mémoire: les mémoires résistives. Cependant, les défauts inhérents dont celles-ci sont affligées les rendent difficiles à utiliser en tant que poids synaptique discret et précis. Il devient donc très intéressant de considérer certaines sources de variabilité de ces mémoires émergentes lors de l'entraînement des réseaux neuronaux afin d'exploiter leurs facultés d'apprentissage pour les rendre ainsi aptes à classifier efficacement en les utilisant malgré leur nombreuses non-idéalités. Ces réseaux stochastiques sont donc robustes à la variabilité matérielle des dispositifs. Une enquête du potentiel de réseaux neuronaux considérant ces défauts stochastiques fut menée durant ce projet de maîtrise. De nouvelles techniques de caractérisation de la variabilité des crossbars et des mémoires résistives furent élaborées. L'utilisation de ces données pour injecter du bruit sur les poids synaptiques du réseau lors de son entraînement permet de créer un réseau plus robuste. Il est prouvé en simulation qu'un réseau conscient des non-idéalités est considérablement plus précis qu'un réseau entraîné naïvement pour une même tâche de classification de demi-lunes lorsque les variabilités sont prises en compte

Tailored electrical characteristics in multilayer metal-oxide-based-memristive devices

Auf Mehrlagen-Metalloxiden basierende memristive Bauelemente sind einer der vielversprechendsten Kandidaten für neuromorphes Computing. Allerdings stellen spezifische Anwendungen des neuromorphen Computings unterschiedliche Anforderungen an die memristiven Bauelemente. Eine ungelöste Herausforderung in der technologischen Entwicklung ist daher das maßgeschneiderte Design von memristiven Bauelementen für spezifische Anwendungen. Insbesondere die unterschiedlichen Materialien des Schichtstapels erschweren die Herstellungsprozesse aufgrund einer großen Anzahl von Parametern, wie z. B. der Stapelsequenzen und -dicken und der Qualität sowie der Eigenschaften der einzelnen Schichten. Daher sind systematische Untersuchungen der einzelnen Bauelementparameter besonders entscheidend. Darüber hinaus müssen sie mit einem tiefgreifenden Verständnis der zugrundeliegenden physikalischen Prozesse kombiniert werden, um die Lücke zwischen Materialdesign und elektrischen Eigenschaften der resultierenden memristiven Bauelemente zuschließen. Um memristive Bauelemente mit unterschiedlichen resistiven Schalteigenschaften zu erhalten, werden verschiedene Abfolgen und Kombinationen von drei Metalloxidschichten (TiOx, HfOx, und AlOx) hergestellt und untersucht. Zunächst werden einschichtige Oxidbauelemente untersucht, um Kandidaten für mehrschichtige Stapel zu identifizieren. Zweitens werden zweischichtige TiOx/HfOx Oxidbauelemente hergestellt. Anhand von systematischen Experimenten und statistischen Analysen wird gezeigt, dass die Stöchiometrie, die Dicke, und die Fläche des Bauelements die Betriebsspannungen, die Nichtlinearität beim resistiven Schalten und die Variabilität beeinflussen. Drittens werden TiOx/AlOx/HfOx-basierte Bauelemente hergestellt. Durch das Hinzufügen von AlOx in die zweischichtigen Oxidstapel weisen diese dreischichtigen Bauelemente optimale elektrische Eigenschaften für den Einsatz in neuromorpher Hardware auf, wie z. B. elektroformierungsfreies und strombegrenzungsloses Schalten sowie eine lange Lebensdauer. Die entwickelten memristiven Bauelemente werden in Systeme, wie Kreuzpunkt-Strukturen und Ein-Transistor-ein-Memristor-Konfigurationen integriert. Hier wird die Eignung für effizientes neuromorphes Computing bewertet. Außerdem werden Methoden zur stufenlosen analogen Einstellung des Widerstands der Bauelemente demonstriert. Diese Eigenschaft ermöglicht effiziente neuromorphe Rechenschemata. Diese umfassende Studie beleuchtet die Beziehung zwischen den Bauelementparametern und den elektrischen Eigenschaften von mehrschichtigen memristiven Bauelementen auf Metalloxidbasis. Auf dieser Grundlage werden maßgeschneiderte Methoden für spezifische neuromorphe Anwendungen entwickelt.Multilayer metal-oxide-based-memristive devices are one of the most promising candidates for neuromorphic computing. However, specific applications of neuromorphic computing call for different requirements for memristive devices. Therefore, an open challenge in technological development is the tailored design of memristive devices for specific applications. In particular, multilayer stacks complicate fabrication processes due to a large number of device parameters such as staking sequences and thicknesses, quality, and property of each layer. Therefore, systematic investigations of the individual device parameters are particularly decisive. Moreover, they need to be combined with a profound understanding of the underlying physical processes to bridge the gap between material design and electrical characteristics of the resulting memristive devices. To obtain memristive devices with different resistance switching characteristics, various sequences and combinations of three metal oxide layers (TiOx, HfOx, and AlOx) are fabricated and studied. First, single-layer oxide devices are investigated to find desirable multilayer stacks for memristive devices. Second, TiOx/HfOx-based bilayer oxide devices are fabricated. Via systematic experiments and statistical analysis, it is shown that the stoichiometry, thickness, and device area influence operating voltages, non-linearity in resistive switching, and variability. Third, TiOx/AlOx/HfOx-based devices are fabricated. By adding AlOx into the bilayer oxide stacks, these trilayer devices present favorable electrical features for use in neuromorphic hardware, such as electroforming-free and compliance-free switching as well as long retention. The developed memristive devices are integrated into systems such as crossbar structures and one-transistor-one-memristor configurations. Here, suitability for efficient neuromorphic computing is assessed. Also, methods to tune the device resistance gradually in an analog fashion are demonstrated. This feature allows for efficient neuromorphic computation. This comprehensive study highlights the relationship between device parameters and electrical properties of multilayer metal-oxide-based memristive devices. On this basis, tailoring methodologies are established for specific neuromorphic applications