Neutron Scattering and magnetization studies of Ba2_2Cu2.95_{2.95}Co0.05_{0.05}O4_4Cl2_2: A decorated two-dimensional antiferromagnet

Ba$_2$Cu$_3$O$_4$Cl$_2$ has two inter-penetrating square Cu sublattices, one with square root 2 times the in-plane spacing of the other. Isotropic magnetic interactions between the two sublattices are completely frustrated. Quantum fluctuations resolve the intrinsic degeneracy in the ordering direction of the more weakly coupled sublattice in favor of collinear ordering. We present neutron scattering and magnetization studies of the magnetic structure when the Cu ions are substituted with Co. The Co spins create new magnetic interactions between the two sublattices. The ordering behavior of both Cu sublattices is retained largely unmodified. Between the phase transitions of the two sublattices spin-glass behavior is observed. Magnetization results show a strong enhancement to the ferromagnetic aspect of the magnetic structure. The combination of glassy behavior and large moments strongly suggest that the Co moments induce the formation of local canted states.Comment: 4 figure

Complete set of polarization transfer coefficients for the 3He(p,n){}^{3}{\rm He}(p,n) reaction at 346 MeV and 0 degrees

We report measurements of the cross-section and a complete set of polarization transfer coefficients for the ${}^{3}{\rm He}(p,n)$ reaction at a bombarding energy $T_p$ = 346 MeV and a reaction angle $\theta_{\rm lab}$ = $0^{\circ}$. The data are compared with the corresponding free nucleon-nucleon values on the basis of the predominance of quasi-elastic scattering processes. Significant discrepancies have been observed in the polarization transfer $D_{LL}(0^{\circ})$, which are presumably the result of the three-proton $T$ = 3/2 resonance. The spin--parity of the resonance is estimated to be $1/2^-$, and the distribution is consistent with previous results obtained for the same reaction at $T_p$ = 48.8 MeV.Comment: 4 figures, Accepted for publication in Physical Review

Study of nuclear correlation effects via 12C(p,n)12N(g.s.,1+) at 296 MeV

We report measurements of the cross section and a complete set of polarization observables for the Gamow--Teller ${}^{12}{\rm C}(\vec{p},\vec{n}){}^{12}{\rm N}({\rm g.s.},1^+)$ reaction at a bombarding energy of 296 MeV. The data are compared with distorted wave impulse approximation calculations employing transition form factors normalized to reproduce the observed beta-decay $ft$ value. The cross section is significantly under-predicted by the calculations at momentum transfers $q \gtrsim$ 0.5 ${\rm fm^{-1}}$. The discrepancy is partly resolved by considering the non-locality of the nuclear mean field. However, the calculations still under-predict the cross section at large momentum transfers of $q$ $\simeq$ 1.6 ${\rm fm^{-1}}$. We also performed calculations employing random phase approximation response functions and found that the observed enhancement can be attributed in part to pionic correlations in nuclei.Comment: 5 figures, submitted to Phys. Lett.

Charge-Density-Wave Ordering in the Metal-Insulator Transition Compound PrRu4P12

X-ray and electron diffraction measurements on the metal-insulator (M-I) transition compound PrRu$_4$P$_{12}$ have revealed the emergence of a periodic ordering of charge density around the Pr atoms. It is found that the ordering is associated with the onset of a low temperature insulator phase. These conclusions are supported by the facts that the space group of the crystal structure transforms from Im$\bar{3}$ to Pm$\bar{3}$ below the M-I transition temperature and also that the temperature dependence of the superlattice peaks in the insulator phase follows the squared BCS function. The M-I transition could be originated from the perfect nesting of the Fermi surface and/or the instability of the $f$ electrons.Comment: 4 pages, 5 figures, Phys. Rev. B (2004) (in press

Thin Ice Target for 16^{16}O(p,p') experiment

A windowless and self-supporting ice target is described. An ice sheet with a thickness of 29.7 mg/cm$^2$ cooled by liquid nitrogen was placed at the target position of a magnetic spectrometer and worked stably in the $^{16}$O$(p,p')$ experiment at $E_{p}=392$ MeV. Background-free spectra were obtained.Comment: 14 pages, 4 figures, Nucl. Instr. & Meth. A (in press

