620 research outputs found

    Nonclassical statistics of intracavity coupled χ(2)\chi^{(2)} waveguides: the quantum optical dimer

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    A model is proposed where two χ(2)\chi^{(2)} nonlinear waveguides are contained in a cavity suited for second-harmonic generation. The evanescent wave coupling between the waveguides is considered as weak, and the interplay between this coupling and the nonlinear interaction within the waveguides gives rise to quantum violations of the classical limit. These violations are particularly strong when two instabilities are competing, where twin-beam behavior is found as almost complete noise suppression in the difference of the fundamental intensities. Moreover, close to bistable transitions perfect twin-beam correlations are seen in the sum of the fundamental intensities, and also the self-pulsing instability as well as the transition from symmetric to asymmetric states display nonclassical twin-beam correlations of both fundamental and second-harmonic intensities. The results are based on the full quantum Langevin equations derived from the Hamiltonian and including cavity damping effects. The intensity correlations of the output fields are calculated semi-analytically using a linearized version of the Langevin equations derived through the positive-P representation. Confirmation of the analytical results are obtained by numerical simulations of the nonlinear Langevin equations derived using the truncated Wigner representation.Comment: 15 pages, 8 figures, submitted to Phys. Rev.

    Photon blockade and quantum dynamics in intracavity coherent photoassociation of Bose-Einstein condensates

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    We demonstrate that a photon blockade effect exists in the intracavity coherent photoassociation of an atomic Bose-Einstein condensate and that the dynamics of the coupled atomic and molecular condensates can only be successfully described by a quantum treatment of all the interacting fields. We show that the usual mean-field calculational approaches give answers that are qualitatively wrong, even for the mean fields. The quantization of the fields gives a degree of freedom that is not present in analogous nonlinear optical processes. The difference between the semiclassical and quantum predictions can actually increase as the three fields increase in size so that there is no obvious classical limit for this process

    Effects of χ(3) nonlinearities in second-harmonic generation

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    We investigate the effects of higher-order, chi ((3)), nonlinearities on the process of second-harmonic generation. In the traveling-wave case we find substantive differences in the macroscopic behavior of the fields when the chi ((3)) components are present. In the intracavity cage, which has been investigated before using a Linearized analysis, we investigate regions where these analyses may not be valid, comparing and contrasting the full quantum simulations with previous results

    Quantum superchemistry: Role of trapping profile and quantum statistics

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    The process of Raman photoassociation of a trapped atomic condensate to form condensed molecules has been labeled superchemistry because it can occur at 0 K and experiences coherent bosonic stimulation. We show here that the differences from ordinary chemical processes go even deeper, with the conversion rates depending on the quantum state of the reactants, as expressed by the Wigner function. We consider different initial quantum states of the trapped atomic condensate and different forms of the confining potentials, demonstrating the importance of the quantum statistics and the extra degrees of freedom which massive particles and trapping potentials make available over the analogous optical process of second-harmonic generation. We show that both mean-field analyses and quantum calculations using an inappropriate initial condition can make inaccurate predictions for a given system. This is possible whether using a spatially dependent analysis or a zero-dimensional approach as commonly used in quantum optics

    Role of quantum statistics in the photoassociation of Bose-Einstein condensates

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    We show that the photoassociation of an atomic Bose-Einstein condensate to form condensed molecules is a chemical process which not only does not obey the Arrhenius rules for chemical reactions, but that it can also depend on the quantum statistics of the reactants. Comparing the predictions of a truncated Wigner representation for different initial quantum states, we find that, even when the quantum prediction for an initial coherent state is close to the Gross-Pitaevskii prediction, other quantum states may result in very different dynamics

    Quantum properties of transverse pattern formation in second-harmonic generation

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    We investigate the spatial quantum noise properties of the one dimensional transverse pattern formation instability in intra-cavity second-harmonic generation. The Q representation of a quasi-probability distribution is implemented in terms of nonlinear stochastic Langevin equations. We study these equations through extensive numerical simulations and analytically in the linearized limit. Our study, made below and above the threshold of pattern formation, is guided by a microscopic scheme of photon interaction underlying pattern formation in second-harmonic generation. Close to the threshold for pattern formation, beams with opposite direction of the off-axis critical wave numbers are shown to be highly correlated. This is observed for the fundamental field, for the second harmonic field and also for the cross-correlation between the two fields. Nonlinear correlations involving the homogeneous transverse wave number, which are not identified in a linearized analysis, are also described. The intensity differences between opposite points of the far fields are shown to exhibit sub-Poissonian statistics, revealing the quantum nature of the correlations. We observe twin beam correlations in both the fundamental and second-harmonic fields, and also nonclassical correlations between them.Comment: 18 pages, 17 figures, submitted to Phys. Rev.

    Model study on the photoassociation of a pair of trapped atoms into an ultralong-range molecule

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    Using the method of quantum-defect theory, we calculate the ultralong-range molecular vibrational states near the dissociation threshold of a diatomic molecular potential which asymptotically varies as 1/R3-1/R^3. The properties of these states are of considerable interest as they can be formed by photoassociation (PA) of two ground state atoms. The Franck-Condon overlap integrals between the harmonically trapped atom-pair states and the ultralong-range molecular vibrational states are estimated and compared with their values for a pair of untrapped free atoms in the low-energy scattering state. We find that the binding between a pair of ground-state atoms by a harmonic trap has significant effect on the Franck-Condon integrals and thus can be used to influence PA. Trap-induced binding between two ground-state atoms may facilitate coherent PA dynamics between the two atoms and the photoassociated diatomic molecule.Comment: 11 pages, 4 figures, to appear in Phys. Rev. A (September, 2003

    Quantum-noise-induced macroscopic revivals in second-harmonic generation

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    We investigate the behavior of the fundamental and second-harmonic fields in phase-matched traveling plane-wave second-harmonic generation, using the full-operator equations of motion. We find that, after a certain interaction length, both the macroscopic and quantum-statistical properties of the harmonic and fundamental fields are qualitatively different from those found in previous analyses. The mean fields do not vary in a monotonic way, but oscillate with the propagation length, leading to an unexpected periodic revival of the fundamental field, triggered by the quantum fluctuations always present in the mode. Accordingly, the amplitude noise of the fundamental, previously predicted to be perfectly squeezed for long interaction lengths, actually reaches a very small minimum for a definite length, then increases again

    Quantum-nondemolition criteria in traveling-wave second-harmonic generation

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    Using the full nonlinear equations of motion, we calculate the quantum-nondemolition (QND) correlations for the traveling-wave second-harmonic generation. We find that, after a short interaction length, these are qualitatively different from results calculated previously using a linearized fluctuation analysis. We demonstrate that, although individual QND criteria can be very good in certain regions, there is no region where all three of the standard criteria are perfect, as has previously been claimed. We also show that only the amplitude quadrature of the output field can be considered as a QND quantity, with the phase quadrature not satisfying all the criteria

    Excess-noise-enhanced parametric down conversion

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    We calculate the influence of excess noise on parametric down conversion in an unstable optical parametric oscillator (OPO), using a quantum quasimode description. We find a strongly enhanced pair photon generation rate below threshold as compared to a conventional stable cavity setup of comparable gain and loss. In addition, the oscillation threshold is lowered due to the influence of the excess noise and the squeezing properties of the emitted light are significantly changed. In general, the maximal quantum-noise suppression in one quadrature component is reduced, which poses strong limitations for the practical usefulness of a geometrically unstable OPO source. The analytical results from our quasimode description are in good agreement with numerical simulations using a positive-P representation of the field in mode space and in position space
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