59 research outputs found
A Causal Disentangled Multi-Granularity Graph Classification Method
Graph data widely exists in real life, with large amounts of data and complex
structures. It is necessary to map graph data to low-dimensional embedding.
Graph classification, a critical graph task, mainly relies on identifying the
important substructures within the graph. At present, some graph classification
methods do not combine the multi-granularity characteristics of graph data.
This lack of granularity distinction in modeling leads to a conflation of key
information and false correlations within the model. So, achieving the desired
goal of a credible and interpretable model becomes challenging. This paper
proposes a causal disentangled multi-granularity graph representation learning
method (CDM-GNN) to solve this challenge. The CDM-GNN model disentangles the
important substructures and bias parts within the graph from a
multi-granularity perspective. The disentanglement of the CDM-GNN model reveals
important and bias parts, forming the foundation for its classification task,
specifically, model interpretations. The CDM-GNN model exhibits strong
classification performance and generates explanatory outcomes aligning with
human cognitive patterns. In order to verify the effectiveness of the model,
this paper compares the three real-world datasets MUTAG, PTC, and IMDM-M. Six
state-of-the-art models, namely GCN, GAT, Top-k, ASAPool, SUGAR, and SAT are
employed for comparison purposes. Additionally, a qualitative analysis of the
interpretation results is conducted
Diseño de 1600 ML de adoquinado, ubicado en los barrios: anexo a la villa Victoria de julio, Antonio Mendoza y Rubén Ulloa; en el casco urbano de Tipitapa, municipio de Managua
El desarrollo de nuestro país se basa en elementos fundamentales, como: agricultura industria, ganadería, comercio, turismo, etc. Pero el factor determinante entre estos es el sistema nacional de transporte es decir: transporte terrestre, transporte aéreo, transporte marítimo, etc. el cual es el enlace principal para el desarrollo de la sociedad. En Nicaragua el transporte terrestre es el más utilizado por la población, y debido al aumento de la movilización de vehículos con motores más potentes por las vías, obliga a la modernización de la infraestructura vial, permitiendo un tránsito más seguro y eficiente. El incremento de la red vial está vinculado directamente con la economía de nuestro país, pues su papel es primordial en las actividades que se realizan a diario en los diferentes sectores que aportan a la economía nacional. Actualmente la construcción de nuevas vías de comunicación, rehabilitación de carreteras y mejoras de los caminos ya existentes debe ser una necesidad para los gobiernos, ya que constituyen un componente fundamental para el bienestar y desarrollo de la sociedad, además su diseño debe adoptar las condiciones necesarias para obtener una obra de calidad; cumpliéndose en el todos los principios y normas correspondientes al diseño de carreteras. El presente trabajo denominado ‘‘Diseño de 1600 ML de calle, ubicados en los barrios: Anexo la Villa Rubén Ulloa, Villa Victoria de Julio y Antonio Mendoza localizados en el casco urbano de Tipitapa, municipio de Managua’’. Muestra en su contenido los estudios, métodos y normas aplicables para elaborar: el diseño geométrico de la vía, diseño hidráulico y de la estructura de pavimento, tomando en cuenta las especificaciones correspondientes al diseño de carreteras en Nicaragua
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Heterogeneous N2O5 reactions on atmospheric aerosols at four Chinese sites : improving model representation of uptake parameters
Heterogeneous reactivity of N2O5 on aerosols is a critical parameter in assessing NOx fate, nitrate production, and particulate chloride activation. Accurate measurement of its uptake coefficient (gamma N2O5) and representation in air quality models are challenging, especially in the polluted environment. With an in situ aerosol flow-tube system, the gamma N2O5 was directly measured on ambient aerosols at two rural sites in northern and southern China. The results were analyzed together with the gamma N2O5 derived from previous field studies in China to obtain a holistic picture of gamma N2O5 uptake and the influencing factors under various climatic and chemical conditions. The field-derived or measured gamma N2O5 was generally promoted by the aerosol water content and suppressed by particle nitrate. Significant discrepancies were found between the measured gamma N2O5 and that estimated from laboratory-determined parameterizations. An observation-based empirical parameterization was derived in the present work, which better reproduced the mean value and variability of the observed gamma N2O5. Incorporating this new parameterization into a regional air quality model (WRF-CMAQ) has improved the simulation of N2O5, nitrogen oxides, and secondary nitrate in the polluted regions of China.Peer reviewe