Scalar and vector form factors of the in-medium nucleon

Using the quark-meson coupling model, we calculate the form factors at sigma- and omega-nucleon strong-interaction vertices in nuclear matter. The Peierls-Yoccoz projection technique is used to take account of center of mass and recoil corrections. We also apply the Lorentz contraction to the internal quark wave function. The form factors are reduced by the nuclear medium relative to those in vacuum. At normal nuclear matter density and Q^2 = 1 GeV^2, the reduction rate in the scalar form factor is about 15%, which is almost identical to that in the vector one. We parameterize the ratios of the form factors in symmetric nuclear matter to those in vacuum as a function of nuclear density and momentum transfer.Comment: 13 pages, 2 figures, references are up date

Performance of the neutron polarimeter NPOL3 for high resolution measurements

We describe the neutron polarimeter NPOL3 for the measurement of polarization transfer observables $D_{ij}$ with a typical high resolution of $\sim$300 keV at $T_n$ $\simeq$ 200 MeV. The NPOL3 system consists of three planes of neutron detectors. The first two planes for neutron polarization analysis are made of 20 sets of one-dimensional position-sensitive plastic scintillation counters with a size of 100 cm $\times$ 10 cm $\times$ 5 cm, and they cover the area of 100 $\times$ 100 $\mathrm{cm}^2$. The last plane for detecting doubly scattered neutrons or recoiled protons is made of the two-dimensional position-sensitive liquid scintillation counter with a size of 100 cm $\times$ 100 cm $\times$ 10 cm. The effective analyzing powers $A_{y;\mathrm{eff}}$ and double scattering efficiencies $\epsilon_{\mathrm{D.S.}}$ were measured by using the three kinds of polarized neutrons from the ${}^{2}{\rm H}(\vec{p},\vec{n})pp$, ${}^{6}{\rm Li}(\vec{p},\vec{n}){}^{6}{\rm Be}(\mathrm{g.s.})$, and ${}^{12}{\rm C}(\vec{p},\vec{n}){}^{12}{\rm N}(\mathrm{g.s.})$ reactions at $T_p$ = 198 MeV. The performance of NPOL3 defined as $\epsilon_{\mathrm{D.S.}}(A_{y;\mathrm{eff}})^2$ are similar to that of the Indiana Neutron POLarimeter (INPOL) by taking into account for the counter configuration difference between these two neutron polarimeters.Comment: 28 pages, 18 figures, submitted to Nucl. Instrum. Methods Phys. Res.

Tight-binding parameters and exchange integrals of Ba_2Cu_3O_4Cl_2

Band structure calculations for Ba_2Cu_3O_4Cl_2 within the local density approximation (LDA) are presented. The investigated compound is similar to the antiferromagnetic parent compounds of cuprate superconductors but contains additional Cu_B atoms in the planes. Within the LDA, metallic behavior is found with two bands crossing the Fermi surface (FS). These bands are built mainly from Cu 3d_{x^2-y^2} and O 2p_{x,y} orbitals, and a corresponding tight-binding (TB) model has been parameterized. All orbitals can be subdivided in two sets corresponding to the A- and B-subsystems, respectively, the coupling between which is found to be small. To describe the experimentally observed antiferromagnetic insulating state, we propose an extended Hubbard model with the derived TB parameters and local correlation terms characteristic for cuprates. Using the derived parameter set we calculate the exchange integrals for the Cu_3O_4 plane. The results are in quite reasonable agreement with the experimental values for the isostructural compound Sr_2Cu_3O_4Cl_2.Comment: 5 pages (2 tables included), 4 ps-figure

Anomalous Spin Dynamics observed by High Frequency ESR in Honeycomb Lattice Antiferromagnet InCu2/3V1/3O3

High-frequency ESR results on the S=1/2 Heisenberg hexagonal antiferromagnet InCu2/3V1/3O3 are reported. This compound appears to be a rare model substance for the honeycomb lattice antiferromagnet with very weak interlayer couplings. The high-temperature magnetic susceptibility can be interpreted by the S=1/2 honeycomb lattice antiferromagnet, and it shows a magnetic-order-like anomaly at TN=38 K. Although, the resonance field of our high-frequency ESR shows the typical behavior of the antiferromagnetic resonance, the linewidth of our high-frequency ESR continues to increase below TN, while it tends to decrease as the temperature in a conventional three-dimensional antiferromagnet decreases. In general, a honeycomb lattice antiferromagnet is expected to show a simple antiferromagnetic order similar to that of a square lattice antiferromagnet theoretically because both antiferromagnets are bipartite lattices. However, we suggest that the observed anomalous spin dynamics below TN is the peculiar feature of the honeycomb lattice antiferromagnet that is not observed in the square lattice antiferromagnet.Comment: 5 pages, 5 figure