1,730 research outputs found
PT-symmetry in honeycomb photonic lattices
We apply gain/loss to honeycomb photonic lattices and show that the
dispersion relation is identical to tachyons - particles with imaginary mass
that travel faster than the speed of light. This is accompanied by PT-symmetry
breaking in this structure. We further show that the PT-symmetry can be
restored by deforming the lattice
Carbon release by selective alloying of transition metal carbides
We have performed first principles density functional theory calculations on
TiC alloyed on the Ti sublattice with 3d transition metals ranging from Sc to
Zn. The theory is accompanied with experimental investigations, both as regards
materials synthesis as well as characterization. Our results show that by
dissolving a metal with a weak ability to form carbides, the stability of the
alloy is lowered and a driving force for the release of carbon from the carbide
is created. During thin film growth of a metal carbide this effect will favor
the formation of a nanocomposite with carbide grains in a carbon matrix. The
choice of alloying elements as well as their concentrations will affect the
relative amount of carbon in the carbide and in the carbon matrix. This can be
used to design the structure of nanocomposites and their physical and chemical
properties. One example of applications is as low-friction coatings. Of the
materials studied, we suggest the late 3d transition metals as the most
promising elements for this phenomenon, at least when alloying with TiC.Comment: 9 pages, 6 figure
Experimental Demonstration of Squeezed State Quantum Averaging
We propose and experimentally demonstrate a universal quantum averaging
process implementing the harmonic mean of quadrature variances. The harmonic
mean protocol can be used to efficiently stabilize a set of fragile squeezed
light sources with statistically fluctuating noise levels. The averaged
variances are prepared probabilistically by means of linear optical
interference and measurement induced conditioning. We verify that the
implemented harmonic mean outperforms the standard arithmetic mean strategy.
The effect of quantum averaging is experimentally tested both for uncorrelated
and partially correlated noise sources with sub-Poissonian shot noise or
super-Poissonian shot noise characteristics.Comment: 4 pages, 5 figure
A novel wear-resistant magnetic thin film material based on a nanocomposite alloy
In this study we report on the film growth and characterization of thin
(approximately 50 nm thick) Ti-Fe-C films deposited on amorphous quartz. The
experimental studies have been complemented by first principles density
functional theory (DFT) calculations. Upon annealing of as-prepared films, the
composition of the metastable Ti-Fe-C film changes. An iron-rich phase is first
formed close to the film surface, but with increasing annealing time this phase
is gradually displaced toward the film-substrate interface where its position
stabilizes. Both the magnetic ordering temperature and the saturation
magnetization changes significantly upon annealing. The DFT calculations show
that the critical temperature and the magnetic moment both increase with
increasing Fe and C-vacancy concentration. The formation of the metastable
iron-rich Ti-Fe-C compound is reflected in the strong increase of the magnetic
ordering temperature. Eventually, after enough annealing time (
minutes), nano-crystalline -Fe starts to precipitate and the amount and
size of these precipitates can be controlled by the annealing procedure; after
20 minutes of annealing, the experimental results indicate a nano-crystalline
iron-film embedded in a wear resistant TiC compound. This conclusion is further
supported by transmission electron microscopy studies on epitaxial Ti-Fe-C
films deposited on single crystalline MgO substrates where, upon annealing, an
iron film embedded in TiC is formed. Our results suggest that annealing of
metastable Ti-Fe-C films can be used as an efficient way of creating a
wear-resistant magnetic thin film material.Comment: 23 pages, 13 figure
Imaging a 1-electron InAs quantum dot in an InAs/InP nanowire
Nanowire heterostructures define high-quality few-electron quantum dots for
nanoelectronics, spintronics and quantum information processing. We use a
cooled scanning probe microscope (SPM) to image and control an InAs quantum dot
in an InAs/InP nanowire, using the tip as a movable gate. Images of dot
conductance vs. tip position at T = 4.2 K show concentric rings as electrons
are added, starting with the first electron. The SPM can locate a dot along a
nanowire and individually tune its charge, abilities that will be very useful
for the control of coupled nanowire dots
Control and femtosecond time-resolved imaging of torsion in a chiral molecule
We study how the combination of long and short laser pulses, can be used to
induce torsion in an axially chiral biphenyl derivative
(3,5-difluoro-3',5'-dibromo-4'-cyanobiphenyl). A long, with respect to the
molecular rotational periods, elliptically polarized laser pulse produces 3D
alignment of the molecules, and a linearly polarized short pulse initiates