Seasonal variation in oxygenated organic molecules in urban Beijing and their contribution to secondary organic aerosol
Oxygenated organic molecules (OOMs) are crucial for atmospheric new particle formation and secondary organic aerosol (SOA) growth. Therefore, understanding their chemical composition, temporal behavior, and sources is of great importance. Previous studies on OOMs mainly focus on environments where biogenic sources are predominant, yet studies on sites with dominant anthropogenic emissions, such as megacities, have been lacking. Here, we conducted long-term measurements of OOMs, covering four seasons of the year 2019, in urban Beijing. The OOM concentration was found to be the highest in summer (1.6 x 10(8) cm(-3)), followed by autumn (7.9 x 10(7) cm(-3)), spring (5.7 x 10(7) cm(-3)) and winter (2.3 x 10(7) cm(-3)), suggesting that enhanced photo-oxidation together with the rise in temperature promote the formation of OOMs. Most OOMs contained 5 to 10 carbon atoms and 3 to 7 effective oxygen atoms (nO(eff) = nO - 2 x nN). The average nO(eff )increased with increasing atmospheric photo-oxidation capacity, which was the highest in summer and the lowest in winter and autumn. By performing a newly developed workflow, OOMs were classified into the following four types: aromatic OOMs, aliphatic OOMs, isoprene OOMs, and monoterpene OOMs. Among them, aromatic OOMs (29 %-41 %) and aliphatic OOMs (26 %-41 %) were the main contributors in all seasons, indicating that OOMs in Beijing were dominated by anthropogenic sources. The contribution of isoprene OOMs increased significantly in summer (33 %), which is much higher than those in the other three seasons (8 %-10 %). Concentrations of isoprene (0.2-5.3 x 10(7) cm(-3)) and monoterpene (1.1-8.4 x 10(6) cm(-3)) OOMs in Beijing were lower than those reported at other sites, and they possessed lower oxygen and higher nitrogen contents due to high NO, levels (9.5-38.3 ppbv - parts per billion by volume) in Beijing. With regard to the nitrogen content of the two anthropogenic OOMs, aromatic OOMs were mainly composed of CHO and CHON species, while aliphatic OOMs were dominated by CHON and CHON2 ones. Such prominent differences suggest varying formation pathways between these two OOMs. By combining the measurements and an aerosol dynamic model, we estimated that the SOA growth rate through OOM condensation could reach 0.64, 0.61, 0.41, and 0.30 mu g m(-3) h(-1) in autumn, summer, spring, and winter, respectively. Despite the similar concentrations of aromatic and aliphatic OOMs, the former had lower volatilities and, therefore, showed higher contributions (46 %-62 %) to SOA than the latter (14 %-32 %). By contrast, monoterpene OOMs and isoprene OOMs, limited by low abundances or high volatilities, had low contributions of 8 %-12 % and 3 %-5 %, respectively. Overall, our results improve the understanding of the concentration, chemical composition, seasonal variation, and potential atmospheric impacts of OOMs, which can help formulate refined restriction policy specific to SOA control in urban areas.Peer reviewe
Gray solitary-wave solutions in nonlinear negative-index materials
We predict the existence of gray (dark) solitary waves in negative-index materials on the basis of a derived higher-order nonlinear Schrödinger equation. The conditions for the formation of three cases of gray solitary waves and exact analytical express
Mechanically Robust and Flexible GO/PI Hybrid Aerogels as Highly Efficient Oil Absorbents
Herein, mechanically robust and flexible graphene oxide/polyimide (GO/PI) hybrid aerogels (GIAs) were fabricated by a facile method, in which the mixed suspensions of the water-soluble polyimide precursor and graphene oxide (GO) sheets were freeze-dried, which was followed by a routine thermal imidation process. The porous GIAs obtained not only exhibit excellent elasticity and extremely low density values (from 33.3 to 38.9 mg.cm−3), but they also possess a superior compressive strength (121.7 KPa). The GIAs could support a weight of up to 31,250 times of its own weight, and such a weight-carrying capacity is much higher than that of other typical carbon-based aerogels. Having such a porous structure, and high strength and toughness properties make GIAs ideal candidates for oil spill cleanup materials. The oil/organic solvents’ absorption capacity ranges from 14.6 to 85, which is higher than that of most other aerogels (sponges). With their broad temperature tolerance and acidic stability, the unique multifunctional GIAs are expected to further extend their application range into extreme environments
Influence of Moisture Content on Electromagnetic Response of Concrete Studied Using a Homemade Apparatus