torsion about the stereogenic axis. The torsional motion is monitored in
real-time by measuring the dihedral angle using femtosecond time-resolved
Coulomb explosion imaging. Within the first 4 picoseconds, torsion occurs with
a period of 1.25 picoseconds and an amplitude of 3 degrees in excellent
agreement with theoretical calculations. At larger times the quantum states of
the molecules describing the torsional motion dephase and an almost isotropic
distribution of the dihedral angle is measured. We demonstrate an original
application of covariance analysis of two-dimensional ion images to reveal
strong correlations between specific ejected ionic fragments from Coulomb
explosion. This technique strengthens our interpretation of the experimental
data.Comment: 11 pages, 9 figure
Temporal multimode storage of entangled photon pairs
Multiplexed quantum memories capable of storing and processing entangled
photons are essential for the development of quantum networks. In this context,
we demonstrate the simultaneous storage and retrieval of two entangled photons
inside a solid-state quantum memory and measure a temporal multimode capacity
of ten modes. This is achieved by producing two polarization entangled pairs
from parametric down conversion and mapping one photon of each pair onto a
rare-earth-ion doped (REID) crystal using the atomic frequency comb (AFC)
protocol. We develop a concept of indirect entanglement witnesses, which can be
used as Schmidt number witness, and we use it to experimentally certify the
presence of more than one entangled pair retrieved from the quantum memory. Our
work puts forward REID-AFC as a platform compatible with temporal multiplexing
of several entangled photon pairs along with a new entanglement certification
method useful for the characterisation of multiplexed quantum memories
Bubbling Orientifolds
We investigate a class of 1/2-BPS bubbling geometries associated to
orientifolds of type IIB string theory and thereby to excited states of the
SO(N)/Sp(N) N=4 supersymmetric Yang-Mills theory. The geometries are in
correspondence with free fermions moving in a harmonic oscillator potential on
the half-line. Branes wrapped on torsion cycles of these geometries are
identified in the fermi fluid description. Besides being of intrinsic interest,
these solutions may also occur as local geometries in flux compactifications
where orientifold planes are present to ensure global charge cancellation. We
comment on the extension of this procedure to M-theory orientifolds.Comment: 25 pages, 11 figures. v2: few references adde
Results of a European interlaboratory comparison on gross alpha/beta activity determination in drinking water
An interlaboratory comparison was organised by the Institute for Reference Materials and Measurements (JRC-IRMM) among environmental radioactivity monitoring laboratories for the determination of gross alpha/beta activity concentration in drinking water. Four independent standard methods were used for the determination of the reference values of three different water samples. The performance of participating laboratories was evaluated with respect to the reference values using relative deviations. Sample preparation and measurement methods used by the participating laboratories are described in detail, in particular in the view of method-dependency of the results. Many of the participants’ results deviate by more than two orders of magnitude from the reference values regardless of the techniques used. This suggests that gross methods need revision.JRC.D.4-Standards for Nuclear Safety, Security and Safeguard
Molecular mechanism for rapid autoxidation in alpha-pinene ozonolysis
Aerosol affects Earth's climate and the health of its inhabitants. A major contributor to aerosol formation is the oxidation of volatile organic compounds. Monoterpenes are an important class of volatile organic compounds, and recent research demonstrate that they can be converted to low-volatility aerosol precursors on sub-second timescales following a single oxidant attack. The alpha -pinene + O-3 system is particularly efficient in this regard. However, the actual mechanism behind this conversion is not understood. The key challenge is the steric strain created by the cyclobutyl ring in the oxidation products. This strain hinders subsequent unimolecular hydrogen-shift reactions essential for lowering volatility. Using quantum chemical calculations and targeted experiments, we show that the excess energy from the initial ozonolysis reaction can lead to novel oxidation intermediates without steric strain, allowing the rapid formation of products with up to 8 oxygen atoms. This is likely a key route for atmospheric organic aerosol formation. Oxidation of volatile organic compounds leads to aerosol formation in the atmosphere, but the mechanism of some fast reactions is still unclear. The authors, using quantum chemical modelling and experiments, reveal that in key monoterpenes the cyclobutyl ring that would hinder the reactivity is broken in the early exothermic steps of the reaction.Peer reviewe
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