In this study, we examined the influence of moisture content on the electromagnetic response of concrete. A novel homemade electromagnetic monitoring apparatus was developed and used to evaluate the Hall effect voltage at both ends of concrete based on our previous study of the Hall effect. We used four different concrete mix water/binder ratios: 0.30, 0.28, 0.26, and 0.24, and three conditions (relative humidity, carbonation, and water absorption) were examined in this experiment. The results show that the moisture content inside concrete influences the relative permeability of concrete. The variation in the Hall effect voltage is more influenced by carbonation than changes in relative humidity; water absorption increases the Hall effect voltage the least amongst the other examined factors. According to the experiment, a calibration system was established, and the relevant correction factors are provided
Volume Deformation of Steam-Cured Concrete with Slag during and after Steam Curing
In order to better predict the development of shrinkage deformation of steam-cured concrete mixed with slag, a deformation-temperature-humidity integrated model test, a hydration heat test, and an elastic modulus test were performed. The effects of the steam-curing process and the content of slag on shrinkage deformation, hydration degree and elastic modulus of concrete were studied. The results indicate that during the steam-curing process, the concrete has an “expansion-shrinkage” pattern. After the steam curing, the deformation of concrete is dominated by drying shrinkage. After the addition of slag, the shrinkage deformation of steam-cured concrete is increased. The autogenous shrinkage increases by 0.5–12%, and the total shrinkage increases by 1.5–8% at 60 days. At the same time, slag reduces the hydration degree of steam-cured concrete and modulus of elasticity. A prediction model for the hydration degree of steam-cured concrete is established, which can be used to calculate the degree of hydration at any curing age. Based on the capillary tension generated by the capillary pores in concrete, an integrated model of autogenous shrinkage and total shrinkage is established with the relative humidity directly related to the water loss in the concrete as the driving parameter. Whether the shrinkage deformation is caused by hydration reaction or the external environment, this model can better predict the shrinkage deformation of steam-cured concrete
Data from: Mechanism of Ca2+, Mg2+ and Fe3+ in fine cassiterite flotation using octanohydroxamic acid
The existence of metal ion should not be ignored in both hydrometallurgy and flotation. In this study, the effects of Ca2+, Mg2+ and Fe3+ on the flotation performance of cassiterite using octanohydroxamic acid (OHA) as the collector were investigated by the micro-flotation tests, X-ray photoelectron spectroscopy (XPS), fourier transform infrared spectroscopy (FTIR), contact angle, zeta (ζ) potential measurements and atomic force microscopy (AFM) imaging. The results of the flotation and contact angle experiments showed that the addition of Ca2+, Mg2+ and Fe3+ significantly decreased both the recovery and contact angle of cassiterite within pH ranged from 6.0 to 12.0 in the presence of OHA collector. ζ–potential measurements, solution chemistry analysis and FTIR measurements indicated that the flotation recovery of the cassiterite declined due to the CaOH+, MgOH+ and Fe(OH)3 sites on the cassiterite surface. XPS results indicated that the chemisorption of OHA on cassiterite surface and its adsorption combined with calcium ions effects finally changed the chemical properties of cassiterite surface. The AFM images also revealed that new species Fe(OH)3 of Fe3+ formed and adsorbed on the cassiterite surface at pH of 9.0. The adsorption of Fe(OH)3 reduced the adsorption of OHA on the cassiterite surface, thus the hydrophobicity of cassiterite was deteriorated
Data from: Mechanism of Ca2+, Mg2+ and Fe3+ in fine cassiterite flotation using octanohydroxamic acid
The existence of metal ion should not be ignored in both hydrometallurgy and flotation. In this study, the effects of Ca2+, Mg2+ and Fe3+ on the flotation performance of cassiterite using octanohydroxamic acid (OHA) as the collector were investigated by the micro-flotation tests, X-ray photoelectron spectroscopy (XPS), fourier transform infrared spectroscopy (FTIR), contact angle, zeta (ζ) potential measurements and atomic force microscopy (AFM) imaging. The results of the flotation and contact angle experiments showed that the addition of Ca2+, Mg2+ and Fe3+ significantly decreased both the recovery and contact angle of cassiterite within pH ranged from 6.0 to 12.0 in the presence of OHA collector. ζ–potential measurements, solution chemistry analysis and FTIR measurements indicated that the flotation recovery of the cassiterite declined due to the CaOH+, MgOH+ and Fe(OH)3 sites on the cassiterite surface. XPS results indicated that the chemisorption of OHA on cassiterite surface and its adsorption combined with calcium ions effects finally changed the chemical properties of cassiterite surface. The AFM images also revealed that new species Fe(OH)3 of Fe3+ formed and adsorbed on the cassiterite surface at pH of 9.0. The adsorption of Fe(OH)3 reduced the adsorption of OHA on the cassiterite surface, thus the hydrophobicity of cassiterite was deteriorated
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